Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment
Dynamics of the forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying and exposure in full-scale conditions has been estimated by the method of successive leaching. According to the results of the research the main part of the radionuclides (> 90 %) contin...
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Format: | Article |
Language: | English |
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Institute for Nuclear Research, National Academy of Sciences of Ukraine
2017-12-01
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Series: | Âderna Fìzika ta Energetika |
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Online Access: | http://jnpae.kinr.kiev.ua/18.4/html/18.4.0341.html |
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author | V. P. Protsak О. О. Odintsov Y. V. Khomutinin M. A. Jurba N. M. Prokopchuk V. O. Kashparov |
author_facet | V. P. Protsak О. О. Odintsov Y. V. Khomutinin M. A. Jurba N. M. Prokopchuk V. O. Kashparov |
author_sort | V. P. Protsak |
collection | DOAJ |
description | Dynamics of the forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying and exposure in full-scale conditions has been estimated by the method of successive leaching. According to the results of the research the main part of the radionuclides (> 90 %) continues to be in the non-exchange state for 4 years after drying. Significant part of the radionuclides remains not recovered from the solid phase of bottom sediments of cooling pond of the ChNPP even after using "super-hard" extraction conditions. This indicates the presence of 90Sr, 238,239,240Pu, 241Am and part of 137Cs in the composition of chemically stable fuel particles. Therefore, this part of radionuclides can not be mobilized in natural conditions for dozens of years. The obtained results indicate that on the drained parts of the cooling pond bed of the ChNPP one should not expect significant increase of mobility and bioavailability of radionuclides in the next 5 - 10 years. |
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format | Article |
id | doaj.art-36a23bd81f244157866610a480e0580b |
institution | Directory Open Access Journal |
issn | 1818-331X 2074-0565 |
language | English |
last_indexed | 2024-12-22T19:08:01Z |
publishDate | 2017-12-01 |
publisher | Institute for Nuclear Research, National Academy of Sciences of Ukraine |
record_format | Article |
series | Âderna Fìzika ta Energetika |
spelling | doaj.art-36a23bd81f244157866610a480e0580b2022-12-21T18:15:45ZengInstitute for Nuclear Research, National Academy of Sciences of UkraineÂderna Fìzika ta Energetika1818-331X2074-05652017-12-01184341349Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experimentV. P. Protsak0О. О. Odintsov1Y. V. Khomutinin2M. A. Jurba3N. M. Prokopchuk4V. O. Kashparov5Ukrainian Institute of Agricultural Radiology, National University of Life and Environmental Sciences of Ukraine, Kyiv, Ukraine Institute of Safety of NPP, National Academy of Sciences of Ukraine, Kyiv, Ukraine Ukrainian Institute of Agricultural Radiology, National University of Life and Environmental Sciences of Ukraine, Kyiv, Ukraine Ukrainian Institute of Agricultural Radiology, National University of Life and Environmental Sciences of Ukraine, Kyiv, Ukraine Ukrainian Institute of Agricultural Radiology, National University of Life and Environmental Sciences of Ukraine, Kyiv, Ukraine Ukrainian Institute of Agricultural Radiology, National University of Life and Environmental Sciences of Ukraine, Kyiv, Ukraine Dynamics of the forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying and exposure in full-scale conditions has been estimated by the method of successive leaching. According to the results of the research the main part of the radionuclides (> 90 %) continues to be in the non-exchange state for 4 years after drying. Significant part of the radionuclides remains not recovered from the solid phase of bottom sediments of cooling pond of the ChNPP even after using "super-hard" extraction conditions. This indicates the presence of 90Sr, 238,239,240Pu, 241Am and part of 137Cs in the composition of chemically stable fuel particles. Therefore, this part of radionuclides can not be mobilized in natural conditions for dozens of years. The obtained results indicate that on the drained parts of the cooling pond bed of the ChNPP one should not expect significant increase of mobility and bioavailability of radionuclides in the next 5 - 10 years.http://jnpae.kinr.kiev.ua/18.4/html/18.4.0341.htmlsequential leaching of radionuclidesforms finding of radionuclidesradioactive contaminationbottom sedimentscooling pond of the ChNPP |
spellingShingle | V. P. Protsak О. О. Odintsov Y. V. Khomutinin M. A. Jurba N. M. Prokopchuk V. O. Kashparov Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment Âderna Fìzika ta Energetika sequential leaching of radionuclides forms finding of radionuclides radioactive contamination bottom sediments cooling pond of the ChNPP |
title | Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment |
title_full | Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment |
title_fullStr | Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment |
title_full_unstemmed | Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment |
title_short | Dynamics of physico-chemical forms of radionuclides in the bottom sediments of cooling pond of the ChNPP after their drying: 1. Model experiment |
title_sort | dynamics of physico chemical forms of radionuclides in the bottom sediments of cooling pond of the chnpp after their drying 1 model experiment |
topic | sequential leaching of radionuclides forms finding of radionuclides radioactive contamination bottom sediments cooling pond of the ChNPP |
url | http://jnpae.kinr.kiev.ua/18.4/html/18.4.0341.html |
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