Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals

Abstract Cherenkov radiation (CR) excited by fast charges can serve as on-chip light sources with a nanoscale footprint and broad frequency range. The reversed CR, which usually occurs in media with the negative refractive index or negative group-velocity dispersion, is highly desired because it can...

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Main Authors: Xiangdong Guo, Chenchen Wu, Shu Zhang, Debo Hu, Shunping Zhang, Qiao Jiang, Xiaokang Dai, Yu Duan, Xiaoxia Yang, Zhipei Sun, Shuang Zhang, Hongxing Xu, Qing Dai
Format: Article
Language:English
Published: Nature Portfolio 2023-05-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-37923-w
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author Xiangdong Guo
Chenchen Wu
Shu Zhang
Debo Hu
Shunping Zhang
Qiao Jiang
Xiaokang Dai
Yu Duan
Xiaoxia Yang
Zhipei Sun
Shuang Zhang
Hongxing Xu
Qing Dai
author_facet Xiangdong Guo
Chenchen Wu
Shu Zhang
Debo Hu
Shunping Zhang
Qiao Jiang
Xiaokang Dai
Yu Duan
Xiaoxia Yang
Zhipei Sun
Shuang Zhang
Hongxing Xu
Qing Dai
author_sort Xiangdong Guo
collection DOAJ
description Abstract Cherenkov radiation (CR) excited by fast charges can serve as on-chip light sources with a nanoscale footprint and broad frequency range. The reversed CR, which usually occurs in media with the negative refractive index or negative group-velocity dispersion, is highly desired because it can effectively separate the radiated light from fast charges thanks to the obtuse radiation angle. However, reversed CR at the mid-infrared remains challenging due to the significant loss of conventional artificial structures. Here we observe mid-infrared analogue polaritonic reversed CR in a natural van der Waals (vdW) material (i.e., α-MoO3), whose hyperbolic phonon polaritons exhibit negative group velocity. Further, the real-space image results of analogue polaritonic reversed CR indicate that the radiation distributions and angles are closely related to the in-plane isofrequency contours of α-MoO3, which can be further tuned in the heterostructures based on α-MoO3. This work demonstrates that natural vdW heterostructures can be used as a promising platform of reversed CR to design on-chip mid-infrared nano-light sources.
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spelling doaj.art-21c1c228611e41fc94900c7d5540d88c2023-05-07T11:18:19ZengNature PortfolioNature Communications2041-17232023-05-011411710.1038/s41467-023-37923-wMid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystalsXiangdong Guo0Chenchen Wu1Shu Zhang2Debo Hu3Shunping Zhang4Qiao Jiang5Xiaokang Dai6Yu Duan7Xiaoxia Yang8Zhipei Sun9Shuang Zhang10Hongxing Xu11Qing Dai12CAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologySchool of Physics and Technology, Center for Nanoscience and Nanotechnology, and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan UniversityCollege of Physics, Chongqing UniversityCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyDepartment of Electronics and Nanoengineering and QTF Centre of Excellence, Department of Applied Physics, Aalto UniversityDepartment of Physics, University of Hong KongSchool of Physics and Technology, Center for Nanoscience and Nanotechnology, and Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, Wuhan UniversityCAS Key Laboratory of Nanophotonic Materials and Devices, CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and TechnologyAbstract Cherenkov radiation (CR) excited by fast charges can serve as on-chip light sources with a nanoscale footprint and broad frequency range. The reversed CR, which usually occurs in media with the negative refractive index or negative group-velocity dispersion, is highly desired because it can effectively separate the radiated light from fast charges thanks to the obtuse radiation angle. However, reversed CR at the mid-infrared remains challenging due to the significant loss of conventional artificial structures. Here we observe mid-infrared analogue polaritonic reversed CR in a natural van der Waals (vdW) material (i.e., α-MoO3), whose hyperbolic phonon polaritons exhibit negative group velocity. Further, the real-space image results of analogue polaritonic reversed CR indicate that the radiation distributions and angles are closely related to the in-plane isofrequency contours of α-MoO3, which can be further tuned in the heterostructures based on α-MoO3. This work demonstrates that natural vdW heterostructures can be used as a promising platform of reversed CR to design on-chip mid-infrared nano-light sources.https://doi.org/10.1038/s41467-023-37923-w
spellingShingle Xiangdong Guo
Chenchen Wu
Shu Zhang
Debo Hu
Shunping Zhang
Qiao Jiang
Xiaokang Dai
Yu Duan
Xiaoxia Yang
Zhipei Sun
Shuang Zhang
Hongxing Xu
Qing Dai
Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
Nature Communications
title Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
title_full Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
title_fullStr Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
title_full_unstemmed Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
title_short Mid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
title_sort mid infrared analogue polaritonic reversed cherenkov radiation in natural anisotropic crystals
url https://doi.org/10.1038/s41467-023-37923-w
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