Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review

The review discusses the most effective methods for reducing droplet density on the surface of thin films during pulsed laser deposition. This review highlights pulsed laser deposition as a promising technique for producing thin films from a wide range of materials. However, a significant challenge...

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Main Author: O.V. Devitsky
Format: Article
Language:Russian
Published: Tver State University 2024-12-01
Series:Физико-химические аспекты изучения кластеров, наноструктур и наноматериалов
Subjects:
Online Access:https://physchemaspects.ru/2024/doi-10-26456-pcascnn-2024-16-631/?lang=en
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author O.V. Devitsky
author_facet O.V. Devitsky
author_sort O.V. Devitsky
collection DOAJ
description The review discusses the most effective methods for reducing droplet density on the surface of thin films during pulsed laser deposition. This review highlights pulsed laser deposition as a promising technique for producing thin films from a wide range of materials. However, a significant challenge to its industrial application is the formation of droplets on the thin film surface. The primary causes of the droplet formation are identified, and a classification of methods to reduce the droplet density during pulsed laser deposition is provided. Completely eliminating droplets without compromising the quality or altering the stoichiometric composition of the thin films is exceedingly difficult, and no researchers have achieved this to date. The most effective strategy for reducing the droplet density involves optimizing the pulsed laser deposition parameters for specific material groups. Techniques such as using a segmented crystalline target, periodically rotating it at a specific speed, and employing excimer lasers at the energy densities slightly above the ablation threshold have been shown to reduce the droplet density on the thin film surface to as low as 103 cm-2. The physical and chemical processes occurring on the target surface have the greatest impact on the droplet formation. Among active methods, high-speed filtration is the most effective, capable of reducing droplet density to approximately 2 ⋅ 103 cm-2.
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spelling doaj.art-2513af6c3aab47ca813e07092a9ff96b2024-12-28T15:28:40ZrusTver State UniversityФизико-химические аспекты изучения кластеров, наноструктур и наноматериалов2226-44422658-43602024-12-011663164210.26456/pcascnn/2024.16.631Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: reviewO.V. Devitsky0Federal Research Center Southern Scientific Center of the RAS, North Caucasus Federal University The review discusses the most effective methods for reducing droplet density on the surface of thin films during pulsed laser deposition. This review highlights pulsed laser deposition as a promising technique for producing thin films from a wide range of materials. However, a significant challenge to its industrial application is the formation of droplets on the thin film surface. The primary causes of the droplet formation are identified, and a classification of methods to reduce the droplet density during pulsed laser deposition is provided. Completely eliminating droplets without compromising the quality or altering the stoichiometric composition of the thin films is exceedingly difficult, and no researchers have achieved this to date. The most effective strategy for reducing the droplet density involves optimizing the pulsed laser deposition parameters for specific material groups. Techniques such as using a segmented crystalline target, periodically rotating it at a specific speed, and employing excimer lasers at the energy densities slightly above the ablation threshold have been shown to reduce the droplet density on the thin film surface to as low as 103 cm-2. The physical and chemical processes occurring on the target surface have the greatest impact on the droplet formation. Among active methods, high-speed filtration is the most effective, capable of reducing droplet density to approximately 2 ⋅ 103 cm-2. https://physchemaspects.ru/2024/doi-10-26456-pcascnn-2024-16-631/?lang=enpulsed laser depositionthin filmsdroplet densityhigh-speed filtrationsegmented targetdual-pulse laser depositionlaser energy density
spellingShingle O.V. Devitsky
Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
Физико-химические аспекты изучения кластеров, наноструктур и наноматериалов
pulsed laser deposition
thin films
droplet density
high-speed filtration
segmented target
dual-pulse laser deposition
laser energy density
title Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
title_full Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
title_fullStr Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
title_full_unstemmed Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
title_short Methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition: review
title_sort methods for reducing droplet formation density on the surface of thin semiconductor films by pulse laser deposition review
topic pulsed laser deposition
thin films
droplet density
high-speed filtration
segmented target
dual-pulse laser deposition
laser energy density
url https://physchemaspects.ru/2024/doi-10-26456-pcascnn-2024-16-631/?lang=en
work_keys_str_mv AT ovdevitsky methodsforreducingdropletformationdensityonthesurfaceofthinsemiconductorfilmsbypulselaserdepositionreview