Single-Step Organization of Plasmonic Gold Metamaterials with Self-Assembled DNA Nanostructures

Self-assembled DNA nanostructures hold great promise as nanoscale templates for organizing nanoparticles (NPs) with near-atomistic resolution. However, large-scale organization of NPs with high yield is highly desirable for nanoelectronics and nanophotonic applications. Here, we design five-strand D...

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Bibliographic Details
Main Authors: Shaokang Ren, Jun Wang, Chunyuan Song, Qian Li, Yanjun Yang, Nan Teng, Shao Su, Dan Zhu, Wei Huang, Jie Chao, Lianhui Wang, Chunhai Fan
Format: Article
Language:English
Published: American Association for the Advancement of Science (AAAS) 2019-01-01
Series:Research
Online Access:http://dx.doi.org/10.34133/2019/7403580
Description
Summary:Self-assembled DNA nanostructures hold great promise as nanoscale templates for organizing nanoparticles (NPs) with near-atomistic resolution. However, large-scale organization of NPs with high yield is highly desirable for nanoelectronics and nanophotonic applications. Here, we design five-strand DNA tiles that can readily self-assemble into well-organized micrometer-scale DNA nanostructures. By organizing gold nanoparticles (AuNPs) on these self-assembled DNA nanostructures, we realize the fabrication of one- and two-dimensional Au nanostructures in single steps. We further demonstrate the one-pot synthesis of Au metamaterials for highly amplified surface-enhanced Raman Scattering (SERS). This single-step and high-yield strategy thus holds great potential for fabricating plasmonic metamaterials.
ISSN:2639-5274