Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy
Solid electrolyte interphase (SEI) formation on Li-ion battery anodes is critical for long-term performance. Here, the authors use operando soft X-ray absorption spectroscopy in total electron yield mode to resolve the chemical evolution of the SEI during electrochemical formation on silicon anodes.
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2022-10-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-33691-1 |
| _version_ | 1811238702963228672 |
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| author | Jack E. N. Swallow Michael W. Fraser Nis-Julian H. Kneusels Jodie F. Charlton Christopher G. Sole Conor M. E. Phelan Erik Björklund Peter Bencok Carlos Escudero Virginia Pérez-Dieste Clare P. Grey Rebecca J. Nicholls Robert S. Weatherup |
| author_facet | Jack E. N. Swallow Michael W. Fraser Nis-Julian H. Kneusels Jodie F. Charlton Christopher G. Sole Conor M. E. Phelan Erik Björklund Peter Bencok Carlos Escudero Virginia Pérez-Dieste Clare P. Grey Rebecca J. Nicholls Robert S. Weatherup |
| author_sort | Jack E. N. Swallow |
| collection | DOAJ |
| description | Solid electrolyte interphase (SEI) formation on Li-ion battery anodes is critical for long-term performance. Here, the authors use operando soft X-ray absorption spectroscopy in total electron yield mode to resolve the chemical evolution of the SEI during electrochemical formation on silicon anodes. |
| first_indexed | 2024-04-12T12:46:52Z |
| format | Article |
| id | doaj.art-2d218cef217b4f4b9655451483eb4bed |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-04-12T12:46:52Z |
| publishDate | 2022-10-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-2d218cef217b4f4b9655451483eb4bed2022-12-22T03:32:36ZengNature PortfolioNature Communications2041-17232022-10-0113111410.1038/s41467-022-33691-1Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopyJack E. N. Swallow0Michael W. Fraser1Nis-Julian H. Kneusels2Jodie F. Charlton3Christopher G. Sole4Conor M. E. Phelan5Erik Björklund6Peter Bencok7Carlos Escudero8Virginia Pérez-Dieste9Clare P. Grey10Rebecca J. Nicholls11Robert S. Weatherup12Department of Materials, University of OxfordDepartment of Materials, University of OxfordDepartment of Chemistry, University of CambridgeDepartment of Materials, University of OxfordDiamond Light Source, DidcotDepartment of Materials, University of OxfordDepartment of Materials, University of OxfordDiamond Light Source, DidcotALBA Synchrotron Light SourceALBA Synchrotron Light SourceDepartment of Chemistry, University of CambridgeDepartment of Materials, University of OxfordDepartment of Materials, University of OxfordSolid electrolyte interphase (SEI) formation on Li-ion battery anodes is critical for long-term performance. Here, the authors use operando soft X-ray absorption spectroscopy in total electron yield mode to resolve the chemical evolution of the SEI during electrochemical formation on silicon anodes.https://doi.org/10.1038/s41467-022-33691-1 |
| spellingShingle | Jack E. N. Swallow Michael W. Fraser Nis-Julian H. Kneusels Jodie F. Charlton Christopher G. Sole Conor M. E. Phelan Erik Björklund Peter Bencok Carlos Escudero Virginia Pérez-Dieste Clare P. Grey Rebecca J. Nicholls Robert S. Weatherup Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy Nature Communications |
| title | Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy |
| title_full | Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy |
| title_fullStr | Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy |
| title_full_unstemmed | Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy |
| title_short | Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy |
| title_sort | revealing solid electrolyte interphase formation through interface sensitive operando x ray absorption spectroscopy |
| url | https://doi.org/10.1038/s41467-022-33691-1 |
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