Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries

Engineering design of battery configurations and new battery system development are alternative approaches to achieve high performance batteries. A novel flexible and ultra-light graphite anode is fabricated by simple friction drawing on filter paper with a commercial 8B pencil. Compared with the tr...

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Main Authors: Zhixin Tai, Yajie Liu, Qing Zhang, Tengfei Zhou, Zaiping Guo, Hua Kun Liu, Shi Xue Dou
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2017-07-01
Series:Green Energy & Environment
Online Access:http://www.sciencedirect.com/science/article/pii/S2468025717300328
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author Zhixin Tai
Yajie Liu
Qing Zhang
Tengfei Zhou
Zaiping Guo
Hua Kun Liu
Shi Xue Dou
author_facet Zhixin Tai
Yajie Liu
Qing Zhang
Tengfei Zhou
Zaiping Guo
Hua Kun Liu
Shi Xue Dou
author_sort Zhixin Tai
collection DOAJ
description Engineering design of battery configurations and new battery system development are alternative approaches to achieve high performance batteries. A novel flexible and ultra-light graphite anode is fabricated by simple friction drawing on filter paper with a commercial 8B pencil. Compared with the traditional anode using copper foil as current collector, this innovative current-collector-free design presents capacity improvement of over 200% by reducing the inert weight of the electrode. The as-prepared pencil-trace electrode exhibits excellent rate performance in potassium-ion batteries (KIBs), significantly better than in lithium-ion batteries (LIBs), with capacity retention of 66% for the KIB vs. 28% for the LIB from 0.1 to 0.5 A gâ1. It also shows a high reversible capacity of â¼230 mAh gâ1 at 0.2 A gâ1, 75% capacity retention over 350 cycles at 0.4 A gâ1and the highest rate performance (based on the total electrode weight) among graphite electrodes for K+ storage reported so far. Keywords: Current-collector-free, Flexible pencil-trace electrode, Potassium-ion battery, Lithium-ion battery, Layer-by-layer interconnected architecture
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publisher KeAi Communications Co., Ltd.
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spelling doaj.art-1d4c12637d7b4de19e362999943f768f2022-12-21T22:05:02ZengKeAi Communications Co., Ltd.Green Energy & Environment2468-02572017-07-0123278284Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteriesZhixin Tai0Yajie Liu1Qing Zhang2Tengfei Zhou3Zaiping Guo4Hua Kun Liu5Shi Xue Dou6Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaInstitute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaInstitute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaInstitute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaInstitute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, Australia; School of Mechanical, Materials and Mechatronics Engineering, University of Wollongong, North Wollongong, NSW 2500, Australia; Corresponding author. Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500. Australia.Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaInstitute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong, Innovation Campus, North Wollongong, NSW 2500, AustraliaEngineering design of battery configurations and new battery system development are alternative approaches to achieve high performance batteries. A novel flexible and ultra-light graphite anode is fabricated by simple friction drawing on filter paper with a commercial 8B pencil. Compared with the traditional anode using copper foil as current collector, this innovative current-collector-free design presents capacity improvement of over 200% by reducing the inert weight of the electrode. The as-prepared pencil-trace electrode exhibits excellent rate performance in potassium-ion batteries (KIBs), significantly better than in lithium-ion batteries (LIBs), with capacity retention of 66% for the KIB vs. 28% for the LIB from 0.1 to 0.5 A gâ1. It also shows a high reversible capacity of â¼230 mAh gâ1 at 0.2 A gâ1, 75% capacity retention over 350 cycles at 0.4 A gâ1and the highest rate performance (based on the total electrode weight) among graphite electrodes for K+ storage reported so far. Keywords: Current-collector-free, Flexible pencil-trace electrode, Potassium-ion battery, Lithium-ion battery, Layer-by-layer interconnected architecturehttp://www.sciencedirect.com/science/article/pii/S2468025717300328
spellingShingle Zhixin Tai
Yajie Liu
Qing Zhang
Tengfei Zhou
Zaiping Guo
Hua Kun Liu
Shi Xue Dou
Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
Green Energy & Environment
title Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
title_full Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
title_fullStr Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
title_full_unstemmed Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
title_short Ultra-light and flexible pencil-trace anode for high performance potassium-ion and lithium-ion batteries
title_sort ultra light and flexible pencil trace anode for high performance potassium ion and lithium ion batteries
url http://www.sciencedirect.com/science/article/pii/S2468025717300328
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