Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization

Carbon fiber-reinforced polymer (CFRP) composite materials are widely used in engineering applications, but their production generates a significant amount of waste. This paper aims to explore the potential of incorporating mechanically recycled aerospace prepreg waste in thermoplastic composite mat...

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Main Authors: José Antonio Butenegro, Mohsen Bahrami, Yentl Swolfs, Jan Ivens, Miguel Ángel Martínez, Juana Abenojar
Format: Article
Language:English
Published: MDPI AG 2023-08-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/15/16/3447
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author José Antonio Butenegro
Mohsen Bahrami
Yentl Swolfs
Jan Ivens
Miguel Ángel Martínez
Juana Abenojar
author_facet José Antonio Butenegro
Mohsen Bahrami
Yentl Swolfs
Jan Ivens
Miguel Ángel Martínez
Juana Abenojar
author_sort José Antonio Butenegro
collection DOAJ
description Carbon fiber-reinforced polymer (CFRP) composite materials are widely used in engineering applications, but their production generates a significant amount of waste. This paper aims to explore the potential of incorporating mechanically recycled aerospace prepreg waste in thermoplastic composite materials to reduce the environmental impact of composite material production and promote the use of recycled materials. The composite material developed in this study incorporates a bio−based thermoplastic polymer, polyamide 11 (PA11), as the matrix material and recycled aerospace prepreg waste quasi-one-dimensionally arranged as reinforcement. Mechanical, thermal, and thermomechanical characterizations were performed through tensile, flexural, and impact tests, as well as differential scanning calorimetry (DSC) and dynamic mechanical analysis (DMA). Compared to previous studies that used a different recycled CFRP in the shape of rods, the results show that the recycled prepregs are a suitable reinforcement, enhancing the reinforcement-matrix adhesion and leading to higher mechanical properties. The tensile results were evaluated by SEM, and the impact tests were evaluated by CT scans. The results demonstrate the potential of incorporating recycled aerospace prepreg waste in thermoplastic composite materials to produce high-performance and sustainable components in the aerospace and automotive industries.
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spelling doaj.art-2a9528529d12429a9000e75bf63d3d092023-11-19T02:44:27ZengMDPI AGPolymers2073-43602023-08-011516344710.3390/polym15163447Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and CharacterizationJosé Antonio Butenegro0Mohsen Bahrami1Yentl Swolfs2Jan Ivens3Miguel Ángel Martínez4Juana Abenojar5Materials Science and Engineering and Chemical Engineering Department, IAAB, University Carlos III Madrid, 28911 Leganés, SpainMaterials Science and Engineering and Chemical Engineering Department, IAAB, University Carlos III Madrid, 28911 Leganés, SpainDepartment of Materials Engineering, KU Leuven, Kasteelpark Arenberg 44, B-3001 Leuven, BelgiumDepartment of Materials Engineering, KU Leuven, Kasteelpark Arenberg 44, B-3001 Leuven, BelgiumMaterials Science and Engineering and Chemical Engineering Department, IAAB, University Carlos III Madrid, 28911 Leganés, SpainMaterials Science and Engineering and Chemical Engineering Department, IAAB, University Carlos III Madrid, 28911 Leganés, SpainCarbon fiber-reinforced polymer (CFRP) composite materials are widely used in engineering applications, but their production generates a significant amount of waste. This paper aims to explore the potential of incorporating mechanically recycled aerospace prepreg waste in thermoplastic composite materials to reduce the environmental impact of composite material production and promote the use of recycled materials. The composite material developed in this study incorporates a bio−based thermoplastic polymer, polyamide 11 (PA11), as the matrix material and recycled aerospace prepreg waste quasi-one-dimensionally arranged as reinforcement. Mechanical, thermal, and thermomechanical characterizations were performed through tensile, flexural, and impact tests, as well as differential scanning calorimetry (DSC) and dynamic mechanical analysis (DMA). Compared to previous studies that used a different recycled CFRP in the shape of rods, the results show that the recycled prepregs are a suitable reinforcement, enhancing the reinforcement-matrix adhesion and leading to higher mechanical properties. The tensile results were evaluated by SEM, and the impact tests were evaluated by CT scans. The results demonstrate the potential of incorporating recycled aerospace prepreg waste in thermoplastic composite materials to produce high-performance and sustainable components in the aerospace and automotive industries.https://www.mdpi.com/2073-4360/15/16/3447polymer matrix composites (PMCs)carbon fiber-reinforced polymersdiscontinuous reinforcementthermoplastic polymersmechanical properties
spellingShingle José Antonio Butenegro
Mohsen Bahrami
Yentl Swolfs
Jan Ivens
Miguel Ángel Martínez
Juana Abenojar
Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
Polymers
polymer matrix composites (PMCs)
carbon fiber-reinforced polymers
discontinuous reinforcement
thermoplastic polymers
mechanical properties
title Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
title_full Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
title_fullStr Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
title_full_unstemmed Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
title_short Novel Sustainable Composites Incorporating a Biobased Thermoplastic Matrix and Recycled Aerospace Prepreg Waste: Development and Characterization
title_sort novel sustainable composites incorporating a biobased thermoplastic matrix and recycled aerospace prepreg waste development and characterization
topic polymer matrix composites (PMCs)
carbon fiber-reinforced polymers
discontinuous reinforcement
thermoplastic polymers
mechanical properties
url https://www.mdpi.com/2073-4360/15/16/3447
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