The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames

Utilizing efficiently and securely hydrogen as clean energy source, it is required not only to analyze the experimental data under a certain condition but also to create the mathematical model for the prediction of flame propagation velocity under various conditions. Thus, it is significant to under...

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Main Authors: Toshiyuki KATSUMI, Yasuhito YOSHIDA, Ryo NAKAGAWA, Shinya YAZAWA, Masashi KUMADA, Daisuke SATO, Thwe Thwe Aung, Nabiha CHAUMEIX, Satoshi KADOWAKI
Format: Article
Language:English
Published: The Japan Society of Mechanical Engineers 2021-05-01
Series:Journal of Thermal Science and Technology
Subjects:
Online Access:https://www.jstage.jst.go.jp/article/jtst/16/2/16_2021jtst0026/_pdf/-char/en
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author Toshiyuki KATSUMI
Yasuhito YOSHIDA
Ryo NAKAGAWA
Shinya YAZAWA
Masashi KUMADA
Daisuke SATO
Thwe Thwe Aung
Nabiha CHAUMEIX
Satoshi KADOWAKI
author_facet Toshiyuki KATSUMI
Yasuhito YOSHIDA
Ryo NAKAGAWA
Shinya YAZAWA
Masashi KUMADA
Daisuke SATO
Thwe Thwe Aung
Nabiha CHAUMEIX
Satoshi KADOWAKI
author_sort Toshiyuki KATSUMI
collection DOAJ
description Utilizing efficiently and securely hydrogen as clean energy source, it is required not only to analyze the experimental data under a certain condition but also to create the mathematical model for the prediction of flame propagation velocity under various conditions. Thus, it is significant to understand the characteristics of dynamic behavior of hydrogen/air premixed flames and to elucidate the effects of addition of inert gas, i.e. carbon dioxide CO2 and water vapor H2O. We performed the experiments of hydrogen explosion in two types of closed chambers to observe spherically expanding flames using Schlieren photography. Wrinkles on the flame surface were clearly observed in low equivalence ratios. Analyzing the Schlieren images, the flame propagation velocity depending on the flame radius was obtained. Increasing the addition of inert gas, the propagation velocity decreased, especially in the case of CO2 addition. The propagation velocity increased monotonically as the flame radius became larger. The appearance of flame acceleration was found, which was caused by the evolution of wrinkles on the flame surface. Moreover, the Markstein length decreased as the concentration of inert gas became higher, indicating that the addition of inert gas promoted the instability of hydrogen flames. Furthermore, the wrinkling factor, closely related with the increment in propagation velocity, decreased as the inert-gas concentration became higher. The wrinkling factor normalized by the propagation velocity of flat flame increased, on the other hand, under the conditions of high inert-gas concentration, except for near the quenching conditions. This indicated that the addition of CO2 or H2O promoted the unstable motion of hydrogen flames, which could be due to the enhancement of the diffusive-thermal effect. Based on the characteristics of dynamic behavior of hydrogen flames, the parameters used in the mathematical model on propagation velocity including flame acceleration was obtained, and then the flame propagation velocity under various conditions was predicted.
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spelling doaj.art-2acff0746bfa4e89917227e4e5e8e5fe2022-12-21T23:51:10ZengThe Japan Society of Mechanical EngineersJournal of Thermal Science and Technology1880-55662021-05-01162JTST0026JTST002610.1299/jtst.2021jtst0026jtstThe effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flamesToshiyuki KATSUMI0Yasuhito YOSHIDA1Ryo NAKAGAWA2Shinya YAZAWA3Masashi KUMADA4Daisuke SATO5Thwe Thwe Aung6Nabiha CHAUMEIX7Satoshi KADOWAKI8Department of Mechanical Engineering, Nagaoka University of TechnologyDepartment of Mechanical Engineering, Nagaoka University of TechnologyDepartment of Mechanical Engineering, Nagaoka University of TechnologyDepartment of Mechanical Engineering, Nagaoka University of TechnologyDepartment of Mechanical Engineering, Nagaoka University of TechnologyDepartment of System Safety, Nagaoka University of TechnologyCollaborative Laboratories for Advanced Decommissioning Science, Japan Atomic Energy AgencyInstitut de Combustion, Aérothermique, Réactivité et Environnement, CNRSDepartment of System Safety, Nagaoka University of TechnologyUtilizing efficiently and securely hydrogen as clean energy source, it is required not only to analyze the experimental data under a certain condition but also to create the mathematical model for the prediction of flame propagation velocity under various conditions. Thus, it is significant to understand the characteristics of dynamic behavior of hydrogen/air premixed flames and to elucidate the effects of addition of inert gas, i.e. carbon dioxide CO2 and water vapor H2O. We performed the experiments of hydrogen explosion in two types of closed chambers to observe spherically expanding flames using Schlieren photography. Wrinkles on the flame surface were clearly observed in low equivalence ratios. Analyzing the Schlieren images, the flame propagation velocity depending on the flame radius was obtained. Increasing the addition of inert gas, the propagation velocity decreased, especially in the case of CO2 addition. The propagation velocity increased monotonically as the flame radius became larger. The appearance of flame acceleration was found, which was caused by the evolution of wrinkles on the flame surface. Moreover, the Markstein length decreased as the concentration of inert gas became higher, indicating that the addition of inert gas promoted the instability of hydrogen flames. Furthermore, the wrinkling factor, closely related with the increment in propagation velocity, decreased as the inert-gas concentration became higher. The wrinkling factor normalized by the propagation velocity of flat flame increased, on the other hand, under the conditions of high inert-gas concentration, except for near the quenching conditions. This indicated that the addition of CO2 or H2O promoted the unstable motion of hydrogen flames, which could be due to the enhancement of the diffusive-thermal effect. Based on the characteristics of dynamic behavior of hydrogen flames, the parameters used in the mathematical model on propagation velocity including flame acceleration was obtained, and then the flame propagation velocity under various conditions was predicted.https://www.jstage.jst.go.jp/article/jtst/16/2/16_2021jtst0026/_pdf/-char/enhydrogen-air premixed combustionspherically expanding flamecarbon dioxidewater vapordynamic behaviorflame accelerationintrinsic instability
spellingShingle Toshiyuki KATSUMI
Yasuhito YOSHIDA
Ryo NAKAGAWA
Shinya YAZAWA
Masashi KUMADA
Daisuke SATO
Thwe Thwe Aung
Nabiha CHAUMEIX
Satoshi KADOWAKI
The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
Journal of Thermal Science and Technology
hydrogen-air premixed combustion
spherically expanding flame
carbon dioxide
water vapor
dynamic behavior
flame acceleration
intrinsic instability
title The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
title_full The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
title_fullStr The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
title_full_unstemmed The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
title_short The effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen/air premixed flames
title_sort effects of addition of carbon dioxide and water vapor on the dynamic behavior of spherically expanding hydrogen air premixed flames
topic hydrogen-air premixed combustion
spherically expanding flame
carbon dioxide
water vapor
dynamic behavior
flame acceleration
intrinsic instability
url https://www.jstage.jst.go.jp/article/jtst/16/2/16_2021jtst0026/_pdf/-char/en
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