Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment

Two different types of graphene materials were used as functional nanofillers for the mechanical and tribological improvement of silicon carbide/graphene nanocomposites. On the one hand is thermally reduced graphite oxide (TRGO) reduced at three different temperatures, and on the other hand is graph...

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Main Authors: Bernadette Schlüter, Christian Schröder, Wenli Zhang, Rolf Mülhaupt, Ulrich Degenhardt, Richard Sedlák, Ján Dusza, Katalin Balázsi, Csaba Balázsi, Andreas Kailer
Format: Article
Language:English
Published: MDPI AG 2022-11-01
Series:Materials
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Online Access:https://www.mdpi.com/1996-1944/15/21/7755
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author Bernadette Schlüter
Christian Schröder
Wenli Zhang
Rolf Mülhaupt
Ulrich Degenhardt
Richard Sedlák
Ján Dusza
Katalin Balázsi
Csaba Balázsi
Andreas Kailer
author_facet Bernadette Schlüter
Christian Schröder
Wenli Zhang
Rolf Mülhaupt
Ulrich Degenhardt
Richard Sedlák
Ján Dusza
Katalin Balázsi
Csaba Balázsi
Andreas Kailer
author_sort Bernadette Schlüter
collection DOAJ
description Two different types of graphene materials were used as functional nanofillers for the mechanical and tribological improvement of silicon carbide/graphene nanocomposites. On the one hand is thermally reduced graphite oxide (TRGO) reduced at three different temperatures, and on the other hand is graphene made of three different organic precursors, which were directly coated on silicon carbide (SiC) platelets (GSiC). Additionally, benchmark materials were also used as carbon fillers. The SiC/graphene nanocomposites with 2 wt% filler content were manufactured by pressureless sintering (PLS). Some composites were produced with higher graphene contents of 4% and 8% and sintered by spark plasma sintering (SPS). Microstructural analyses were conducted using scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Underwater lubrication, the SP sintered TRGO and GSiC materials with high graphene content have shown the most promising tribological performance. Furthermore, the reduced size of the homogeneously distributed nanoparticles promotes the formation of surface states, which improve the friction and wear properties.
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spelling doaj.art-22c3a7b1e85a47c7b39d92590a9004fa2023-11-24T05:40:15ZengMDPI AGMaterials1996-19442022-11-011521775510.3390/ma15217755Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous EnvironmentBernadette Schlüter0Christian Schröder1Wenli Zhang2Rolf Mülhaupt3Ulrich Degenhardt4Richard Sedlák5Ján Dusza6Katalin Balázsi7Csaba Balázsi8Andreas Kailer9Fraunhofer Institute for Mechanics of Materials IWM, Woehlerstr. 11, 79108 Freiburg, GermanyFraunhofer Institute for Mechanics of Materials IWM, Woehlerstr. 11, 79108 Freiburg, GermanyFreiburg Materials Research Center (FMF), Institute for Macromolecular Chemistry, University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, GermanyFreiburg Materials Research Center (FMF), Institute for Macromolecular Chemistry, University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, GermanyQSIL Ingenieurkeramik GmbH, Rauenstein, Gewerbepark 11, 96528 Frankenblick, GermanyDivision of Ceramic and Non-Metallic Systems, Institute of Materials Research, Slovak Academy of Sciences, Watsonova 47, 040 01 Košice, SlovakiaDivision of Ceramic and Non-Metallic Systems, Institute of Materials Research, Slovak Academy of Sciences, Watsonova 47, 040 01 Košice, SlovakiaCentre for Energy Research, Institute for Technical Physics and Materials Science, Hungarian Academy of Sciences, 1121 Konkoly-Thege Miklos Str. 29-33, H-1525 Budapest, HungaryCentre for Energy Research, Institute for Technical Physics and Materials Science, Hungarian Academy of Sciences, 1121 Konkoly-Thege Miklos Str. 29-33, H-1525 Budapest, HungaryFraunhofer Institute for Mechanics of Materials IWM, Woehlerstr. 11, 79108 Freiburg, GermanyTwo different types of graphene materials were used as functional nanofillers for the mechanical and tribological improvement of silicon carbide/graphene nanocomposites. On the one hand is thermally reduced graphite oxide (TRGO) reduced at three different temperatures, and on the other hand is graphene made of three different organic precursors, which were directly coated on silicon carbide (SiC) platelets (GSiC). Additionally, benchmark materials were also used as carbon fillers. The SiC/graphene nanocomposites with 2 wt% filler content were manufactured by pressureless sintering (PLS). Some composites were produced with higher graphene contents of 4% and 8% and sintered by spark plasma sintering (SPS). Microstructural analyses were conducted using scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Underwater lubrication, the SP sintered TRGO and GSiC materials with high graphene content have shown the most promising tribological performance. Furthermore, the reduced size of the homogeneously distributed nanoparticles promotes the formation of surface states, which improve the friction and wear properties.https://www.mdpi.com/1996-1944/15/21/7755silicon carbidegraphene nanocompositegraphene coatingspark plasma sinteringfrictionwear
spellingShingle Bernadette Schlüter
Christian Schröder
Wenli Zhang
Rolf Mülhaupt
Ulrich Degenhardt
Richard Sedlák
Ján Dusza
Katalin Balázsi
Csaba Balázsi
Andreas Kailer
Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
Materials
silicon carbide
graphene nanocomposite
graphene coating
spark plasma sintering
friction
wear
title Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
title_full Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
title_fullStr Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
title_full_unstemmed Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
title_short Influence of Graphene Type and Content on Friction and Wear of Silicon Carbide/Graphene Nanocomposites in Aqueous Environment
title_sort influence of graphene type and content on friction and wear of silicon carbide graphene nanocomposites in aqueous environment
topic silicon carbide
graphene nanocomposite
graphene coating
spark plasma sintering
friction
wear
url https://www.mdpi.com/1996-1944/15/21/7755
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