Synthesizing optical spectra using computer-generated holography techniques

Experimental control and detection of atoms and molecules often rely on optical transitions between different electronic states. In many cases, substructure such as hyperfine or spin-rotation structure leads to the need for multiple optical frequencies spaced by MHz to GHz. The task of creating mult...

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Main Authors: Connor M Holland, Yukai Lu, Lawrence W Cheuk
Format: Article
Language:English
Published: IOP Publishing 2021-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/abe973
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author Connor M Holland
Yukai Lu
Lawrence W Cheuk
author_facet Connor M Holland
Yukai Lu
Lawrence W Cheuk
author_sort Connor M Holland
collection DOAJ
description Experimental control and detection of atoms and molecules often rely on optical transitions between different electronic states. In many cases, substructure such as hyperfine or spin-rotation structure leads to the need for multiple optical frequencies spaced by MHz to GHz. The task of creating multiple optical frequencies—optical spectral engineering—becomes challenging when the number of frequencies becomes large, a situation that one could encounter in complex molecules and atoms in large magnetic fields. In this work, we point out a novel mapping between computer-generated holography (CGH) and spectrum generation via phase modulation, which is an established technique. Using this mapping, we synthesize arbitrary optical spectra by modulating a monochromatic light field with a time-dependent phase generated through CGH techniques. Our method is compatible with non-linear optical processes such as sum frequency generation and second harmonic generation. Additional requirements that arise from the finite lifetimes of excited states can also be satisfied in our approach. As a proof-of-principle demonstration, we generate spectra suitable for cycling photons on the X – B transition in CaF, and verify via optical Bloch equation simulations that one can achieve high photon scattering rates, which are important for fluorescent detection and laser cooling. Our method could offer significant simplifications in future experiments that would otherwise be prohibitively complex.
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spelling doaj.art-352c74e8510041f3ac6286a910b7ca1a2023-08-08T15:31:52ZengIOP PublishingNew Journal of Physics1367-26302021-01-0123303302810.1088/1367-2630/abe973Synthesizing optical spectra using computer-generated holography techniquesConnor M Holland0https://orcid.org/0000-0003-1759-5912Yukai Lu1https://orcid.org/0000-0001-7404-0767Lawrence W Cheuk2https://orcid.org/0000-0002-8329-8812Department of Physics, Princeton University , Princeton, NJ 08544, United States of AmericaDepartment of Physics, Princeton University , Princeton, NJ 08544, United States of America; Department of Electrical and Computer Engineering, Princeton University , Princeton NJ 08544, United States of AmericaDepartment of Physics, Princeton University , Princeton, NJ 08544, United States of AmericaExperimental control and detection of atoms and molecules often rely on optical transitions between different electronic states. In many cases, substructure such as hyperfine or spin-rotation structure leads to the need for multiple optical frequencies spaced by MHz to GHz. The task of creating multiple optical frequencies—optical spectral engineering—becomes challenging when the number of frequencies becomes large, a situation that one could encounter in complex molecules and atoms in large magnetic fields. In this work, we point out a novel mapping between computer-generated holography (CGH) and spectrum generation via phase modulation, which is an established technique. Using this mapping, we synthesize arbitrary optical spectra by modulating a monochromatic light field with a time-dependent phase generated through CGH techniques. Our method is compatible with non-linear optical processes such as sum frequency generation and second harmonic generation. Additional requirements that arise from the finite lifetimes of excited states can also be satisfied in our approach. As a proof-of-principle demonstration, we generate spectra suitable for cycling photons on the X – B transition in CaF, and verify via optical Bloch equation simulations that one can achieve high photon scattering rates, which are important for fluorescent detection and laser cooling. Our method could offer significant simplifications in future experiments that would otherwise be prohibitively complex.https://doi.org/10.1088/1367-2630/abe973computer-generated holographylaser coolingultracold moleculeslight–matter interactionsultracold atoms
spellingShingle Connor M Holland
Yukai Lu
Lawrence W Cheuk
Synthesizing optical spectra using computer-generated holography techniques
New Journal of Physics
computer-generated holography
laser cooling
ultracold molecules
light–matter interactions
ultracold atoms
title Synthesizing optical spectra using computer-generated holography techniques
title_full Synthesizing optical spectra using computer-generated holography techniques
title_fullStr Synthesizing optical spectra using computer-generated holography techniques
title_full_unstemmed Synthesizing optical spectra using computer-generated holography techniques
title_short Synthesizing optical spectra using computer-generated holography techniques
title_sort synthesizing optical spectra using computer generated holography techniques
topic computer-generated holography
laser cooling
ultracold molecules
light–matter interactions
ultracold atoms
url https://doi.org/10.1088/1367-2630/abe973
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