Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors
The review is devoted to the analysis of the compositional disordering potential of the crystal matrix of a scintillator to improve its scintillation parameters. Technological capabilities to complicate crystal matrices both in anionic and cationic sublattices of a variety of compounds are examined....
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Format: | Article |
Language: | English |
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MDPI AG
2022-12-01
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Series: | Nanomaterials |
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Online Access: | https://www.mdpi.com/2079-4991/12/23/4295 |
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author | Vasili Retivov Valery Dubov Ilia Komendo Petr Karpyuk Daria Kuznetsova Petr Sokolov Yauheni Talochka Mikhail Korzhik |
author_facet | Vasili Retivov Valery Dubov Ilia Komendo Petr Karpyuk Daria Kuznetsova Petr Sokolov Yauheni Talochka Mikhail Korzhik |
author_sort | Vasili Retivov |
collection | DOAJ |
description | The review is devoted to the analysis of the compositional disordering potential of the crystal matrix of a scintillator to improve its scintillation parameters. Technological capabilities to complicate crystal matrices both in anionic and cationic sublattices of a variety of compounds are examined. The effects of the disorder at nano-level on the landscape at the bottom of the conduction band, which is adjacent to the band gap, have been discussed. The ways to control the composition of polycationic compounds when creating precursors, the role of disorder in the anionic sublattice in alkali halide compounds, a positive role of Gd based matrices on scintillation properties, and the control of the heterovalent state of the activator by creation of disorder in silicates have been considered as well. The benefits of introducing a 3D printing method, which is prospective for the engineering and production of scintillators at the nanoscale level, have been manifested. |
first_indexed | 2024-03-09T17:37:29Z |
format | Article |
id | doaj.art-2b5a57f39ca445fa840e0a9b82c7b35c |
institution | Directory Open Access Journal |
issn | 2079-4991 |
language | English |
last_indexed | 2024-03-09T17:37:29Z |
publishDate | 2022-12-01 |
publisher | MDPI AG |
record_format | Article |
series | Nanomaterials |
spelling | doaj.art-2b5a57f39ca445fa840e0a9b82c7b35c2023-11-24T11:48:39ZengMDPI AGNanomaterials2079-49912022-12-011223429510.3390/nano12234295Compositionally Disordered Crystalline Compounds for Next Generation of Radiation DetectorsVasili Retivov0Valery Dubov1Ilia Komendo2Petr Karpyuk3Daria Kuznetsova4Petr Sokolov5Yauheni Talochka6Mikhail Korzhik7National Research Center “Kurchatov Institute”, Moscow 123098, RussiaNational Research Center “Kurchatov Institute”, Moscow 123098, RussiaNational Research Center “Kurchatov Institute”, Moscow 123098, RussiaNational Research Center “Kurchatov Institute”, Moscow 123098, RussiaNational Research Center “Kurchatov Institute”, Moscow 123098, RussiaNational Research Center “Kurchatov Institute”—Institute of Reactives, IREA, Moscow 107076, RussiaInstitute for Nuclear Problems, Belarus State University, 220030 Minsk, BelarusNational Research Center “Kurchatov Institute”, Moscow 123098, RussiaThe review is devoted to the analysis of the compositional disordering potential of the crystal matrix of a scintillator to improve its scintillation parameters. Technological capabilities to complicate crystal matrices both in anionic and cationic sublattices of a variety of compounds are examined. The effects of the disorder at nano-level on the landscape at the bottom of the conduction band, which is adjacent to the band gap, have been discussed. The ways to control the composition of polycationic compounds when creating precursors, the role of disorder in the anionic sublattice in alkali halide compounds, a positive role of Gd based matrices on scintillation properties, and the control of the heterovalent state of the activator by creation of disorder in silicates have been considered as well. The benefits of introducing a 3D printing method, which is prospective for the engineering and production of scintillators at the nanoscale level, have been manifested.https://www.mdpi.com/2079-4991/12/23/4295inorganic compoundcrystalline materialscintillatorcompositional disorderlight yieldscintillation kinetics |
spellingShingle | Vasili Retivov Valery Dubov Ilia Komendo Petr Karpyuk Daria Kuznetsova Petr Sokolov Yauheni Talochka Mikhail Korzhik Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors Nanomaterials inorganic compound crystalline material scintillator compositional disorder light yield scintillation kinetics |
title | Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors |
title_full | Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors |
title_fullStr | Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors |
title_full_unstemmed | Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors |
title_short | Compositionally Disordered Crystalline Compounds for Next Generation of Radiation Detectors |
title_sort | compositionally disordered crystalline compounds for next generation of radiation detectors |
topic | inorganic compound crystalline material scintillator compositional disorder light yield scintillation kinetics |
url | https://www.mdpi.com/2079-4991/12/23/4295 |
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