A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE

Nuclear technologies have strong potential and a unique role to play in delivering reliable low carbon energy to enable a net-zero society for future generations. However, to assure the sustainability required for its long-term success, nuclear will need to deliver innovative solutions as proposed i...

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Main Authors: Bruno Merk, Anna Detkina, Dzianis Litskevich, Omid Noori-kalkhoran, Lakshay Jain, Gregory Cartland-Glover
Format: Article
Language:English
Published: MDPI AG 2022-12-01
Series:Energies
Subjects:
Online Access:https://www.mdpi.com/1996-1073/15/24/9638
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author Bruno Merk
Anna Detkina
Dzianis Litskevich
Omid Noori-kalkhoran
Lakshay Jain
Gregory Cartland-Glover
author_facet Bruno Merk
Anna Detkina
Dzianis Litskevich
Omid Noori-kalkhoran
Lakshay Jain
Gregory Cartland-Glover
author_sort Bruno Merk
collection DOAJ
description Nuclear technologies have strong potential and a unique role to play in delivering reliable low carbon energy to enable a net-zero society for future generations. However, to assure the sustainability required for its long-term success, nuclear will need to deliver innovative solutions as proposed in iMAGINE. One of the most attractive features, but also a key challenge for the envisaged highly integrated nuclear energy system iMAGINE, is the need for a demand driven salt clean-up system based on the principles of reverse reprocessing. The work described provides an insight into the dynamic interplay between a potential salt clean-up system and reactor operation in a plutonium-started core in a dynamic approach. The results presented will help to optimise the parameters for the salt clean-up process as well as to understand the differences which appear between a core started with enriched uranium and plutonium as the fissile material. The integrated model is used to investigate the effects of the initial fissile material on core size, achievable burnup, and long-term operation. Different approaches are tested to achieve a higher burnup in the significantly smaller Pu-driven core. The effects of different clean-up system throughputs on the concentration of fission products in the reactor salt and its consequences are discussed for general molten salt reactor design. Finally, an investigation into how a plutonium loaded core could be used to provide fuel for future reactors through fuel salt splitting is presented, with the outcome that one Pu-started reactor of the same size as a uranium-started core could deliver fuel for 1.5 new cores due to enhanced breeding. The results provide an essential understanding for the progress of iMAGINE as well as the basis for inter-disciplinary work required for optimising iMAGINE.
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spelling doaj.art-29b57b80ea774cfab164db6ee1e3ea982023-11-24T14:40:38ZengMDPI AGEnergies1996-10732022-12-011524963810.3390/en15249638A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINEBruno Merk0Anna Detkina1Dzianis Litskevich2Omid Noori-kalkhoran3Lakshay Jain4Gregory Cartland-Glover5School of Engineering, The University of Liverpool, Liverpool L69 3GH, UKSchool of Engineering, The University of Liverpool, Liverpool L69 3GH, UKSchool of Engineering, The University of Liverpool, Liverpool L69 3GH, UKSchool of Engineering, The University of Liverpool, Liverpool L69 3GH, UKSchool of Engineering, The University of Liverpool, Liverpool L69 3GH, UKSTFC Daresbury Laboratory, Daresbury WA4 4AD, UKNuclear technologies have strong potential and a unique role to play in delivering reliable low carbon energy to enable a net-zero society for future generations. However, to assure the sustainability required for its long-term success, nuclear will need to deliver innovative solutions as proposed in iMAGINE. One of the most attractive features, but also a key challenge for the envisaged highly integrated nuclear energy system iMAGINE, is the need for a demand driven salt clean-up system based on the principles of reverse reprocessing. The work described provides an insight into the dynamic interplay between a potential salt clean-up system and reactor operation in a plutonium-started core in a dynamic approach. The results presented will help to optimise the parameters for the salt clean-up process as well as to understand the differences which appear between a core started with enriched uranium and plutonium as the fissile material. The integrated model is used to investigate the effects of the initial fissile material on core size, achievable burnup, and long-term operation. Different approaches are tested to achieve a higher burnup in the significantly smaller Pu-driven core. The effects of different clean-up system throughputs on the concentration of fission products in the reactor salt and its consequences are discussed for general molten salt reactor design. Finally, an investigation into how a plutonium loaded core could be used to provide fuel for future reactors through fuel salt splitting is presented, with the outcome that one Pu-started reactor of the same size as a uranium-started core could deliver fuel for 1.5 new cores due to enhanced breeding. The results provide an essential understanding for the progress of iMAGINE as well as the basis for inter-disciplinary work required for optimising iMAGINE.https://www.mdpi.com/1996-1073/15/24/9638nuclearnuclear energynuclear reactorsreactor physicsmodelling and simulationmolten salt reactors
spellingShingle Bruno Merk
Anna Detkina
Dzianis Litskevich
Omid Noori-kalkhoran
Lakshay Jain
Gregory Cartland-Glover
A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
Energies
nuclear
nuclear energy
nuclear reactors
reactor physics
modelling and simulation
molten salt reactors
title A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
title_full A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
title_fullStr A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
title_full_unstemmed A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
title_short A HELIOS-Based Dynamic Salt Clean-Up Study Analysing the Effects of a Plutonium-Based Initial Core for iMAGINE
title_sort helios based dynamic salt clean up study analysing the effects of a plutonium based initial core for imagine
topic nuclear
nuclear energy
nuclear reactors
reactor physics
modelling and simulation
molten salt reactors
url https://www.mdpi.com/1996-1073/15/24/9638
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