Preparation of a graphene oxide membrane for air purification

Environmental issues such as particulate matter (PM) have become more and more serious because of their detrimental effects on human health. The development of an effective way to remove PM is in high demand. In this study, a graphene oxide (GO) membrane with a large specific surface area and a cont...

Full description

Bibliographic Details
Main Authors: Weiwu Zou, Baoshan Gu, Shiqing Sun, Shidong Wang, Xin Li, Haoqi Zhao, Peiyan Yang
Format: Article
Language:English
Published: IOP Publishing 2019-01-01
Series:Materials Research Express
Subjects:
Online Access:https://doi.org/10.1088/2053-1591/ab3eec
_version_ 1797747221820604416
author Weiwu Zou
Baoshan Gu
Shiqing Sun
Shidong Wang
Xin Li
Haoqi Zhao
Peiyan Yang
author_facet Weiwu Zou
Baoshan Gu
Shiqing Sun
Shidong Wang
Xin Li
Haoqi Zhao
Peiyan Yang
author_sort Weiwu Zou
collection DOAJ
description Environmental issues such as particulate matter (PM) have become more and more serious because of their detrimental effects on human health. The development of an effective way to remove PM is in high demand. In this study, a graphene oxide (GO) membrane with a large specific surface area and a continuous pore structure was prepared via a coating method. The morphology, composition and structure of the GO membrane were characterized by scanning electron microscopy (SEM), an energy dispersive spectrometer (EDS), X-ray diffraction (XRD), FT-IR spectra, X-ray photoelectron spectra (XPS) and Raman spectroscopy. The removal efficiency for PM and the influence of pollutant concentration and wind velocity on the GO membrane were studied. As a result, when the wind velocity was 0.1 m s ^−1 , the PM _2.5 removal efficiency of the GO membrane exhibited the highest efficiency (99.46%) with a low pressure drop (7 Pa) and a high quality factor (QF) of 0.75 Pa ^−1 . The GO membrane maintained a high adsorption performance for a long time. The GO membrane removal efficiency was more significant when the import concentration was higher and the wind velocity was lower. In particular, SEM and EDS clearly revealed that the PM _2.5 was successfully captured by the GO membrane. The preparation of the GO membrane involves a simple and pollution-free process, which provides a new way to deal with air pollution.
first_indexed 2024-03-12T15:47:44Z
format Article
id doaj.art-34f08ba04f1e4ff4a85db37a823d36e4
institution Directory Open Access Journal
issn 2053-1591
language English
last_indexed 2024-03-12T15:47:44Z
publishDate 2019-01-01
publisher IOP Publishing
record_format Article
series Materials Research Express
spelling doaj.art-34f08ba04f1e4ff4a85db37a823d36e42023-08-09T15:20:48ZengIOP PublishingMaterials Research Express2053-15912019-01-0161010562410.1088/2053-1591/ab3eecPreparation of a graphene oxide membrane for air purificationWeiwu Zou0https://orcid.org/0000-0001-7776-2706Baoshan Gu1Shiqing Sun2Shidong Wang3Xin Li4Haoqi Zhao5Peiyan Yang6School of Materials Science and Engineering, Hebei University of Science & Technology , Shijiazhuang 050000, People’s Republic of China; National Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaNational Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaSchool of Materials Science and Engineering, Hebei University of Science & Technology , Shijiazhuang 050000, People’s Republic of ChinaSchool of Materials Science and Engineering, Hebei University of Science & Technology , Shijiazhuang 050000, People’s Republic of China; National Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaNational Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaNational Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaNational Engineering Laboratory for Advanced Coatings Technology of Metal Materials, China Iron and Steel Research Institute Group, Beijing 100081, People’s Republic of ChinaEnvironmental issues such as particulate matter (PM) have become more and more serious because of their detrimental effects on human health. The development of an effective way to remove PM is in high demand. In this study, a graphene oxide (GO) membrane with a large specific surface area and a continuous pore structure was prepared via a coating method. The morphology, composition and structure of the GO membrane were characterized by scanning electron microscopy (SEM), an energy dispersive spectrometer (EDS), X-ray diffraction (XRD), FT-IR spectra, X-ray photoelectron spectra (XPS) and Raman spectroscopy. The removal efficiency for PM and the influence of pollutant concentration and wind velocity on the GO membrane were studied. As a result, when the wind velocity was 0.1 m s ^−1 , the PM _2.5 removal efficiency of the GO membrane exhibited the highest efficiency (99.46%) with a low pressure drop (7 Pa) and a high quality factor (QF) of 0.75 Pa ^−1 . The GO membrane maintained a high adsorption performance for a long time. The GO membrane removal efficiency was more significant when the import concentration was higher and the wind velocity was lower. In particular, SEM and EDS clearly revealed that the PM _2.5 was successfully captured by the GO membrane. The preparation of the GO membrane involves a simple and pollution-free process, which provides a new way to deal with air pollution.https://doi.org/10.1088/2053-1591/ab3eecgraphene oxidemembranecoatingair purificationparticulate matter
spellingShingle Weiwu Zou
Baoshan Gu
Shiqing Sun
Shidong Wang
Xin Li
Haoqi Zhao
Peiyan Yang
Preparation of a graphene oxide membrane for air purification
Materials Research Express
graphene oxide
membrane
coating
air purification
particulate matter
title Preparation of a graphene oxide membrane for air purification
title_full Preparation of a graphene oxide membrane for air purification
title_fullStr Preparation of a graphene oxide membrane for air purification
title_full_unstemmed Preparation of a graphene oxide membrane for air purification
title_short Preparation of a graphene oxide membrane for air purification
title_sort preparation of a graphene oxide membrane for air purification
topic graphene oxide
membrane
coating
air purification
particulate matter
url https://doi.org/10.1088/2053-1591/ab3eec
work_keys_str_mv AT weiwuzou preparationofagrapheneoxidemembraneforairpurification
AT baoshangu preparationofagrapheneoxidemembraneforairpurification
AT shiqingsun preparationofagrapheneoxidemembraneforairpurification
AT shidongwang preparationofagrapheneoxidemembraneforairpurification
AT xinli preparationofagrapheneoxidemembraneforairpurification
AT haoqizhao preparationofagrapheneoxidemembraneforairpurification
AT peiyanyang preparationofagrapheneoxidemembraneforairpurification