The envelope Hamiltonian for electron interaction with ultrashort pulses

For ultrashort VUV pulses with a pulse length comparable to the orbital time of the bound electrons they couple to, we propose a simplified envelope Hamiltonian. It is based on the Kramers–Henneberger representation in connection with a Floquet expansion of the strong-field dynamics but keeps the ti...

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Main Authors: Koudai Toyota, Ulf Saalmann, Jan M Rost
Format: Article
Language:English
Published: IOP Publishing 2015-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/17/7/073005
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author Koudai Toyota
Ulf Saalmann
Jan M Rost
author_facet Koudai Toyota
Ulf Saalmann
Jan M Rost
author_sort Koudai Toyota
collection DOAJ
description For ultrashort VUV pulses with a pulse length comparable to the orbital time of the bound electrons they couple to, we propose a simplified envelope Hamiltonian. It is based on the Kramers–Henneberger representation in connection with a Floquet expansion of the strong-field dynamics but keeps the time dependence of the pulse envelope explicit. Thereby, the envelope Hamiltonian captures the essence of the physics—light-induced shifts of bound states, single-photon absorption, and non-adiabatic electronic transitions. It delivers quantitatively accurate ionization dynamics and allows for a physical insight into the processes occurring. Its minimal requirements for construction in terms of laser parameters make it ideally suited for a large class of atomic and molecular problems.
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spelling doaj.art-2ecdf51258ef41af8fd65c7d8598963e2023-08-08T14:19:19ZengIOP PublishingNew Journal of Physics1367-26302015-01-0117707300510.1088/1367-2630/17/7/073005The envelope Hamiltonian for electron interaction with ultrashort pulsesKoudai Toyota0Ulf Saalmann1Jan M Rost2Max Planck Institute for the Physics of Complex Systems, Nöthnitzer Straße 38, D-01187 Dresden, GermanyMax Planck Institute for the Physics of Complex Systems, Nöthnitzer Straße 38, D-01187 Dresden, GermanyMax Planck Institute for the Physics of Complex Systems, Nöthnitzer Straße 38, D-01187 Dresden, GermanyFor ultrashort VUV pulses with a pulse length comparable to the orbital time of the bound electrons they couple to, we propose a simplified envelope Hamiltonian. It is based on the Kramers–Henneberger representation in connection with a Floquet expansion of the strong-field dynamics but keeps the time dependence of the pulse envelope explicit. Thereby, the envelope Hamiltonian captures the essence of the physics—light-induced shifts of bound states, single-photon absorption, and non-adiabatic electronic transitions. It delivers quantitatively accurate ionization dynamics and allows for a physical insight into the processes occurring. Its minimal requirements for construction in terms of laser parameters make it ideally suited for a large class of atomic and molecular problems.https://doi.org/10.1088/1367-2630/17/7/073005photo-ionizationfree-electrons laserFloquet expansionlight–matter coupling33.60.+q32.80.Wr
spellingShingle Koudai Toyota
Ulf Saalmann
Jan M Rost
The envelope Hamiltonian for electron interaction with ultrashort pulses
New Journal of Physics
photo-ionization
free-electrons laser
Floquet expansion
light–matter coupling
33.60.+q
32.80.Wr
title The envelope Hamiltonian for electron interaction with ultrashort pulses
title_full The envelope Hamiltonian for electron interaction with ultrashort pulses
title_fullStr The envelope Hamiltonian for electron interaction with ultrashort pulses
title_full_unstemmed The envelope Hamiltonian for electron interaction with ultrashort pulses
title_short The envelope Hamiltonian for electron interaction with ultrashort pulses
title_sort envelope hamiltonian for electron interaction with ultrashort pulses
topic photo-ionization
free-electrons laser
Floquet expansion
light–matter coupling
33.60.+q
32.80.Wr
url https://doi.org/10.1088/1367-2630/17/7/073005
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