Two-Channel Charge-Kondo Physics in Graphene Quantum Dots

Nanoelectronic quantum dot devices exploiting the charge-Kondo paradigm have been established as versatile and accurate analogue quantum simulators of fundamental quantum impurity models. In particular, hybrid metal–semiconductor dots connected to two metallic leads realize the two-channel Kondo (2C...

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Main Authors: Emma L. Minarelli, Jonas B. Rigo, Andrew K. Mitchell
Format: Article
Language:English
Published: MDPI AG 2022-04-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/12/9/1513
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author Emma L. Minarelli
Jonas B. Rigo
Andrew K. Mitchell
author_facet Emma L. Minarelli
Jonas B. Rigo
Andrew K. Mitchell
author_sort Emma L. Minarelli
collection DOAJ
description Nanoelectronic quantum dot devices exploiting the charge-Kondo paradigm have been established as versatile and accurate analogue quantum simulators of fundamental quantum impurity models. In particular, hybrid metal–semiconductor dots connected to two metallic leads realize the two-channel Kondo (2CK) model, in which Kondo screening of the dot charge pseudospin is frustrated. In this article, a two-channel charge-Kondo device made instead from graphene components is considered, realizing a pseudogapped version of the 2CK model. The model is solved using Wilson’s Numerical Renormalization Group method, uncovering a rich phase diagram as a function of dot–lead coupling strength, channel asymmetry, and potential scattering. The complex physics of this system is explored through its thermodynamic properties, scattering T-matrix, and experimentally measurable conductance. The strong coupling pseudogap Kondo phase is found to persist in the channel-asymmetric two-channel context, while in the channel-symmetric case, frustration results in a novel quantum phase transition. Remarkably, despite the vanishing density of states in the graphene leads at low energies, a <i>finite</i> linear conductance is found at zero temperature at the frustrated critical point, which is of a non-Fermi liquid type. Our results suggest that the graphene charge-Kondo platform offers a unique possibility to access multichannel pseudogap Kondo physics.
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spelling doaj.art-2c15de4ecf694277906ef5996d138be42023-11-23T08:55:21ZengMDPI AGNanomaterials2079-49912022-04-01129151310.3390/nano12091513Two-Channel Charge-Kondo Physics in Graphene Quantum DotsEmma L. Minarelli0Jonas B. Rigo1Andrew K. Mitchell2School of Physics, University College Dublin, Dublin 4, IrelandSchool of Physics, University College Dublin, Dublin 4, IrelandSchool of Physics, University College Dublin, Dublin 4, IrelandNanoelectronic quantum dot devices exploiting the charge-Kondo paradigm have been established as versatile and accurate analogue quantum simulators of fundamental quantum impurity models. In particular, hybrid metal–semiconductor dots connected to two metallic leads realize the two-channel Kondo (2CK) model, in which Kondo screening of the dot charge pseudospin is frustrated. In this article, a two-channel charge-Kondo device made instead from graphene components is considered, realizing a pseudogapped version of the 2CK model. The model is solved using Wilson’s Numerical Renormalization Group method, uncovering a rich phase diagram as a function of dot–lead coupling strength, channel asymmetry, and potential scattering. The complex physics of this system is explored through its thermodynamic properties, scattering T-matrix, and experimentally measurable conductance. The strong coupling pseudogap Kondo phase is found to persist in the channel-asymmetric two-channel context, while in the channel-symmetric case, frustration results in a novel quantum phase transition. Remarkably, despite the vanishing density of states in the graphene leads at low energies, a <i>finite</i> linear conductance is found at zero temperature at the frustrated critical point, which is of a non-Fermi liquid type. Our results suggest that the graphene charge-Kondo platform offers a unique possibility to access multichannel pseudogap Kondo physics.https://www.mdpi.com/2079-4991/12/9/1513Kondo effectgrapheneelectronic transportquantum dots
spellingShingle Emma L. Minarelli
Jonas B. Rigo
Andrew K. Mitchell
Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
Nanomaterials
Kondo effect
graphene
electronic transport
quantum dots
title Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
title_full Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
title_fullStr Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
title_full_unstemmed Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
title_short Two-Channel Charge-Kondo Physics in Graphene Quantum Dots
title_sort two channel charge kondo physics in graphene quantum dots
topic Kondo effect
graphene
electronic transport
quantum dots
url https://www.mdpi.com/2079-4991/12/9/1513
work_keys_str_mv AT emmalminarelli twochannelchargekondophysicsingraphenequantumdots
AT jonasbrigo twochannelchargekondophysicsingraphenequantumdots
AT andrewkmitchell twochannelchargekondophysicsingraphenequantumdots