Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts
Traditional approach to oxidation catalysts relies on metal/oxide supported peripheral interfacial oxygen activity. Here the authors show surface oxygenation of platinum-alloyed multicomponent nanoparticles, and reveals irregular oscillatory kinetics associated with the surface oxygenated sites.
Main Authors: | , , , , , , , , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Nature Portfolio
2020-08-01
|
Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-020-18017-3 |
_version_ | 1818842251560747008 |
---|---|
author | Shiyao Shan Jing Li Yazan Maswadeh Casey O’Brien Haval Kareem Dat T. Tran Ivan C. Lee Zhi-Peng Wu Shan Wang Shan Yan Hannah Cronk Derrick Mott Lefu Yang Jin Luo Valeri Petkov Chuan-Jian Zhong |
author_facet | Shiyao Shan Jing Li Yazan Maswadeh Casey O’Brien Haval Kareem Dat T. Tran Ivan C. Lee Zhi-Peng Wu Shan Wang Shan Yan Hannah Cronk Derrick Mott Lefu Yang Jin Luo Valeri Petkov Chuan-Jian Zhong |
author_sort | Shiyao Shan |
collection | DOAJ |
description | Traditional approach to oxidation catalysts relies on metal/oxide supported peripheral interfacial oxygen activity. Here the authors show surface oxygenation of platinum-alloyed multicomponent nanoparticles, and reveals irregular oscillatory kinetics associated with the surface oxygenated sites. |
first_indexed | 2024-12-19T04:39:00Z |
format | Article |
id | doaj.art-2b7a2359b685481ba2224d660edc30fe |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-19T04:39:00Z |
publishDate | 2020-08-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-2b7a2359b685481ba2224d660edc30fe2022-12-21T20:35:39ZengNature PortfolioNature Communications2041-17232020-08-011111910.1038/s41467-020-18017-3Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalystsShiyao Shan0Jing Li1Yazan Maswadeh2Casey O’Brien3Haval Kareem4Dat T. Tran5Ivan C. Lee6Zhi-Peng Wu7Shan Wang8Shan Yan9Hannah Cronk10Derrick Mott11Lefu Yang12Jin Luo13Valeri Petkov14Chuan-Jian Zhong15Department of Chemistry, State University of New York at BinghamtonDepartment of Chemistry, State University of New York at BinghamtonDepartment of Physics, Central Michigan UniversityCCDC Army Research Laboratory, FCDD-RLS-CCDepartment of Chemistry, State University of New York at BinghamtonCCDC Army Research Laboratory, FCDD-RLS-CCCCDC Army Research Laboratory, FCDD-RLS-CCDepartment of Chemistry, State University of New York at BinghamtonDepartment of Chemistry, State University of New York at BinghamtonDepartment of Chemistry, State University of New York at BinghamtonDepartment of Chemistry, State University of New York at BinghamtonSchool of Materials Science, JAISTCollege of Chemistry and Chemical Engineering, Xiamen UniversityDepartment of Chemistry, State University of New York at BinghamtonDepartment of Physics, Central Michigan UniversityDepartment of Chemistry, State University of New York at BinghamtonTraditional approach to oxidation catalysts relies on metal/oxide supported peripheral interfacial oxygen activity. Here the authors show surface oxygenation of platinum-alloyed multicomponent nanoparticles, and reveals irregular oscillatory kinetics associated with the surface oxygenated sites.https://doi.org/10.1038/s41467-020-18017-3 |
spellingShingle | Shiyao Shan Jing Li Yazan Maswadeh Casey O’Brien Haval Kareem Dat T. Tran Ivan C. Lee Zhi-Peng Wu Shan Wang Shan Yan Hannah Cronk Derrick Mott Lefu Yang Jin Luo Valeri Petkov Chuan-Jian Zhong Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts Nature Communications |
title | Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
title_full | Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
title_fullStr | Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
title_full_unstemmed | Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
title_short | Surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
title_sort | surface oxygenation of multicomponent nanoparticles toward active and stable oxidation catalysts |
url | https://doi.org/10.1038/s41467-020-18017-3 |
work_keys_str_mv | AT shiyaoshan surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT jingli surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT yazanmaswadeh surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT caseyobrien surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT havalkareem surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT datttran surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT ivanclee surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT zhipengwu surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT shanwang surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT shanyan surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT hannahcronk surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT derrickmott surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT lefuyang surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT jinluo surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT valeripetkov surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts AT chuanjianzhong surfaceoxygenationofmulticomponentnanoparticlestowardactiveandstableoxidationcatalysts |