A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring

Ionic conductive hydrogels have shown great potential in areas such as wearable devices and electronic skins. Aiming at the sensitivity and biodegradability of the traditional flexible hydrogel electronic skin, this paper developed an ionic skin (S−iSkin) based on edible starch–sodium alginate (star...

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Main Authors: Zhaoxin Li, Haoyan Xu, Na Jia, Yifei Li, Liangkuan Zhu, Zhuangzhi Sun
Format: Article
Language:English
Published: MDPI AG 2022-05-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/14/9/1902
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author Zhaoxin Li
Haoyan Xu
Na Jia
Yifei Li
Liangkuan Zhu
Zhuangzhi Sun
author_facet Zhaoxin Li
Haoyan Xu
Na Jia
Yifei Li
Liangkuan Zhu
Zhuangzhi Sun
author_sort Zhaoxin Li
collection DOAJ
description Ionic conductive hydrogels have shown great potential in areas such as wearable devices and electronic skins. Aiming at the sensitivity and biodegradability of the traditional flexible hydrogel electronic skin, this paper developed an ionic skin (S−iSkin) based on edible starch–sodium alginate (starch–SA), which can convert the external strain stimulus into a voltage signal without an external power supply. As an excellent ion conductive polymer, S−iSkin exhibited good stretchability, low hydrophilicity and outstanding electrochemical and sensing properties. Driven by sodium ions, the ion charge transfer resistance of S−iSkin is reduced by 4 times, the capacitance value is increased by 2 times and its conductivity is increased by 7 times. Additionally, S−iSkin has excellent sensitivity and linearity (R<sup>2</sup> = 0.998), a long service life and good biocompatibility. Under the action of micro-stress, it can produce a voltage change ratio of 2.6 times, and its sensitivity is 52.04. The service life test showed that it can work stably for 2000 s and work more than 200 stress–voltage response cycles. These findings provide a foundation for the development of health monitoring systems and micro-stress sensing devices based on renewable biomass materials.
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spelling doaj.art-2ae0ed788fa14b189f1b189afc5abd362023-11-23T09:07:58ZengMDPI AGPolymers2073-43602022-05-01149190210.3390/polym14091902A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion MonitoringZhaoxin Li0Haoyan Xu1Na Jia2Yifei Li3Liangkuan Zhu4Zhuangzhi Sun5Province Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaProvince Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaProvince Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaProvince Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaProvince Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaProvince Key Laboratory of Forestry Intelligent Equipment Engineering, College of Mechanical and Electrical Engineering, Northeast Forestry University, Harbin 150000, ChinaIonic conductive hydrogels have shown great potential in areas such as wearable devices and electronic skins. Aiming at the sensitivity and biodegradability of the traditional flexible hydrogel electronic skin, this paper developed an ionic skin (S−iSkin) based on edible starch–sodium alginate (starch–SA), which can convert the external strain stimulus into a voltage signal without an external power supply. As an excellent ion conductive polymer, S−iSkin exhibited good stretchability, low hydrophilicity and outstanding electrochemical and sensing properties. Driven by sodium ions, the ion charge transfer resistance of S−iSkin is reduced by 4 times, the capacitance value is increased by 2 times and its conductivity is increased by 7 times. Additionally, S−iSkin has excellent sensitivity and linearity (R<sup>2</sup> = 0.998), a long service life and good biocompatibility. Under the action of micro-stress, it can produce a voltage change ratio of 2.6 times, and its sensitivity is 52.04. The service life test showed that it can work stably for 2000 s and work more than 200 stress–voltage response cycles. These findings provide a foundation for the development of health monitoring systems and micro-stress sensing devices based on renewable biomass materials.https://www.mdpi.com/2073-4360/14/9/1902ionic skinstarchsensitivitymotion monitoring
spellingShingle Zhaoxin Li
Haoyan Xu
Na Jia
Yifei Li
Liangkuan Zhu
Zhuangzhi Sun
A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
Polymers
ionic skin
starch
sensitivity
motion monitoring
title A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
title_full A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
title_fullStr A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
title_full_unstemmed A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
title_short A Highly Sensitive, Ultra-Durable, Eco-Friendly Ionic Skin for Human Motion Monitoring
title_sort highly sensitive ultra durable eco friendly ionic skin for human motion monitoring
topic ionic skin
starch
sensitivity
motion monitoring
url https://www.mdpi.com/2073-4360/14/9/1902
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