Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system

To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum yields are enhanced as compared to the single band-gap solar cell...

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Main Authors: Shun-Cai Zhao, Jing-Yi Chen
Format: Article
Language:English
Published: IOP Publishing 2019-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/ab473a
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author Shun-Cai Zhao
Jing-Yi Chen
author_facet Shun-Cai Zhao
Jing-Yi Chen
author_sort Shun-Cai Zhao
collection DOAJ
description To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum yields are enhanced as compared to the single band-gap solar cell, and the photo-to-charge efficiencies are larger than Shockley and Queisser efficiency in the same absorbed spectrum. What is more, at the room temperature the efficiency limits are well beyond 63% achieved by Luque and Marti (1997 Phys. Rev. Lett. 78 5014) due to absorbing the low-energy photons via two sub-bands in this proposed photocell system. The achievements may reveal a novel theoretical approach to enhance the QD photocell performance modeled a multi-level absorbing photons system.
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spelling doaj.art-230611f65da14984b81d5e1c3a4fc6262023-08-08T15:24:00ZengIOP PublishingNew Journal of Physics1367-26302019-01-01211010301510.1088/1367-2630/ab473aEnhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level systemShun-Cai Zhao0https://orcid.org/0000-0003-1565-6208Jing-Yi Chen1Department of Physics, Faculty of Science, Kunming University of Science and Technology , Kunming, 650500, People's Republic of ChinaDepartment of Physics, Faculty of Science, Kunming University of Science and Technology , Kunming, 650500, People's Republic of ChinaTo absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum yields are enhanced as compared to the single band-gap solar cell, and the photo-to-charge efficiencies are larger than Shockley and Queisser efficiency in the same absorbed spectrum. What is more, at the room temperature the efficiency limits are well beyond 63% achieved by Luque and Marti (1997 Phys. Rev. Lett. 78 5014) due to absorbing the low-energy photons via two sub-bands in this proposed photocell system. The achievements may reveal a novel theoretical approach to enhance the QD photocell performance modeled a multi-level absorbing photons system.https://doi.org/10.1088/1367-2630/ab473aquantum dot photocell modeled by a multi-level systemphoto-to-charge efficiencylow-energy photonsquantum yields
spellingShingle Shun-Cai Zhao
Jing-Yi Chen
Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
New Journal of Physics
quantum dot photocell modeled by a multi-level system
photo-to-charge efficiency
low-energy photons
quantum yields
title Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
title_full Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
title_fullStr Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
title_full_unstemmed Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
title_short Enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi-level system
title_sort enhanced quantum yields and efficiency in a quantum dot photocell modeled by a multi level system
topic quantum dot photocell modeled by a multi-level system
photo-to-charge efficiency
low-energy photons
quantum yields
url https://doi.org/10.1088/1367-2630/ab473a
work_keys_str_mv AT shuncaizhao enhancedquantumyieldsandefficiencyinaquantumdotphotocellmodeledbyamultilevelsystem
AT jingyichen enhancedquantumyieldsandefficiencyinaquantumdotphotocellmodeledbyamultilevelsystem