A thin-film broadband perfect absorber based on plasmonic copper nanoparticles
Increasing the efficiency of solar thermal collectors is extremely important as they are essential for many applications, ranging from the UV up to the NIR spectral range, from water heating systems up to micro-electromechanical systems. In this work, a plasmonic multilayer nanocomposite thin-film s...
主要な著者: | , , , , , , , |
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フォーマット: | 論文 |
言語: | English |
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Elsevier
2022-08-01
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シリーズ: | Micro and Nano Engineering |
主題: | |
オンライン・アクセス: | http://www.sciencedirect.com/science/article/pii/S259000722200051X |
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author | Nanda Perdana Jonas Drewes Felix Pohl Alexander Vahl Thomas Strunskus Mady Elbahri Carsten Rockstuhl Franz Faupel |
author_facet | Nanda Perdana Jonas Drewes Felix Pohl Alexander Vahl Thomas Strunskus Mady Elbahri Carsten Rockstuhl Franz Faupel |
author_sort | Nanda Perdana |
collection | DOAJ |
description | Increasing the efficiency of solar thermal collectors is extremely important as they are essential for many applications, ranging from the UV up to the NIR spectral range, from water heating systems up to micro-electromechanical systems. In this work, a plasmonic multilayer nanocomposite thin-film system that efficiently absorbs solar radiation across an extended spectral range was simulated and experimentally tested. Novel to our approach, copper nanoparticles in an alumina matrix were chosen as the nanocomposite material. Compared to other plasmonic materials such as gold or silver, copper is more abundant and economic. The alumina matrix provides high thermal stability, good optical properties, and corrosion protection. Using a multiscale-modeling approach, we inspect on computational grounds the effect of the nanoparticle filling factor, the angle of incidence, and the thin-film thicknesses on the absorber performance. We found that an optimally designed device absorbs up to 90% light energy from 200 nm to 1800 nm. To validate the simulations, two promising absorber layouts are experimentally realized. Their performance compares very well with simulations. |
first_indexed | 2024-12-10T15:46:26Z |
format | Article |
id | doaj.art-2f1e4787b51a4104a2cf415151f6acab |
institution | Directory Open Access Journal |
issn | 2590-0072 |
language | English |
last_indexed | 2024-12-10T15:46:26Z |
publishDate | 2022-08-01 |
publisher | Elsevier |
record_format | Article |
series | Micro and Nano Engineering |
spelling | doaj.art-2f1e4787b51a4104a2cf415151f6acab2022-12-22T01:42:56ZengElsevierMicro and Nano Engineering2590-00722022-08-0116100154A thin-film broadband perfect absorber based on plasmonic copper nanoparticlesNanda Perdana0Jonas Drewes1Felix Pohl2Alexander Vahl3Thomas Strunskus4Mady Elbahri5Carsten Rockstuhl6Franz Faupel7Institute of Theoretical Solid State Physics, Karlsruhe Institute of Technology (KIT), Karlsruhe 76137, Germany; Corresponding author.Institute of Material Science, Chair for Multicomponent Materials, Kiel University, Kiel 24143, GermanyInstitute of Material Science, Chair for Multicomponent Materials, Kiel University, Kiel 24143, GermanyInstitute of Material Science, Chair for Multicomponent Materials, Kiel University, Kiel 24143, GermanyInstitute of Material Science, Chair for Multicomponent Materials, Kiel University, Kiel 24143, GermanyNanochemistry and Nanoengineering, School of Chemical Engineering, Department of Chemistry and Materials Science, Aalto University, Aalto 00076, FinlandInstitute of Theoretical Solid State Physics, Karlsruhe Institute of Technology (KIT), Karlsruhe 76137, Germany; Institute of Nanotechnology, Karlsruhe Institute of Technology (KIT), Karlsruhe 76021, GermanyInstitute of Material Science, Chair for Multicomponent Materials, Kiel University, Kiel 24143, GermanyIncreasing the efficiency of solar thermal collectors is extremely important as they are essential for many applications, ranging from the UV up to the NIR spectral range, from water heating systems up to micro-electromechanical systems. In this work, a plasmonic multilayer nanocomposite thin-film system that efficiently absorbs solar radiation across an extended spectral range was simulated and experimentally tested. Novel to our approach, copper nanoparticles in an alumina matrix were chosen as the nanocomposite material. Compared to other plasmonic materials such as gold or silver, copper is more abundant and economic. The alumina matrix provides high thermal stability, good optical properties, and corrosion protection. Using a multiscale-modeling approach, we inspect on computational grounds the effect of the nanoparticle filling factor, the angle of incidence, and the thin-film thicknesses on the absorber performance. We found that an optimally designed device absorbs up to 90% light energy from 200 nm to 1800 nm. To validate the simulations, two promising absorber layouts are experimentally realized. Their performance compares very well with simulations.http://www.sciencedirect.com/science/article/pii/S259000722200051X36.40.Vz78.20.−e78.20.Ci78.40.−q78.66.−w78.66.Bz |
spellingShingle | Nanda Perdana Jonas Drewes Felix Pohl Alexander Vahl Thomas Strunskus Mady Elbahri Carsten Rockstuhl Franz Faupel A thin-film broadband perfect absorber based on plasmonic copper nanoparticles Micro and Nano Engineering 36.40.Vz 78.20.−e 78.20.Ci 78.40.−q 78.66.−w 78.66.Bz |
title | A thin-film broadband perfect absorber based on plasmonic copper nanoparticles |
title_full | A thin-film broadband perfect absorber based on plasmonic copper nanoparticles |
title_fullStr | A thin-film broadband perfect absorber based on plasmonic copper nanoparticles |
title_full_unstemmed | A thin-film broadband perfect absorber based on plasmonic copper nanoparticles |
title_short | A thin-film broadband perfect absorber based on plasmonic copper nanoparticles |
title_sort | thin film broadband perfect absorber based on plasmonic copper nanoparticles |
topic | 36.40.Vz 78.20.−e 78.20.Ci 78.40.−q 78.66.−w 78.66.Bz |
url | http://www.sciencedirect.com/science/article/pii/S259000722200051X |
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