Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event

The presence of polycyclic aromatic hydrocarbons (PAHs) and particulate matter (PM) in air is known to provoke deleterious effects on human health. This work focused on the monitoring of PM and PAHs in the air over four weeks in a peri-urban site in Strasbourg (France), using a three-stage cascade i...

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Main Authors: Farhan Ramadzan Nursanto, Joana Vaz-Ramos, Olivier Delhomme, Sylvie Bégin-Colin, Stéphane Le Calvé
Format: Article
Language:English
Published: MDPI AG 2022-09-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/13/9/1435
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author Farhan Ramadzan Nursanto
Joana Vaz-Ramos
Olivier Delhomme
Sylvie Bégin-Colin
Stéphane Le Calvé
author_facet Farhan Ramadzan Nursanto
Joana Vaz-Ramos
Olivier Delhomme
Sylvie Bégin-Colin
Stéphane Le Calvé
author_sort Farhan Ramadzan Nursanto
collection DOAJ
description The presence of polycyclic aromatic hydrocarbons (PAHs) and particulate matter (PM) in air is known to provoke deleterious effects on human health. This work focused on the monitoring of PM and PAHs in the air over four weeks in a peri-urban site in Strasbourg (France), using a three-stage cascade impactor and a particle analyser allowing PM<sub>1</sub>, PM<sub>2.5</sub> and PM<sub>10</sub> discrimination. Meteorological conditions were monitored to study their influence on the pollutant levels. The average PM<sub>10</sub> concentration of the cascade impactor and particle analyser varied from 11.8 to 80.2 µg/m<sup>3</sup> and 10.6 to 220.2 µg/m<sup>3</sup>, respectively. The PAH total concentration ranged in 1.1–7.6 ng/m<sup>3</sup> and a predominance of 5- and 6-ring PAHs was observed. PAHs were also more abundant in finer particles (PM<sub>1</sub>). Specifically, identified PAHs are traffic tracers suggesting that vehicular emission was one of its main sources. Two pollution episodes, associated with either a Saharan dust wind episode or traffic pollution, were observed, and led to PM<sub>10</sub> and PM<sub>2.5</sub> surpassing the daily limit values established by the European Union despite the traffic limitations according to the COVID restrictions. The total PAH concentrations were the highest during these periods suggesting PAHs might be bound to and transported via dust particles.
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spelling doaj.art-252a084d7df7412c906d81b1dcb79e2d2023-11-23T14:59:34ZengMDPI AGAtmosphere2073-44332022-09-01139143510.3390/atmos13091435Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust EventFarhan Ramadzan Nursanto0Joana Vaz-Ramos1Olivier Delhomme2Sylvie Bégin-Colin3Stéphane Le Calvé4Institut de Chimie et Procédés pour l’Energie, l’Environnement et la Santé (ICPEES), UMR-7515 CNRS-Université de Strasbourg, 25 Rue Becquerel, 67087 Strasbourg, FranceInstitut de Chimie et Procédés pour l’Energie, l’Environnement et la Santé (ICPEES), UMR-7515 CNRS-Université de Strasbourg, 25 Rue Becquerel, 67087 Strasbourg, FranceInstitut de Chimie et Procédés pour l’Energie, l’Environnement et la Santé (ICPEES), UMR-7515 CNRS-Université de Strasbourg, 25 Rue Becquerel, 67087 Strasbourg, FranceInstitut de Physique et Chimie des Matériaux de Strasbourg (IPCMS), UMR-7504 CNRS-Université de Strasbourg, 23 Rue du Lœss, 67034 Strasbourg, FranceInstitut de Chimie et Procédés pour l’Energie, l’Environnement et la Santé (ICPEES), UMR-7515 CNRS-Université de Strasbourg, 25 Rue Becquerel, 67087 Strasbourg, FranceThe presence of polycyclic aromatic hydrocarbons (PAHs) and particulate matter (PM) in air is known to provoke deleterious effects on human health. This work focused on the monitoring of PM and PAHs in the air over four weeks in a peri-urban site in Strasbourg (France), using a three-stage cascade impactor and a particle analyser allowing PM<sub>1</sub>, PM<sub>2.5</sub> and PM<sub>10</sub> discrimination. Meteorological conditions were monitored to study their influence on the pollutant levels. The average PM<sub>10</sub> concentration of the cascade impactor and particle analyser varied from 11.8 to 80.2 µg/m<sup>3</sup> and 10.6 to 220.2 µg/m<sup>3</sup>, respectively. The PAH total concentration ranged in 1.1–7.6 ng/m<sup>3</sup> and a predominance of 5- and 6-ring PAHs was observed. PAHs were also more abundant in finer particles (PM<sub>1</sub>). Specifically, identified PAHs are traffic tracers suggesting that vehicular emission was one of its main sources. Two pollution episodes, associated with either a Saharan dust wind episode or traffic pollution, were observed, and led to PM<sub>10</sub> and PM<sub>2.5</sub> surpassing the daily limit values established by the European Union despite the traffic limitations according to the COVID restrictions. The total PAH concentrations were the highest during these periods suggesting PAHs might be bound to and transported via dust particles.https://www.mdpi.com/2073-4433/13/9/1435PAHsparticulate matterSaharan dustCOVID confinementoutdoor airparticle analyser
spellingShingle Farhan Ramadzan Nursanto
Joana Vaz-Ramos
Olivier Delhomme
Sylvie Bégin-Colin
Stéphane Le Calvé
Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
Atmosphere
PAHs
particulate matter
Saharan dust
COVID confinement
outdoor air
particle analyser
title Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
title_full Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
title_fullStr Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
title_full_unstemmed Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
title_short Simultaneous Monitoring of Outdoor PAHs and Particles in a French Peri-Urban Site during COVID Restrictions and the Winter Saharan Dust Event
title_sort simultaneous monitoring of outdoor pahs and particles in a french peri urban site during covid restrictions and the winter saharan dust event
topic PAHs
particulate matter
Saharan dust
COVID confinement
outdoor air
particle analyser
url https://www.mdpi.com/2073-4433/13/9/1435
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