Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation

Gallium sulfide (GaS), with a hexagonal structure, has received extensive attention due to its graphene-like structure and derived optical properties. Here, high-quality GaS was obtained via chemical vapor synthesis and then prepared as a saturable absorber by the stamp-assisted localization-transfe...

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Main Authors: Kun Guo, Qiang Yu, Fangqi Liu, Haiqin Deng, Tianan Yi, Bo Ren, Wei Su, Sicong Zhu, Zhiqiang Wang, Jian Wu, Pu Zhou
Format: Article
Language:English
Published: MDPI AG 2022-01-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/12/3/378
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author Kun Guo
Qiang Yu
Fangqi Liu
Haiqin Deng
Tianan Yi
Bo Ren
Wei Su
Sicong Zhu
Zhiqiang Wang
Jian Wu
Pu Zhou
author_facet Kun Guo
Qiang Yu
Fangqi Liu
Haiqin Deng
Tianan Yi
Bo Ren
Wei Su
Sicong Zhu
Zhiqiang Wang
Jian Wu
Pu Zhou
author_sort Kun Guo
collection DOAJ
description Gallium sulfide (GaS), with a hexagonal structure, has received extensive attention due to its graphene-like structure and derived optical properties. Here, high-quality GaS was obtained via chemical vapor synthesis and then prepared as a saturable absorber by the stamp-assisted localization-transfer technique onto fiber end face. The stability of the material and the laser damage threshold are maintained due to the optimized thickness and the cavity integration form. The potential of the GaS for nonlinear optics is explored by constructing a GaS-based Erbium-doped mode-locked fiber laser. Stable femtosecond (~448 fs) mode-locking operation of the single pulse train is achieved, and the robust mode-locked operation (>30 days) was recorded. Experimental results show the potential of GaS for multi-functional ultrafast high-power lasers and promote continuous research on graphene-like materials in nonlinear optics and photonics.
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spelling doaj.art-2a1f878f2f124ce7850e4f290a9654ba2023-11-23T17:19:48ZengMDPI AGNanomaterials2079-49912022-01-0112337810.3390/nano12030378Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse GenerationKun Guo0Qiang Yu1Fangqi Liu2Haiqin Deng3Tianan Yi4Bo Ren5Wei Su6Sicong Zhu7Zhiqiang Wang8Jian Wu9Pu Zhou10College of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaCollege of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaHubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, The State Key Laboratory for Refractories and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, ChinaCollege of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaCollege of Mechanical and Electrical Engineering, Hohai University, Changzhou 213022, ChinaCollege of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaCollege of Mechanical and Electrical Engineering, Hohai University, Changzhou 213022, ChinaHubei Province Key Laboratory of Systems Science in Metallurgical Process, College of Science, The State Key Laboratory for Refractories and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, ChinaAston Institute of Photonic Technologies, Aston University, Birmingham B4 7ET, UKCollege of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaCollege of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, ChinaGallium sulfide (GaS), with a hexagonal structure, has received extensive attention due to its graphene-like structure and derived optical properties. Here, high-quality GaS was obtained via chemical vapor synthesis and then prepared as a saturable absorber by the stamp-assisted localization-transfer technique onto fiber end face. The stability of the material and the laser damage threshold are maintained due to the optimized thickness and the cavity integration form. The potential of the GaS for nonlinear optics is explored by constructing a GaS-based Erbium-doped mode-locked fiber laser. Stable femtosecond (~448 fs) mode-locking operation of the single pulse train is achieved, and the robust mode-locked operation (>30 days) was recorded. Experimental results show the potential of GaS for multi-functional ultrafast high-power lasers and promote continuous research on graphene-like materials in nonlinear optics and photonics.https://www.mdpi.com/2079-4991/12/3/378Gallium sulfidesaturable absorbermode-locked fiber laserultrafast pulse
spellingShingle Kun Guo
Qiang Yu
Fangqi Liu
Haiqin Deng
Tianan Yi
Bo Ren
Wei Su
Sicong Zhu
Zhiqiang Wang
Jian Wu
Pu Zhou
Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
Nanomaterials
Gallium sulfide
saturable absorber
mode-locked fiber laser
ultrafast pulse
title Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
title_full Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
title_fullStr Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
title_full_unstemmed Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
title_short Synthesis of Hexagonal Structured GaS Nanosheets for Robust Femtosecond Pulse Generation
title_sort synthesis of hexagonal structured gas nanosheets for robust femtosecond pulse generation
topic Gallium sulfide
saturable absorber
mode-locked fiber laser
ultrafast pulse
url https://www.mdpi.com/2079-4991/12/3/378
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