How active forces influence nonequilibrium glass transitions

Dense assemblies of self-propelled particles undergo a nonequilibrium form of glassy dynamics. Physical intuition suggests that increasing departure from equilibrium due to active forces fluidifies a glassy system. We falsify this belief by devising a model of self-propelled particles where increasi...

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Main Authors: Ludovic Berthier, Elijah Flenner, Grzegorz Szamel
Format: Article
Language:English
Published: IOP Publishing 2017-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/aa914e
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author Ludovic Berthier
Elijah Flenner
Grzegorz Szamel
author_facet Ludovic Berthier
Elijah Flenner
Grzegorz Szamel
author_sort Ludovic Berthier
collection DOAJ
description Dense assemblies of self-propelled particles undergo a nonequilibrium form of glassy dynamics. Physical intuition suggests that increasing departure from equilibrium due to active forces fluidifies a glassy system. We falsify this belief by devising a model of self-propelled particles where increasing departure from equilibrium can both enhance or depress glassy dynamics, depending on the chosen state point. We analyze a number of static and dynamic observables and suggest that the location of the nonequilibrium glass transition is primarily controlled by the evolution of two-point static density correlations due to active forces. The dependence of the density correlations on the active forces varies non-trivially with the details of the system, and is difficult to predict theoretically. Our results emphasize the need to develop an accurate liquid state theory for nonequilibrium systems.
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spelling doaj.art-2b0c8c72a4c04d40bd585a114d6218f42023-08-08T14:48:38ZengIOP PublishingNew Journal of Physics1367-26302017-01-01191212500610.1088/1367-2630/aa914eHow active forces influence nonequilibrium glass transitionsLudovic Berthier0https://orcid.org/0000-0003-2059-702XElijah Flenner1Grzegorz Szamel2Laboratoire Charles Coulomb, UMR 5221 CNRS, Université Montpellier , Montpellier, FranceDepartment of Chemistry, Colorado State University , Fort Collins, CO 80523, United States of AmericaLaboratoire Charles Coulomb, UMR 5221 CNRS, Université Montpellier , Montpellier, France; Department of Chemistry, Colorado State University , Fort Collins, CO 80523, United States of AmericaDense assemblies of self-propelled particles undergo a nonequilibrium form of glassy dynamics. Physical intuition suggests that increasing departure from equilibrium due to active forces fluidifies a glassy system. We falsify this belief by devising a model of self-propelled particles where increasing departure from equilibrium can both enhance or depress glassy dynamics, depending on the chosen state point. We analyze a number of static and dynamic observables and suggest that the location of the nonequilibrium glass transition is primarily controlled by the evolution of two-point static density correlations due to active forces. The dependence of the density correlations on the active forces varies non-trivially with the details of the system, and is difficult to predict theoretically. Our results emphasize the need to develop an accurate liquid state theory for nonequilibrium systems.https://doi.org/10.1088/1367-2630/aa914eactive matterglass transitiontheory
spellingShingle Ludovic Berthier
Elijah Flenner
Grzegorz Szamel
How active forces influence nonequilibrium glass transitions
New Journal of Physics
active matter
glass transition
theory
title How active forces influence nonequilibrium glass transitions
title_full How active forces influence nonequilibrium glass transitions
title_fullStr How active forces influence nonequilibrium glass transitions
title_full_unstemmed How active forces influence nonequilibrium glass transitions
title_short How active forces influence nonequilibrium glass transitions
title_sort how active forces influence nonequilibrium glass transitions
topic active matter
glass transition
theory
url https://doi.org/10.1088/1367-2630/aa914e
work_keys_str_mv AT ludovicberthier howactiveforcesinfluencenonequilibriumglasstransitions
AT elijahflenner howactiveforcesinfluencenonequilibriumglasstransitions
AT grzegorzszamel howactiveforcesinfluencenonequilibriumglasstransitions