Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations

To investigate interactions between aerosols and clouds, the size and number concentrations of the cloud condensation nuclei (CCN) and the cloud droplets (CDs) were measured at the summit of Mt. Fuji (altitude 3776 m), Japan. The CCN number concentrations (<i>N</i><sub>CCN</sub&...

Full description

Bibliographic Details
Main Authors: Yoko Iwamoto, Ayami Watanabe, Ryota Kataoka, Mitsuo Uematsu, Kazuhiko Miura
Format: Article
Language:English
Published: MDPI AG 2021-09-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/11/18/8439
_version_ 1797520372402225152
author Yoko Iwamoto
Ayami Watanabe
Ryota Kataoka
Mitsuo Uematsu
Kazuhiko Miura
author_facet Yoko Iwamoto
Ayami Watanabe
Ryota Kataoka
Mitsuo Uematsu
Kazuhiko Miura
author_sort Yoko Iwamoto
collection DOAJ
description To investigate interactions between aerosols and clouds, the size and number concentrations of the cloud condensation nuclei (CCN) and the cloud droplets (CDs) were measured at the summit of Mt. Fuji (altitude 3776 m), Japan. The CCN number concentrations (<i>N</i><sub>CCN</sub>) are significantly higher in continental air masses than in air masses from the Pacific Ocean. The hygroscopicity parameter <i>κ</i> did not change much for different air mass origins, indicating that aerosol particles in the free troposphere are well mixed. Based on the CD number concentrations (<i>N</i><sub>CD</sub>), the degree of supersaturation in the ambient air during the cloud-shrouded period was estimated to be 0.15% (25th percentile) to 0.44% (75th percentile). To evaluate factors influencing the <i>N</i><sub>CD</sub>, measured <i>N</i><sub>CD</sub> were compared to ones calculated based on the Köhler theory using aerosol number size distributions, <i>κ</i>, and the degree of supersaturation. The results showed that <i>N</i><sub>CD</sub> could not be reproduced satisfyingly when the mean number size distribution or the mean effective supersaturation were used for the calculation. This study highlights the importance of obtaining information about the degree of supersaturation to predict <i>N</i><sub>CD</sub> in the atmosphere.
first_indexed 2024-03-10T07:55:50Z
format Article
id doaj.art-2239a3d552344ceeb4f67a3d7d483c84
institution Directory Open Access Journal
issn 2076-3417
language English
last_indexed 2024-03-10T07:55:50Z
publishDate 2021-09-01
publisher MDPI AG
record_format Article
series Applied Sciences
spelling doaj.art-2239a3d552344ceeb4f67a3d7d483c842023-11-22T11:52:44ZengMDPI AGApplied Sciences2076-34172021-09-011118843910.3390/app11188439Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number ConcentrationsYoko Iwamoto0Ayami Watanabe1Ryota Kataoka2Mitsuo Uematsu3Kazuhiko Miura4Graduate School of Integrated Sciences for Life, Hiroshima University, Higashi-Hiroshima 739-8521, JapanGraduate School of Science, Tokyo University of Science, Tokyo 162-8601, JapanGraduate School of Science, Tokyo University of Science, Tokyo 162-8601, JapanAtmosphere and Ocean Research Institute, The University of Tokyo, Kashiwa 277-8564, JapanFaculty of Science Division I, Tokyo University of Science, Tokyo 162-8601, JapanTo investigate interactions between aerosols and clouds, the size and number concentrations of the cloud condensation nuclei (CCN) and the cloud droplets (CDs) were measured at the summit of Mt. Fuji (altitude 3776 m), Japan. The CCN number concentrations (<i>N</i><sub>CCN</sub>) are significantly higher in continental air masses than in air masses from the Pacific Ocean. The hygroscopicity parameter <i>κ</i> did not change much for different air mass origins, indicating that aerosol particles in the free troposphere are well mixed. Based on the CD number concentrations (<i>N</i><sub>CD</sub>), the degree of supersaturation in the ambient air during the cloud-shrouded period was estimated to be 0.15% (25th percentile) to 0.44% (75th percentile). To evaluate factors influencing the <i>N</i><sub>CD</sub>, measured <i>N</i><sub>CD</sub> were compared to ones calculated based on the Köhler theory using aerosol number size distributions, <i>κ</i>, and the degree of supersaturation. The results showed that <i>N</i><sub>CD</sub> could not be reproduced satisfyingly when the mean number size distribution or the mean effective supersaturation were used for the calculation. This study highlights the importance of obtaining information about the degree of supersaturation to predict <i>N</i><sub>CD</sub> in the atmosphere.https://www.mdpi.com/2076-3417/11/18/8439cloud condensation nucleihigh alpine sitesize distributionhygroscopicity parameterwater vapor supersaturation
spellingShingle Yoko Iwamoto
Ayami Watanabe
Ryota Kataoka
Mitsuo Uematsu
Kazuhiko Miura
Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
Applied Sciences
cloud condensation nuclei
high alpine site
size distribution
hygroscopicity parameter
water vapor supersaturation
title Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
title_full Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
title_fullStr Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
title_full_unstemmed Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
title_short Aerosol–Cloud Interaction at the Summit of Mt. Fuji, Japan: Factors Influencing Cloud Droplet Number Concentrations
title_sort aerosol cloud interaction at the summit of mt fuji japan factors influencing cloud droplet number concentrations
topic cloud condensation nuclei
high alpine site
size distribution
hygroscopicity parameter
water vapor supersaturation
url https://www.mdpi.com/2076-3417/11/18/8439
work_keys_str_mv AT yokoiwamoto aerosolcloudinteractionatthesummitofmtfujijapanfactorsinfluencingclouddropletnumberconcentrations
AT ayamiwatanabe aerosolcloudinteractionatthesummitofmtfujijapanfactorsinfluencingclouddropletnumberconcentrations
AT ryotakataoka aerosolcloudinteractionatthesummitofmtfujijapanfactorsinfluencingclouddropletnumberconcentrations
AT mitsuouematsu aerosolcloudinteractionatthesummitofmtfujijapanfactorsinfluencingclouddropletnumberconcentrations
AT kazuhikomiura aerosolcloudinteractionatthesummitofmtfujijapanfactorsinfluencingclouddropletnumberconcentrations