Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity
We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correla...
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| Format: | Article |
| Language: | English |
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SciPost
2023-10-01
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| Series: | SciPost Physics |
| Online Access: | https://scipost.org/SciPostPhys.15.4.138 |
| _version_ | 1797665745116594176 |
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| author | Megha Gopalakrishna, Emil Viñas Boström, Claudio Verdozzi |
| author_facet | Megha Gopalakrishna, Emil Viñas Boström, Claudio Verdozzi |
| author_sort | Megha Gopalakrishna, Emil Viñas Boström, Claudio Verdozzi |
| collection | DOAJ |
| description | We introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay. |
| first_indexed | 2024-03-11T19:48:15Z |
| format | Article |
| id | doaj.art-3424bb0780ce4e9290264ac16b5027f7 |
| institution | Directory Open Access Journal |
| issn | 2542-4653 |
| language | English |
| last_indexed | 2024-03-11T19:48:15Z |
| publishDate | 2023-10-01 |
| publisher | SciPost |
| record_format | Article |
| series | SciPost Physics |
| spelling | doaj.art-3424bb0780ce4e9290264ac16b5027f72023-10-05T14:18:55ZengSciPostSciPost Physics2542-46532023-10-0115413810.21468/SciPostPhys.15.4.138Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavityMegha Gopalakrishna, Emil Viñas Boström, Claudio VerdozziWe introduce a model description of a diatomic molecule in an optical cavity, with pump and fluorescent fields, and electron and nuclear motion are treated on equal footing and exactly. The model accounts for several optical response temporal scenarios: A Mollow spectrum hindered by electron correlations, a competition of harmonic generation and molecular dissociation, a dependence of fluorescence on photon pumping rate and dissipation. It is thus a general and flexible template for insight into experiments where quantum photon confinement, leakage, nuclear motion and electronic correlations are at interplay.https://scipost.org/SciPostPhys.15.4.138 |
| spellingShingle | Megha Gopalakrishna, Emil Viñas Boström, Claudio Verdozzi Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity SciPost Physics |
| title | Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| title_full | Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| title_fullStr | Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| title_full_unstemmed | Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| title_short | Photon pumping, photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| title_sort | photon pumping photodissociation and dissipation at interplay for the fluorescence of a molecule in a cavity |
| url | https://scipost.org/SciPostPhys.15.4.138 |
| work_keys_str_mv | AT meghagopalakrishnaemilvinasbostromclaudioverdozzi photonpumpingphotodissociationanddissipationatinterplayforthefluorescenceofamoleculeinacavity |