Time-resolved in situ visualization of the structural response of zeolites during catalysis

Study of structural inhomogeneities in zeolites is important but limited by conventional techniques. Here the authors employ in situ free-electron-laser-based time-resolved coherent X-ray diffraction imaging to visualize the effect of these inhomogeneities during catalytic deoxygenation of NOx.

Bibliographic Details
Main Authors: Jinback Kang, Jerome Carnis, Dongjin Kim, Myungwoo Chung, Jaeseung Kim, Kyuseok Yun, Gukil An, Wonsuk Cha, Ross Harder, Sanghoon Song, Marcin Sikorski, Aymeric Robert, Nguyen Huu Thanh, Heeju Lee, Yong Nam Choi, Xiaojing Huang, Yong S. Chu, Jesse N. Clark, Mee Kyung Song, Kyung Byung Yoon, Ian K. Robinson, Hyunjung Kim
Format: Article
Language:English
Published: Nature Portfolio 2020-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-020-19728-3
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author Jinback Kang
Jerome Carnis
Dongjin Kim
Myungwoo Chung
Jaeseung Kim
Kyuseok Yun
Gukil An
Wonsuk Cha
Ross Harder
Sanghoon Song
Marcin Sikorski
Aymeric Robert
Nguyen Huu Thanh
Heeju Lee
Yong Nam Choi
Xiaojing Huang
Yong S. Chu
Jesse N. Clark
Mee Kyung Song
Kyung Byung Yoon
Ian K. Robinson
Hyunjung Kim
author_facet Jinback Kang
Jerome Carnis
Dongjin Kim
Myungwoo Chung
Jaeseung Kim
Kyuseok Yun
Gukil An
Wonsuk Cha
Ross Harder
Sanghoon Song
Marcin Sikorski
Aymeric Robert
Nguyen Huu Thanh
Heeju Lee
Yong Nam Choi
Xiaojing Huang
Yong S. Chu
Jesse N. Clark
Mee Kyung Song
Kyung Byung Yoon
Ian K. Robinson
Hyunjung Kim
author_sort Jinback Kang
collection DOAJ
description Study of structural inhomogeneities in zeolites is important but limited by conventional techniques. Here the authors employ in situ free-electron-laser-based time-resolved coherent X-ray diffraction imaging to visualize the effect of these inhomogeneities during catalytic deoxygenation of NOx.
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spelling doaj.art-2badad485d3340d9b9ac5c3c53d462752022-12-21T18:33:22ZengNature PortfolioNature Communications2041-17232020-11-011111810.1038/s41467-020-19728-3Time-resolved in situ visualization of the structural response of zeolites during catalysisJinback Kang0Jerome Carnis1Dongjin Kim2Myungwoo Chung3Jaeseung Kim4Kyuseok Yun5Gukil An6Wonsuk Cha7Ross Harder8Sanghoon Song9Marcin Sikorski10Aymeric Robert11Nguyen Huu Thanh12Heeju Lee13Yong Nam Choi14Xiaojing Huang15Yong S. Chu16Jesse N. Clark17Mee Kyung Song18Kyung Byung Yoon19Ian K. Robinson20Hyunjung Kim21Department of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityDepartment of Physics, Sogang UniversityMaterials Science Division, Argonne National LaboratoryAdvanced Photon Source, Argonne National LaboratoryLinac Coherent Light Source, SLAC National Accelerator LaboratoryLinac Coherent Light Source, SLAC National Accelerator LaboratoryLinac Coherent Light Source, SLAC National Accelerator LaboratoryDepartment of Chemistry, Sogang UniversityDepartment of Physics, Sogang UniversityKorea Atomic Energy Research InstituteNational Synchrotron Light Source II (NSLS-II), Brookhaven National LaboratoryNational Synchrotron Light Source II (NSLS-II), Brookhaven National LaboratoryStanford PULSE Institute, SLAC National Accelerator LaboratoryDepartment of Chemistry, Sogang UniversityDepartment of Chemistry, Sogang UniversityLondon Centre for Nanotechnology, University College LondonDepartment of Physics, Sogang UniversityStudy of structural inhomogeneities in zeolites is important but limited by conventional techniques. Here the authors employ in situ free-electron-laser-based time-resolved coherent X-ray diffraction imaging to visualize the effect of these inhomogeneities during catalytic deoxygenation of NOx.https://doi.org/10.1038/s41467-020-19728-3
spellingShingle Jinback Kang
Jerome Carnis
Dongjin Kim
Myungwoo Chung
Jaeseung Kim
Kyuseok Yun
Gukil An
Wonsuk Cha
Ross Harder
Sanghoon Song
Marcin Sikorski
Aymeric Robert
Nguyen Huu Thanh
Heeju Lee
Yong Nam Choi
Xiaojing Huang
Yong S. Chu
Jesse N. Clark
Mee Kyung Song
Kyung Byung Yoon
Ian K. Robinson
Hyunjung Kim
Time-resolved in situ visualization of the structural response of zeolites during catalysis
Nature Communications
title Time-resolved in situ visualization of the structural response of zeolites during catalysis
title_full Time-resolved in situ visualization of the structural response of zeolites during catalysis
title_fullStr Time-resolved in situ visualization of the structural response of zeolites during catalysis
title_full_unstemmed Time-resolved in situ visualization of the structural response of zeolites during catalysis
title_short Time-resolved in situ visualization of the structural response of zeolites during catalysis
title_sort time resolved in situ visualization of the structural response of zeolites during catalysis
url https://doi.org/10.1038/s41467-020-19728-3
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