Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor

In this work, the application of carbon quantum dots as known as CQDs for ethanol detection is pioneered, and a multi-fold improvement in gas sensor performance is achieved through the unique electron transport mechanism of carbon quantum dots. The lychee-like SnO2 hollow microspheres and CQDs are p...

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Main Authors: Zhenyu Yuan, Yongchen Sui, Meige Ding, Hongmin Zhu
Format: Article
Language:English
Published: Elsevier 2023-06-01
Series:Sensors and Actuators Reports
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2666053923000206
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author Zhenyu Yuan
Yongchen Sui
Meige Ding
Hongmin Zhu
author_facet Zhenyu Yuan
Yongchen Sui
Meige Ding
Hongmin Zhu
author_sort Zhenyu Yuan
collection DOAJ
description In this work, the application of carbon quantum dots as known as CQDs for ethanol detection is pioneered, and a multi-fold improvement in gas sensor performance is achieved through the unique electron transport mechanism of carbon quantum dots. The lychee-like SnO2 hollow microspheres and CQDs are prepared by a solvent heat method. The composites are assembled by rapid grinding, ultrasonication, and stirring. The minimum detection limit is 500 ppb. The response/recovery time of the best mass percentage composite is 9 s/16 s to ethanol at 100 ppm with an optimum working temperature of 216℃ in the target gas-sensitive test. Such a fast response speed improvement is ascribed to the excellent electron transfer efficiency of the 5 nm diameter carbon quantum dots (CQDs).
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spelling doaj.art-26a1e94cd3374bf79544bf14526a025c2023-06-16T05:11:44ZengElsevierSensors and Actuators Reports2666-05392023-06-015100157Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensorZhenyu Yuan0Yongchen Sui1Meige Ding2Hongmin Zhu3Corresponding author.; College of Information Science and Engineering, Northeastern University, Shenyang 110819, ChinaCollege of Information Science and Engineering, Northeastern University, Shenyang 110819, ChinaCollege of Information Science and Engineering, Northeastern University, Shenyang 110819, ChinaCollege of Information Science and Engineering, Northeastern University, Shenyang 110819, ChinaIn this work, the application of carbon quantum dots as known as CQDs for ethanol detection is pioneered, and a multi-fold improvement in gas sensor performance is achieved through the unique electron transport mechanism of carbon quantum dots. The lychee-like SnO2 hollow microspheres and CQDs are prepared by a solvent heat method. The composites are assembled by rapid grinding, ultrasonication, and stirring. The minimum detection limit is 500 ppb. The response/recovery time of the best mass percentage composite is 9 s/16 s to ethanol at 100 ppm with an optimum working temperature of 216℃ in the target gas-sensitive test. Such a fast response speed improvement is ascribed to the excellent electron transfer efficiency of the 5 nm diameter carbon quantum dots (CQDs).http://www.sciencedirect.com/science/article/pii/S2666053923000206CqdsSno2Hollow microspheresΠ-states
spellingShingle Zhenyu Yuan
Yongchen Sui
Meige Ding
Hongmin Zhu
Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
Sensors and Actuators Reports
Cqds
Sno2
Hollow microspheres
Π-states
title Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
title_full Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
title_fullStr Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
title_full_unstemmed Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
title_short Lychee-like SnO2 hollow microspheres sensitized by carbon quantum dots for high-sensitivity ethanol sensor
title_sort lychee like sno2 hollow microspheres sensitized by carbon quantum dots for high sensitivity ethanol sensor
topic Cqds
Sno2
Hollow microspheres
Π-states
url http://www.sciencedirect.com/science/article/pii/S2666053923000206
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AT meigeding lycheelikesno2hollowmicrospheressensitizedbycarbonquantumdotsforhighsensitivityethanolsensor
AT hongminzhu lycheelikesno2hollowmicrospheressensitizedbycarbonquantumdotsforhighsensitivityethanolsensor