Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water

To solve the problem of water carryover in the supercritical CO<sub>2</sub> separation and mining process in the CO<sub>2</sub> plume geothermal system, a three-dimensional shell-tube hollow fiber membrane absorption separator is designed in this study. A coupled species tran...

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Main Authors: Zongliang Qiao, Yue Pan, Youfei Tang, Yue Cao, Fengqi Si
Format: Article
Language:English
Published: MDPI AG 2023-11-01
Series:Membranes
Subjects:
Online Access:https://www.mdpi.com/2077-0375/13/12/892
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author Zongliang Qiao
Yue Pan
Youfei Tang
Yue Cao
Fengqi Si
author_facet Zongliang Qiao
Yue Pan
Youfei Tang
Yue Cao
Fengqi Si
author_sort Zongliang Qiao
collection DOAJ
description To solve the problem of water carryover in the supercritical CO<sub>2</sub> separation and mining process in the CO<sub>2</sub> plume geothermal system, a three-dimensional shell-tube hollow fiber membrane absorption separator is designed in this study. A coupled species transport model, a porous medium model, and an absorption mathematical model are established, and the flow field and separation characteristics in the circular and flat tubes are analyzed using numerical simulation. The results show that the membrane separation efficiency increases with an increase in the flatness and membrane tube length. When the inlet velocity of the mixture is 0.1 m/s, the separation efficiency can reach 75.92%. Selecting a smaller flow Reynolds number and a more significant membrane tube flatness will reduce the water mass fraction at the outlet. When adding baffles of different shapes to the membrane tube, the mixture fluid in the membrane tube meanders forward and flows in the shape of “Z” under the blocking effect of the arcuate baffles. With an increase in the number of arcuate baffles in the membrane tube, the membrane separation efficiency of the separator increases continuously. The mixture fluid flows in the membrane tube with the built-in torsional baffles in a spiral manner, and the separation efficiency of the membrane separator increases with a torsion ratio reduction in the membrane tube.
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spelling doaj.art-2bc470fc5c9e4acd9ac31f31c81ce4bf2023-12-22T14:24:16ZengMDPI AGMembranes2077-03752023-11-01131289210.3390/membranes13120892Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and WaterZongliang Qiao0Yue Pan1Youfei Tang2Yue Cao3Fengqi Si4Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, Southeast University, Nanjing 210096, ChinaTo solve the problem of water carryover in the supercritical CO<sub>2</sub> separation and mining process in the CO<sub>2</sub> plume geothermal system, a three-dimensional shell-tube hollow fiber membrane absorption separator is designed in this study. A coupled species transport model, a porous medium model, and an absorption mathematical model are established, and the flow field and separation characteristics in the circular and flat tubes are analyzed using numerical simulation. The results show that the membrane separation efficiency increases with an increase in the flatness and membrane tube length. When the inlet velocity of the mixture is 0.1 m/s, the separation efficiency can reach 75.92%. Selecting a smaller flow Reynolds number and a more significant membrane tube flatness will reduce the water mass fraction at the outlet. When adding baffles of different shapes to the membrane tube, the mixture fluid in the membrane tube meanders forward and flows in the shape of “Z” under the blocking effect of the arcuate baffles. With an increase in the number of arcuate baffles in the membrane tube, the membrane separation efficiency of the separator increases continuously. The mixture fluid flows in the membrane tube with the built-in torsional baffles in a spiral manner, and the separation efficiency of the membrane separator increases with a torsion ratio reduction in the membrane tube.https://www.mdpi.com/2077-0375/13/12/892supercritical carbon dioxidemembrane–absorption separatorhollow fiber membranenumerical simulationseparation efficiency
spellingShingle Zongliang Qiao
Yue Pan
Youfei Tang
Yue Cao
Fengqi Si
Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
Membranes
supercritical carbon dioxide
membrane–absorption separator
hollow fiber membrane
numerical simulation
separation efficiency
title Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
title_full Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
title_fullStr Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
title_full_unstemmed Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
title_short Numerical Simulation of Membrane Separation Characteristics of Supercritical Carbon Dioxide and Water
title_sort numerical simulation of membrane separation characteristics of supercritical carbon dioxide and water
topic supercritical carbon dioxide
membrane–absorption separator
hollow fiber membrane
numerical simulation
separation efficiency
url https://www.mdpi.com/2077-0375/13/12/892
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AT yuepan numericalsimulationofmembraneseparationcharacteristicsofsupercriticalcarbondioxideandwater
AT youfeitang numericalsimulationofmembraneseparationcharacteristicsofsupercriticalcarbondioxideandwater
AT yuecao numericalsimulationofmembraneseparationcharacteristicsofsupercriticalcarbondioxideandwater
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