Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2}
A triangular-lattice antiferromagnet of Ag_{2}FeO_{2} was synthesized under high pressure. Its magnetism was studied in terms of electrical resistivity, magnetic susceptibility, heat capacity, powder neutron scattering, and Mössbauer spectroscopy. The magnetic state of Ag_{2}FeO_{2} changes successi...
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Format: | Article |
Language: | English |
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American Physical Society
2020-11-01
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Series: | Physical Review Research |
Online Access: | http://doi.org/10.1103/PhysRevResearch.2.043211 |
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author | H. K. Yoshida M. Matsuda M. B. Stone C. R. dela Cruz T. Furubayashi M. Onoda E. Takayama-Muromachi M. Isobe |
author_facet | H. K. Yoshida M. Matsuda M. B. Stone C. R. dela Cruz T. Furubayashi M. Onoda E. Takayama-Muromachi M. Isobe |
author_sort | H. K. Yoshida |
collection | DOAJ |
description | A triangular-lattice antiferromagnet of Ag_{2}FeO_{2} was synthesized under high pressure. Its magnetism was studied in terms of electrical resistivity, magnetic susceptibility, heat capacity, powder neutron scattering, and Mössbauer spectroscopy. The magnetic state of Ag_{2}FeO_{2} changes successively through a second-order phase transition at T_{p}=36 K and a crossover at T_{c}=20 K. A partially disordered (PD) state appears below T_{p}, in which ≈2/3 spins are ordered and the remaining ≈1/3 spins fluctuate, which state persists at least down to 5 K. The spin correlation length starts to grow at T_{p}; however, it remains very short (≈27 Å) below T_{c}. This exotic magnetism is concerned with strong frustration in the classic antiferromagnetic triangular lattice. |
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language | English |
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spelling | doaj.art-3504bea4b9174527a4b3ad0a887e74042024-04-12T17:03:43ZengAmerican Physical SocietyPhysical Review Research2643-15642020-11-012404321110.1103/PhysRevResearch.2.043211Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2}H. K. YoshidaM. MatsudaM. B. StoneC. R. dela CruzT. FurubayashiM. OnodaE. Takayama-MuromachiM. IsobeA triangular-lattice antiferromagnet of Ag_{2}FeO_{2} was synthesized under high pressure. Its magnetism was studied in terms of electrical resistivity, magnetic susceptibility, heat capacity, powder neutron scattering, and Mössbauer spectroscopy. The magnetic state of Ag_{2}FeO_{2} changes successively through a second-order phase transition at T_{p}=36 K and a crossover at T_{c}=20 K. A partially disordered (PD) state appears below T_{p}, in which ≈2/3 spins are ordered and the remaining ≈1/3 spins fluctuate, which state persists at least down to 5 K. The spin correlation length starts to grow at T_{p}; however, it remains very short (≈27 Å) below T_{c}. This exotic magnetism is concerned with strong frustration in the classic antiferromagnetic triangular lattice.http://doi.org/10.1103/PhysRevResearch.2.043211 |
spellingShingle | H. K. Yoshida M. Matsuda M. B. Stone C. R. dela Cruz T. Furubayashi M. Onoda E. Takayama-Muromachi M. Isobe Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} Physical Review Research |
title | Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} |
title_full | Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} |
title_fullStr | Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} |
title_full_unstemmed | Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} |
title_short | Partially disordered state with short-range spin correlation in S=5/2 classical triangular antiferromagnet Ag_{2}FeO_{2} |
title_sort | partially disordered state with short range spin correlation in s 5 2 classical triangular antiferromagnet ag 2 feo 2 |
url | http://doi.org/10.1103/PhysRevResearch.2.043211 |
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