Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi

We report on the structural and microscopic superconducting properties of the Ca_{1−x}Sr_{x}AlSi solid solution. Specifically, we have realized the continuous solid solution, which for all members, other than x=0 (CaAlSi), crystallizes in the AlB_{2}-type structure. For CaAlSi, we present an improve...

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Main Authors: Dorota I. Walicka, Zurab Guguchia, Jorge Lago, Olivier Blacque, KeYuan Ma, Huanlong Liu, Rustem Khasanov, Fabian O. von Rohr
Format: Article
Language:English
Published: American Physical Society 2021-08-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.3.033192
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author Dorota I. Walicka
Zurab Guguchia
Jorge Lago
Olivier Blacque
KeYuan Ma
Huanlong Liu
Rustem Khasanov
Fabian O. von Rohr
author_facet Dorota I. Walicka
Zurab Guguchia
Jorge Lago
Olivier Blacque
KeYuan Ma
Huanlong Liu
Rustem Khasanov
Fabian O. von Rohr
author_sort Dorota I. Walicka
collection DOAJ
description We report on the structural and microscopic superconducting properties of the Ca_{1−x}Sr_{x}AlSi solid solution. Specifically, we have realized the continuous solid solution, which for all members, other than x=0 (CaAlSi), crystallizes in the AlB_{2}-type structure. For CaAlSi, we present an improved structural model where all Al/Si layers are buckled, leading to a 6-folded structure along the crystallographic c direction. We, furthermore, find indications for the structural instability in the parent compound CaAlSi to enhance the superconductivity across the solid solution. Our investigation of the magnetic penetration depths by means of muon-spin rotation experiments reveals that CaAlSi is a two-gap superconductor, that SrAlSi is a single-gap superconductor, and that there is a continuous transition from one electronic state to the other across the solid solution. Hence, we show that the Ca_{1−x}Sr_{x}AlSi solid solution is a highly tunable two-gap to single-gap superconducting system on a honeycomb lattice, where the superconductivity is strongly connected to a structural instability, i.e., the buckling of the Al/Si layers.
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spelling doaj.art-35819b8faf474bb6b43288634b1bbb522024-04-12T17:13:21ZengAmerican Physical SocietyPhysical Review Research2643-15642021-08-013303319210.1103/PhysRevResearch.3.033192Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSiDorota I. WalickaZurab GuguchiaJorge LagoOlivier BlacqueKeYuan MaHuanlong LiuRustem KhasanovFabian O. von RohrWe report on the structural and microscopic superconducting properties of the Ca_{1−x}Sr_{x}AlSi solid solution. Specifically, we have realized the continuous solid solution, which for all members, other than x=0 (CaAlSi), crystallizes in the AlB_{2}-type structure. For CaAlSi, we present an improved structural model where all Al/Si layers are buckled, leading to a 6-folded structure along the crystallographic c direction. We, furthermore, find indications for the structural instability in the parent compound CaAlSi to enhance the superconductivity across the solid solution. Our investigation of the magnetic penetration depths by means of muon-spin rotation experiments reveals that CaAlSi is a two-gap superconductor, that SrAlSi is a single-gap superconductor, and that there is a continuous transition from one electronic state to the other across the solid solution. Hence, we show that the Ca_{1−x}Sr_{x}AlSi solid solution is a highly tunable two-gap to single-gap superconducting system on a honeycomb lattice, where the superconductivity is strongly connected to a structural instability, i.e., the buckling of the Al/Si layers.http://doi.org/10.1103/PhysRevResearch.3.033192
spellingShingle Dorota I. Walicka
Zurab Guguchia
Jorge Lago
Olivier Blacque
KeYuan Ma
Huanlong Liu
Rustem Khasanov
Fabian O. von Rohr
Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
Physical Review Research
title Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
title_full Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
title_fullStr Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
title_full_unstemmed Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
title_short Two-gap to single-gap superconducting transition on a honeycomb lattice in Ca_{1−x}Sr_{x}AlSi
title_sort two gap to single gap superconducting transition on a honeycomb lattice in ca 1 x sr x alsi
url http://doi.org/10.1103/PhysRevResearch.3.033192
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