Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell

The generation of high-order harmonics in a semi-infinite cell by femtosecond laser pulses is a common practice for reliable coherent and low divergence XUV source beams for applications. Despite the relative simplicity of the experimental method, several phenomena coexist that affect the generated...

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Main Authors: Stylianos Petrakis, Makis Bakarezos, Michael Tatarakis, Emmanouil P. Benis, Nektarios A. Papadogiannis
Format: Article
Language:English
Published: MDPI AG 2022-05-01
Series:Atoms
Subjects:
Online Access:https://www.mdpi.com/2218-2004/10/2/53
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author Stylianos Petrakis
Makis Bakarezos
Michael Tatarakis
Emmanouil P. Benis
Nektarios A. Papadogiannis
author_facet Stylianos Petrakis
Makis Bakarezos
Michael Tatarakis
Emmanouil P. Benis
Nektarios A. Papadogiannis
author_sort Stylianos Petrakis
collection DOAJ
description The generation of high-order harmonics in a semi-infinite cell by femtosecond laser pulses is a common practice for reliable coherent and low divergence XUV source beams for applications. Despite the relative simplicity of the experimental method, several phenomena coexist that affect the generated spectral and divergence characteristics of the high harmonic XUV frequency comb. The ionisation degree of the medium and the consequent plasma formation length imposes a spatiotemporal evolution of the fundamental EM field and XUV absorption. Varying the laser pulse chirp and the focusing conditions, as well as the gas density, we measured intense harmonic spectral and divergence variations attributed mainly to self-phase modulations of the laser EM field in the partially ionised medium. Additionally, low-divergence high harmonics are observed for certain laser chirp values attributed to the strong phase matching of only the short electron quantum path. Thus, a tunable, low divergent, and coherent XUV source can be realised for spatiotemporal imaging applications in the nanoscale.
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spelling doaj.art-27190c59dc97486b8ee7c159bb1fb5502023-11-23T15:34:18ZengMDPI AGAtoms2218-20042022-05-011025310.3390/atoms10020053Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas CellStylianos Petrakis0Makis Bakarezos1Michael Tatarakis2Emmanouil P. Benis3Nektarios A. Papadogiannis4Department of Physics, University of Ioannina, 45110 Ioannina, GreeceInstitute of Plasma Physics and Lasers, Hellenic Mediterranean University Research Centre, 74100 Rethymno, GreeceInstitute of Plasma Physics and Lasers, Hellenic Mediterranean University Research Centre, 74100 Rethymno, GreeceDepartment of Physics, University of Ioannina, 45110 Ioannina, GreeceInstitute of Plasma Physics and Lasers, Hellenic Mediterranean University Research Centre, 74100 Rethymno, GreeceThe generation of high-order harmonics in a semi-infinite cell by femtosecond laser pulses is a common practice for reliable coherent and low divergence XUV source beams for applications. Despite the relative simplicity of the experimental method, several phenomena coexist that affect the generated spectral and divergence characteristics of the high harmonic XUV frequency comb. The ionisation degree of the medium and the consequent plasma formation length imposes a spatiotemporal evolution of the fundamental EM field and XUV absorption. Varying the laser pulse chirp and the focusing conditions, as well as the gas density, we measured intense harmonic spectral and divergence variations attributed mainly to self-phase modulations of the laser EM field in the partially ionised medium. Additionally, low-divergence high harmonics are observed for certain laser chirp values attributed to the strong phase matching of only the short electron quantum path. Thus, a tunable, low divergent, and coherent XUV source can be realised for spatiotemporal imaging applications in the nanoscale.https://www.mdpi.com/2218-2004/10/2/53high-order harmonic generationself-phase modulationsemi-infinite cellchirped laser pulses
spellingShingle Stylianos Petrakis
Makis Bakarezos
Michael Tatarakis
Emmanouil P. Benis
Nektarios A. Papadogiannis
Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
Atoms
high-order harmonic generation
self-phase modulation
semi-infinite cell
chirped laser pulses
title Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
title_full Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
title_fullStr Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
title_full_unstemmed Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
title_short Spectral and Divergence Characteristics of Plateau High-Order Harmonics Generated by Femtosecond Chirped Laser Pulses in a Semi-Infinite Gas Cell
title_sort spectral and divergence characteristics of plateau high order harmonics generated by femtosecond chirped laser pulses in a semi infinite gas cell
topic high-order harmonic generation
self-phase modulation
semi-infinite cell
chirped laser pulses
url https://www.mdpi.com/2218-2004/10/2/53
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