Magnetic boson peak in classical spin glasses

We revisited spin dynamics in archetypical classical spin-glass (SG) systems, such as Cu_{1−x}Mn_{x} (x=0.017, 0.034, and 0.067) dilute alloys and iron aluminosilicate glass, using a modern neutron scattering spectrometer with high neutron flux. The former is crystalline, and the latter is amorphous...

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Main Authors: Maiko Kofu, Seiko Ohira-Kawamura, Naoki Murai, Rieko Ishii, Daigorou Hirai, Hiroshi Arima, Kenichi Funakoshi
Format: Article
Language:English
Published: American Physical Society 2024-01-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.6.013006
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author Maiko Kofu
Seiko Ohira-Kawamura
Naoki Murai
Rieko Ishii
Daigorou Hirai
Hiroshi Arima
Kenichi Funakoshi
author_facet Maiko Kofu
Seiko Ohira-Kawamura
Naoki Murai
Rieko Ishii
Daigorou Hirai
Hiroshi Arima
Kenichi Funakoshi
author_sort Maiko Kofu
collection DOAJ
description We revisited spin dynamics in archetypical classical spin-glass (SG) systems, such as Cu_{1−x}Mn_{x} (x=0.017, 0.034, and 0.067) dilute alloys and iron aluminosilicate glass, using a modern neutron scattering spectrometer with high neutron flux. The former is crystalline, and the latter is amorphous, where their SG state is well separated from magnetically ordered phases. Bose-scaled localized magnetic excitations were observed in both compounds below the spin-freezing temperature (T_{f}). The spectrum exhibits a maximum at low energy and a broad tail on the high-energy side. The excitation energy tends to be higher for the material with higher T_{f}. Above T_{f}, the spectrum considerably changes with temperature, thereby indicating the emergence of the magnetic relaxation process. The magnetic excitation in the SG state has much in common with the boson peak in structural glasses. We consider that the Bose-scaled broad excitation peak is an elementary excitation inherent in disordered systems.
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spelling doaj.art-2ab492ca687446bb9a01d9a0e3e898b22024-04-12T17:37:36ZengAmerican Physical SocietyPhysical Review Research2643-15642024-01-016101300610.1103/PhysRevResearch.6.013006Magnetic boson peak in classical spin glassesMaiko KofuSeiko Ohira-KawamuraNaoki MuraiRieko IshiiDaigorou HiraiHiroshi ArimaKenichi FunakoshiWe revisited spin dynamics in archetypical classical spin-glass (SG) systems, such as Cu_{1−x}Mn_{x} (x=0.017, 0.034, and 0.067) dilute alloys and iron aluminosilicate glass, using a modern neutron scattering spectrometer with high neutron flux. The former is crystalline, and the latter is amorphous, where their SG state is well separated from magnetically ordered phases. Bose-scaled localized magnetic excitations were observed in both compounds below the spin-freezing temperature (T_{f}). The spectrum exhibits a maximum at low energy and a broad tail on the high-energy side. The excitation energy tends to be higher for the material with higher T_{f}. Above T_{f}, the spectrum considerably changes with temperature, thereby indicating the emergence of the magnetic relaxation process. The magnetic excitation in the SG state has much in common with the boson peak in structural glasses. We consider that the Bose-scaled broad excitation peak is an elementary excitation inherent in disordered systems.http://doi.org/10.1103/PhysRevResearch.6.013006
spellingShingle Maiko Kofu
Seiko Ohira-Kawamura
Naoki Murai
Rieko Ishii
Daigorou Hirai
Hiroshi Arima
Kenichi Funakoshi
Magnetic boson peak in classical spin glasses
Physical Review Research
title Magnetic boson peak in classical spin glasses
title_full Magnetic boson peak in classical spin glasses
title_fullStr Magnetic boson peak in classical spin glasses
title_full_unstemmed Magnetic boson peak in classical spin glasses
title_short Magnetic boson peak in classical spin glasses
title_sort magnetic boson peak in classical spin glasses
url http://doi.org/10.1103/PhysRevResearch.6.013006
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AT daigorouhirai magneticbosonpeakinclassicalspinglasses
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