Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping

Abstract Optically induced nuclear spin–spin coupling in semiconductors is expected to serve for gate operations in nuclear-magnetic-resonance (NMR) quantum computations. However, not much is known about its characteristics. In this study, we investigate optically induced couplings in GaAs via doubl...

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Main Authors: Atsushi Goto, Kenjiro Hashi, Shinobu Ohki, Tadashi Shimizu
Format: Article
Language:English
Published: Nature Portfolio 2022-05-01
Series:npj Quantum Information
Online Access:https://doi.org/10.1038/s41534-022-00571-x
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author Atsushi Goto
Kenjiro Hashi
Shinobu Ohki
Tadashi Shimizu
author_facet Atsushi Goto
Kenjiro Hashi
Shinobu Ohki
Tadashi Shimizu
author_sort Atsushi Goto
collection DOAJ
description Abstract Optically induced nuclear spin–spin coupling in semiconductors is expected to serve for gate operations in nuclear-magnetic-resonance (NMR) quantum computations. However, not much is known about its characteristics. In this study, we investigate optically induced couplings in GaAs via double-resonance spin-echo decay experiments under optical pumping. The squared echo decay rate $$\left( {1/T_2} \right)^2$$ 1 / T 2 2 of 71Ga measured under various light powers revealed that optically induced couplings increase with increasing light power, and the sign of heteronuclear couplings between Ga–As pairs is opposite to that of dipolar couplings, which cancel each other out. Under higher light power, the optically induced “controllable” coupling is expected to eventually surpass the “uncontrollable” nuclear dipolar coupling, becoming dominant, which is preferable for the gate operation in NMR quantum computation.
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spelling doaj.art-328fa02382064caa834ba15d1f3bb42e2022-12-22T02:34:24ZengNature Portfolionpj Quantum Information2056-63872022-05-01811610.1038/s41534-022-00571-xOptically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumpingAtsushi Goto0Kenjiro Hashi1Shinobu Ohki2Tadashi Shimizu3National Institute for Materials ScienceNational Institute for Materials ScienceNational Institute for Materials ScienceNational Institute for Materials ScienceAbstract Optically induced nuclear spin–spin coupling in semiconductors is expected to serve for gate operations in nuclear-magnetic-resonance (NMR) quantum computations. However, not much is known about its characteristics. In this study, we investigate optically induced couplings in GaAs via double-resonance spin-echo decay experiments under optical pumping. The squared echo decay rate $$\left( {1/T_2} \right)^2$$ 1 / T 2 2 of 71Ga measured under various light powers revealed that optically induced couplings increase with increasing light power, and the sign of heteronuclear couplings between Ga–As pairs is opposite to that of dipolar couplings, which cancel each other out. Under higher light power, the optically induced “controllable” coupling is expected to eventually surpass the “uncontrollable” nuclear dipolar coupling, becoming dominant, which is preferable for the gate operation in NMR quantum computation.https://doi.org/10.1038/s41534-022-00571-x
spellingShingle Atsushi Goto
Kenjiro Hashi
Shinobu Ohki
Tadashi Shimizu
Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
npj Quantum Information
title Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
title_full Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
title_fullStr Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
title_full_unstemmed Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
title_short Optically induced nuclear spin–spin couplings in GaAs manifested by spin echo decays under optical pumping
title_sort optically induced nuclear spin spin couplings in gaas manifested by spin echo decays under optical pumping
url https://doi.org/10.1038/s41534-022-00571-x
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AT tadashishimizu opticallyinducednuclearspinspincouplingsingaasmanifestedbyspinechodecaysunderopticalpumping