A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau

The impacts of human activities on Zoige peatlands are poorly documented. We determined the concentrations and accumulation rates of As and Hg in a <sup>210</sup>Pb-dated peat profile collected from this area and analyzed the correlations between accumulation rates of both As and Hg and...

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Main Authors: Xuhui Chen, Qianqian Su, Huai Chen, Dan Xue
Format: Article
Language:English
Published: MDPI AG 2021-11-01
Series:Land
Subjects:
Online Access:https://www.mdpi.com/2073-445X/10/11/1241
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author Xuhui Chen
Qianqian Su
Huai Chen
Dan Xue
author_facet Xuhui Chen
Qianqian Su
Huai Chen
Dan Xue
author_sort Xuhui Chen
collection DOAJ
description The impacts of human activities on Zoige peatlands are poorly documented. We determined the concentrations and accumulation rates of As and Hg in a <sup>210</sup>Pb-dated peat profile collected from this area and analyzed the correlations between accumulation rates of both As and Hg and other physicochemical properties. To reconstruct recent conditions of As and Hg, we analyzed peat sediments of Re’er Dam peatland in Zoige using <sup>210</sup>Pb and <sup>137</sup>Cs dating technologies. The concentrations of total As (86.38 to 174.21 μg kg<sup>−1</sup>) and Hg (7.30 to 32.13 μg kg<sup>−1</sup>) in the peat profile clearly increased after the first industrial revolution. From AD 1824 to AD 2010, the average accumulation rates were 129.77 μg m<sup>−2</sup> yr<sup>−1</sup> for As and 18.24 μg m<sup>−2</sup> yr<sup>−1</sup> for Hg. Based on our results, anthropogenic emissions significantly affected the atmospheric fluxes of As and Hg throughout the past 200 years, and As was also likely to be affected by other factors than atmospheric deposition, which needs further identification by future studies. The historical variations in As and Hg concentrations in Re’er Dam peatland in Zoige mirror the industrial development of China.
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spelling doaj.art-243ce3835bfe493fb8ecc5df1d4003732023-11-23T00:02:18ZengMDPI AGLand2073-445X2021-11-011011124110.3390/land10111241A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet PlateauXuhui Chen0Qianqian Su1Huai Chen2Dan Xue3CAS Key Laboratory of Mountain Ecological Restoration and Bioresource Utilization & Ecological Restoration Biodiversity Conservation Key Laboratory of Sichuan Province, Chengdu Institute of Biology, Chinese Academy of Sciences, Chengdu 610041, ChinaCAS Key Laboratory of Mountain Ecological Restoration and Bioresource Utilization & Ecological Restoration Biodiversity Conservation Key Laboratory of Sichuan Province, Chengdu Institute of Biology, Chinese Academy of Sciences, Chengdu 610041, ChinaCAS Key Laboratory of Mountain Ecological Restoration and Bioresource Utilization & Ecological Restoration Biodiversity Conservation Key Laboratory of Sichuan Province, Chengdu Institute of Biology, Chinese Academy of Sciences, Chengdu 610041, ChinaCAS Key Laboratory of Mountain Ecological Restoration and Bioresource Utilization & Ecological Restoration Biodiversity Conservation Key Laboratory of Sichuan Province, Chengdu Institute of Biology, Chinese Academy of Sciences, Chengdu 610041, ChinaThe impacts of human activities on Zoige peatlands are poorly documented. We determined the concentrations and accumulation rates of As and Hg in a <sup>210</sup>Pb-dated peat profile collected from this area and analyzed the correlations between accumulation rates of both As and Hg and other physicochemical properties. To reconstruct recent conditions of As and Hg, we analyzed peat sediments of Re’er Dam peatland in Zoige using <sup>210</sup>Pb and <sup>137</sup>Cs dating technologies. The concentrations of total As (86.38 to 174.21 μg kg<sup>−1</sup>) and Hg (7.30 to 32.13 μg kg<sup>−1</sup>) in the peat profile clearly increased after the first industrial revolution. From AD 1824 to AD 2010, the average accumulation rates were 129.77 μg m<sup>−2</sup> yr<sup>−1</sup> for As and 18.24 μg m<sup>−2</sup> yr<sup>−1</sup> for Hg. Based on our results, anthropogenic emissions significantly affected the atmospheric fluxes of As and Hg throughout the past 200 years, and As was also likely to be affected by other factors than atmospheric deposition, which needs further identification by future studies. The historical variations in As and Hg concentrations in Re’er Dam peatland in Zoige mirror the industrial development of China.https://www.mdpi.com/2073-445X/10/11/1241atmospheric depositionAsHg210Pb137Csaccumulation rate
spellingShingle Xuhui Chen
Qianqian Su
Huai Chen
Dan Xue
A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
Land
atmospheric deposition
As
Hg
210Pb
137Cs
accumulation rate
title A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
title_full A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
title_fullStr A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
title_full_unstemmed A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
title_short A High–Resolution Accumulation Record of Arsenic and Mercury after the First Industrial Revolution from a Peatland in Zoige, Qinghai–Tibet Plateau
title_sort high resolution accumulation record of arsenic and mercury after the first industrial revolution from a peatland in zoige qinghai tibet plateau
topic atmospheric deposition
As
Hg
210Pb
137Cs
accumulation rate
url https://www.mdpi.com/2073-445X/10/11/1241
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