Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs
Abstract Metal–organic frameworks (MOFs) have played a crucial role in recent advancements in developing lithium‐based battery electrolytes, electrodes, and separators. Although many MOF‐based battery components rely on their well‐defined porosity and controllable functionality, they also boast a my...
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Format: | Article |
Language: | English |
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Wiley
2024-01-01
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Series: | Advanced Science |
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Online Access: | https://doi.org/10.1002/advs.202305280 |
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author | Anthony U. Mu Guorui Cai Zheng Chen |
author_facet | Anthony U. Mu Guorui Cai Zheng Chen |
author_sort | Anthony U. Mu |
collection | DOAJ |
description | Abstract Metal–organic frameworks (MOFs) have played a crucial role in recent advancements in developing lithium‐based battery electrolytes, electrodes, and separators. Although many MOF‐based battery components rely on their well‐defined porosity and controllable functionality, they also boast a myriad of other significant properties relevant to battery applications. In this mini‐review, the distinct advantages of MOFs in battery applications are discussed, including using MOFs to 1) scavenge impurities to increase cycling stability, 2) widen the operation temperature range of conventional electrolytes, 3) widen the operation voltage range of common electrolytes, and 4) employ as artificial solid‐electrolyte interphases to prevent lithium dendrite growth. Furthermore, subsisting challenges of developing these emerging MOF‐based battery technologies are discussed and guidance for shaping the future of this field is given. |
first_indexed | 2024-03-08T14:25:51Z |
format | Article |
id | doaj.art-28e12e5b4d774b7a9580040b5147aa15 |
institution | Directory Open Access Journal |
issn | 2198-3844 |
language | English |
last_indexed | 2024-03-08T14:25:51Z |
publishDate | 2024-01-01 |
publisher | Wiley |
record_format | Article |
series | Advanced Science |
spelling | doaj.art-28e12e5b4d774b7a9580040b5147aa152024-01-13T04:23:06ZengWileyAdvanced Science2198-38442024-01-01112n/an/a10.1002/advs.202305280Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional DesignsAnthony U. Mu0Guorui Cai1Zheng Chen2Department of Nano and Chemical Engineering University of California San Diego 9500 Gilman Drive La Jolla CA 92093 USADepartment of Chemical and Biomolecular Engineering University of Maryland 4418 Stadium Dr College Park MD 20742 USADepartment of Nano and Chemical Engineering University of California San Diego 9500 Gilman Drive La Jolla CA 92093 USAAbstract Metal–organic frameworks (MOFs) have played a crucial role in recent advancements in developing lithium‐based battery electrolytes, electrodes, and separators. Although many MOF‐based battery components rely on their well‐defined porosity and controllable functionality, they also boast a myriad of other significant properties relevant to battery applications. In this mini‐review, the distinct advantages of MOFs in battery applications are discussed, including using MOFs to 1) scavenge impurities to increase cycling stability, 2) widen the operation temperature range of conventional electrolytes, 3) widen the operation voltage range of common electrolytes, and 4) employ as artificial solid‐electrolyte interphases to prevent lithium dendrite growth. Furthermore, subsisting challenges of developing these emerging MOF‐based battery technologies are discussed and guidance for shaping the future of this field is given.https://doi.org/10.1002/advs.202305280cycling stabilitylithium‐based batteriesmetal–organic frameworkswide operation voltagewide‐temperature operation |
spellingShingle | Anthony U. Mu Guorui Cai Zheng Chen Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs Advanced Science cycling stability lithium‐based batteries metal–organic frameworks wide operation voltage wide‐temperature operation |
title | Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs |
title_full | Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs |
title_fullStr | Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs |
title_full_unstemmed | Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs |
title_short | Metal–Organic Frameworks for the Enhancement of Lithium‐Based Batteries: A Mini Review on Emerging Functional Designs |
title_sort | metal organic frameworks for the enhancement of lithium based batteries a mini review on emerging functional designs |
topic | cycling stability lithium‐based batteries metal–organic frameworks wide operation voltage wide‐temperature operation |
url | https://doi.org/10.1002/advs.202305280 |
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