Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite

The generation of bound electron and hole pairs—excitons—is a key process in photovoltaic technologies, yet it is challenging to follow their initial dynamics. Here, Luoet al. probe the Rydberg eigenstates that characterize the excitonic transport and coherent conversion in a perovskite material....

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Main Authors: Liang Luo, Long Men, Zhaoyu Liu, Yaroslav Mudryk, Xin Zhao, Yongxin Yao, Joong M. Park, Ruth Shinar, Joseph Shinar, Kai-Ming Ho, Ilias E. Perakis, Javier Vela, Jigang Wang
Format: Article
Language:English
Published: Nature Portfolio 2017-06-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/ncomms15565
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author Liang Luo
Long Men
Zhaoyu Liu
Yaroslav Mudryk
Xin Zhao
Yongxin Yao
Joong M. Park
Ruth Shinar
Joseph Shinar
Kai-Ming Ho
Ilias E. Perakis
Javier Vela
Jigang Wang
author_facet Liang Luo
Long Men
Zhaoyu Liu
Yaroslav Mudryk
Xin Zhao
Yongxin Yao
Joong M. Park
Ruth Shinar
Joseph Shinar
Kai-Ming Ho
Ilias E. Perakis
Javier Vela
Jigang Wang
author_sort Liang Luo
collection DOAJ
description The generation of bound electron and hole pairs—excitons—is a key process in photovoltaic technologies, yet it is challenging to follow their initial dynamics. Here, Luoet al. probe the Rydberg eigenstates that characterize the excitonic transport and coherent conversion in a perovskite material.
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spelling doaj.art-2b7a193744d0448691cd461c6cff8e952022-12-21T20:36:06ZengNature PortfolioNature Communications2041-17232017-06-01811810.1038/ncomms15565Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskiteLiang Luo0Long Men1Zhaoyu Liu2Yaroslav Mudryk3Xin Zhao4Yongxin Yao5Joong M. Park6Ruth Shinar7Joseph Shinar8Kai-Ming Ho9Ilias E. Perakis10Javier Vela11Jigang Wang12Division of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDepartment of Chemistry, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityDepartment of Physics, University of Alabama at BirminghamDepartment of Chemistry, Iowa State UniversityDivision of Materials Science and Engineering, Ames Laboratory, Iowa State UniversityThe generation of bound electron and hole pairs—excitons—is a key process in photovoltaic technologies, yet it is challenging to follow their initial dynamics. Here, Luoet al. probe the Rydberg eigenstates that characterize the excitonic transport and coherent conversion in a perovskite material.https://doi.org/10.1038/ncomms15565
spellingShingle Liang Luo
Long Men
Zhaoyu Liu
Yaroslav Mudryk
Xin Zhao
Yongxin Yao
Joong M. Park
Ruth Shinar
Joseph Shinar
Kai-Ming Ho
Ilias E. Perakis
Javier Vela
Jigang Wang
Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
Nature Communications
title Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
title_full Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
title_fullStr Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
title_full_unstemmed Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
title_short Ultrafast terahertz snapshots of excitonic Rydberg states and electronic coherence in an organometal halide perovskite
title_sort ultrafast terahertz snapshots of excitonic rydberg states and electronic coherence in an organometal halide perovskite
url https://doi.org/10.1038/ncomms15565
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