Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution

Field measurements of aerosols were conducted on Xiaoyangshan Island in the East China Sea in May 2006 to investigate the impact of anthropogenic air pollutants to the coastal environment. MM5/CMAQ was used to model the development of the episode and identify the sources of major ionic species durin...

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Main Authors: Yan Zhang, Qi Yu, Wei-Chun Ma, Li-Min Chen
Format: Article
Language:English
Published: Springer 2010-01-01
Series:Terrestrial, Atmospheric and Oceanic Sciences
Subjects:
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author Yan Zhang
Qi Yu
Wei-Chun Ma
Li-Min Chen
author_facet Yan Zhang
Qi Yu
Wei-Chun Ma
Li-Min Chen
author_sort Yan Zhang
collection DOAJ
description Field measurements of aerosols were conducted on Xiaoyangshan Island in the East China Sea in May 2006 to investigate the impact of anthropogenic air pollutants to the coastal environment. MM5/CMAQ was used to model the development of the episode and identify the sources of major ionic species during the episode. The results showed that the major ionic species in TSP were SO42-, NO3- and NH4+, which accounted for about 76% of the total water soluble ions (TWSI). The mean concentrations of SO42-, NO3- and NH4+ were 20.9, 10.4 and 5.1 £gg m-3, respectively, and the peak values on a foggy day were 69.87, 38.48 and 22.75 £gg m-3, respectively. The most abundant ionic species was SO42-. The increase of SO42- concentration was found to be significantly correlated with the decrease of the atmospheric visibility (correlation coefficient = 0.82). Process analysis implied that advection, diffusion and cloud chemical processes contributed to this pollution episode. Backward trajectory analysis revealed that the airflow on the foggy and most polluted day during the sampling campaign was westerly, i.e., from the continent. Both the measured data and modeling results showed that the coastal atmosphere was seriously affected by terrestrial pollutants in the continental outflow.
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spelling doaj.art-323f1fea488f49bcb44181b5f8b848302022-12-22T02:09:37ZengSpringerTerrestrial, Atmospheric and Oceanic Sciences1017-08392311-76802010-01-0121690510.3319/TAO.2010.03.22.01(A)979Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air PollutionYan ZhangQi YuWei-Chun MaLi-Min ChenField measurements of aerosols were conducted on Xiaoyangshan Island in the East China Sea in May 2006 to investigate the impact of anthropogenic air pollutants to the coastal environment. MM5/CMAQ was used to model the development of the episode and identify the sources of major ionic species during the episode. The results showed that the major ionic species in TSP were SO42-, NO3- and NH4+, which accounted for about 76% of the total water soluble ions (TWSI). The mean concentrations of SO42-, NO3- and NH4+ were 20.9, 10.4 and 5.1 £gg m-3, respectively, and the peak values on a foggy day were 69.87, 38.48 and 22.75 £gg m-3, respectively. The most abundant ionic species was SO42-. The increase of SO42- concentration was found to be significantly correlated with the decrease of the atmospheric visibility (correlation coefficient = 0.82). Process analysis implied that advection, diffusion and cloud chemical processes contributed to this pollution episode. Backward trajectory analysis revealed that the airflow on the foggy and most polluted day during the sampling campaign was westerly, i.e., from the continent. Both the measured data and modeling results showed that the coastal atmosphere was seriously affected by terrestrial pollutants in the continental outflow.Marine aerosolContinental outflowEast China Sea
spellingShingle Yan Zhang
Qi Yu
Wei-Chun Ma
Li-Min Chen
Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
Terrestrial, Atmospheric and Oceanic Sciences
Marine aerosol
Continental outflow
East China Sea
title Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
title_full Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
title_fullStr Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
title_full_unstemmed Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
title_short Influence of Continental Outflows on Marine Aerosols over Xiaoyangshan Island in the East China Sea: An Episode of Heavy Air Pollution
title_sort influence of continental outflows on marine aerosols over xiaoyangshan island in the east china sea an episode of heavy air pollution
topic Marine aerosol
Continental outflow
East China Sea
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AT weichunma influenceofcontinentaloutflowsonmarineaerosolsoverxiaoyangshanislandintheeastchinaseaanepisodeofheavyairpollution
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