The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules

In this study, Sylgard 184 silicone rubber (SylSR) matrix composites with shear thickening fluid (STF) microcapsules (SylSR/STF) were fabricated. Their mechanical behaviors were characterized by dynamic thermo-mechanical analysis (DMA) and quasi-static compression. Their damping properties increased...

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Main Authors: Chun Wei, Xiaofei Hao, Chaoying Mao, Fachun Zhong, Zhongping Liu
Format: Article
Language:English
Published: MDPI AG 2023-06-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/15/12/2704
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author Chun Wei
Xiaofei Hao
Chaoying Mao
Fachun Zhong
Zhongping Liu
author_facet Chun Wei
Xiaofei Hao
Chaoying Mao
Fachun Zhong
Zhongping Liu
author_sort Chun Wei
collection DOAJ
description In this study, Sylgard 184 silicone rubber (SylSR) matrix composites with shear thickening fluid (STF) microcapsules (SylSR/STF) were fabricated. Their mechanical behaviors were characterized by dynamic thermo-mechanical analysis (DMA) and quasi-static compression. Their damping properties increased with the addition ofSTF into the SR in DMA tests and the SylSR/STF composites presented decreased stiffness and an obvious positive strain rate effect in the quasi-static compression test. Moreover, the impact resistance behavior of the SylSR/STF composites was tested by the drop hammer impact test. The addition of STF enhanced the impact protective performance of silicone rubber, and the impact resistance increased with the increase of STF content, which should be ascribed to the shear thickening and energy absorption of STF microcapsules in the composites. Meanwhile, in another matrix, hot vulcanized silicone rubber (HTVSR) with a mechanical strength higher than Sylgard 184, the impact resistance capacity of its composite with STF (HTVSR/STF) was also examined by the drop hammer impact test. It is interesting to note that the strength of the SR matrix obviously influenced the enhancement effect of STF on the impact resistance of SR. The stronger the strength of SR, the better the effect of STF on improving the impact protective performance of SR. This study not only provides a new method for packaging STF and improving the impact resistance behavior of SR, but is also beneficial for the design of STF-related protective functional materials and structures.
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spelling doaj.art-23e5c0ec68474615ac465bac760238ce2023-11-18T12:13:34ZengMDPI AGPolymers2073-43602023-06-011512270410.3390/polym15122704The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid MicrocapsulesChun Wei0Xiaofei Hao1Chaoying Mao2Fachun Zhong3Zhongping Liu4Institute of Chemical Materials, China Academy of Engineering Physics (CAEP), Mianyang 621900, ChinaInstitute of Chemical Materials, China Academy of Engineering Physics (CAEP), Mianyang 621900, ChinaInstitute of Chemical Materials, China Academy of Engineering Physics (CAEP), Mianyang 621900, ChinaInstitute of Chemical Materials, China Academy of Engineering Physics (CAEP), Mianyang 621900, ChinaInstitute of Chemical Materials, China Academy of Engineering Physics (CAEP), Mianyang 621900, ChinaIn this study, Sylgard 184 silicone rubber (SylSR) matrix composites with shear thickening fluid (STF) microcapsules (SylSR/STF) were fabricated. Their mechanical behaviors were characterized by dynamic thermo-mechanical analysis (DMA) and quasi-static compression. Their damping properties increased with the addition ofSTF into the SR in DMA tests and the SylSR/STF composites presented decreased stiffness and an obvious positive strain rate effect in the quasi-static compression test. Moreover, the impact resistance behavior of the SylSR/STF composites was tested by the drop hammer impact test. The addition of STF enhanced the impact protective performance of silicone rubber, and the impact resistance increased with the increase of STF content, which should be ascribed to the shear thickening and energy absorption of STF microcapsules in the composites. Meanwhile, in another matrix, hot vulcanized silicone rubber (HTVSR) with a mechanical strength higher than Sylgard 184, the impact resistance capacity of its composite with STF (HTVSR/STF) was also examined by the drop hammer impact test. It is interesting to note that the strength of the SR matrix obviously influenced the enhancement effect of STF on the impact resistance of SR. The stronger the strength of SR, the better the effect of STF on improving the impact protective performance of SR. This study not only provides a new method for packaging STF and improving the impact resistance behavior of SR, but is also beneficial for the design of STF-related protective functional materials and structures.https://www.mdpi.com/2073-4360/15/12/2704shear thickening fluidsilicone rubbermicrocapsuleimpact resistance behavior
spellingShingle Chun Wei
Xiaofei Hao
Chaoying Mao
Fachun Zhong
Zhongping Liu
The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
Polymers
shear thickening fluid
silicone rubber
microcapsule
impact resistance behavior
title The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
title_full The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
title_fullStr The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
title_full_unstemmed The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
title_short The Mechanical Properties of Silicone Rubber Composites with Shear Thickening Fluid Microcapsules
title_sort mechanical properties of silicone rubber composites with shear thickening fluid microcapsules
topic shear thickening fluid
silicone rubber
microcapsule
impact resistance behavior
url https://www.mdpi.com/2073-4360/15/12/2704
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