Oxidation of propene from air by atmospheric plasma-catalytic hybrid system

The pulsed dielectric barrier discharge (DBD) combined with the palladium supported on alumina beads, was investigated for propene (C3H6) removal from air. The effects of thermal-catalysis, plasma-catalysis (in-plasma catalysis and post-plasma catalysis), and plasma-alone on the propene removal were...

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Main Authors: Pham Thien Huu, Bui Ha Manh, Khacef Ahmed
Format: Article
Language:English
Published: Serbian Chemical Society 2018-01-01
Series:Journal of the Serbian Chemical Society
Subjects:
Online Access:http://www.doiserbia.nb.rs/img/doi/0352-5139/2018/0352-51391800012P.pdf
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author Pham Thien Huu
Bui Ha Manh
Khacef Ahmed
author_facet Pham Thien Huu
Bui Ha Manh
Khacef Ahmed
author_sort Pham Thien Huu
collection DOAJ
description The pulsed dielectric barrier discharge (DBD) combined with the palladium supported on alumina beads, was investigated for propene (C3H6) removal from air. The effects of thermal-catalysis, plasma-catalysis (in-plasma catalysis and post-plasma catalysis), and plasma-alone on the propene removal were compared. Results are presented in the terms of C3H6 removal efficiency, energy consumption, and by-products production. Temperature dependence studies (20–250°C) show that in all conditions of input plasma energy density explored (23–148 J L-1), the plasma-catalysis systems exhibit better propene conversion efficiencies than the thermal catalysis at low temperature (60% at 20°C). Plasma-alone treatment has a similar effectiveness compared to plasma-catalysis at room temperature, but it leads to the formation of high by-products concentrations. It appears that in the plasma-catalyst system, C3H6 removal was the most efficient, whatever was the configuration used, and it was helpful to minimize by-products formation.
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spelling doaj.art-1d763fb96123458687c2488780ebc15e2022-12-21T19:10:53ZengSerbian Chemical SocietyJournal of the Serbian Chemical Society0352-51391820-74212018-01-0183564164910.2298/JSC171014012P0352-51391800012POxidation of propene from air by atmospheric plasma-catalytic hybrid systemPham Thien Huu0Bui Ha Manh1Khacef Ahmed2Vietnam Academy of Science and Technology, Institute of Applied Material Science, Ho Chi Minh City, VietnamSai Gon university, Department of Environmental Sciences, Ho Chi Minh City, VietnamUniversity of Orleans, Research team in GREMI Laboratory, the National centre for Scientific research, Orleans Cedex, FranceThe pulsed dielectric barrier discharge (DBD) combined with the palladium supported on alumina beads, was investigated for propene (C3H6) removal from air. The effects of thermal-catalysis, plasma-catalysis (in-plasma catalysis and post-plasma catalysis), and plasma-alone on the propene removal were compared. Results are presented in the terms of C3H6 removal efficiency, energy consumption, and by-products production. Temperature dependence studies (20–250°C) show that in all conditions of input plasma energy density explored (23–148 J L-1), the plasma-catalysis systems exhibit better propene conversion efficiencies than the thermal catalysis at low temperature (60% at 20°C). Plasma-alone treatment has a similar effectiveness compared to plasma-catalysis at room temperature, but it leads to the formation of high by-products concentrations. It appears that in the plasma-catalyst system, C3H6 removal was the most efficient, whatever was the configuration used, and it was helpful to minimize by-products formation.http://www.doiserbia.nb.rs/img/doi/0352-5139/2018/0352-51391800012P.pdfNon-thermal plasmaC3H6 oxidationpalladium catalyst
spellingShingle Pham Thien Huu
Bui Ha Manh
Khacef Ahmed
Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
Journal of the Serbian Chemical Society
Non-thermal plasma
C3H6 oxidation
palladium catalyst
title Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
title_full Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
title_fullStr Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
title_full_unstemmed Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
title_short Oxidation of propene from air by atmospheric plasma-catalytic hybrid system
title_sort oxidation of propene from air by atmospheric plasma catalytic hybrid system
topic Non-thermal plasma
C3H6 oxidation
palladium catalyst
url http://www.doiserbia.nb.rs/img/doi/0352-5139/2018/0352-51391800012P.pdf
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AT buihamanh oxidationofpropenefromairbyatmosphericplasmacatalytichybridsystem
AT khacefahmed oxidationofpropenefromairbyatmosphericplasmacatalytichybridsystem