Magnetocaloric effect and spin-strain coupling in the spin-nematic state of LiCuVO_{4}

We report on the magnetocaloric effect and ultrasound studies of the frustrated quasi-one-dimensional spin-1/2 compound LiCuVO_{4}, evidencing a spin-nematic state. The magnetic Grüneisen parameter diverges at the transition to the spin-nematic phase, μ_{0}H_{c3}≈40 T, showing quantum criticality ac...

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Bibliographic Details
Main Authors: M. Gen, T. Nomura, D. I. Gorbunov, S. Yasin, P. T. Cong, C. Dong, Y. Kohama, E. L. Green, J. M. Law, M. S. Henriques, J. Wosnitza, A. A. Zvyagin, V. O. Cheranovskii, R. K. Kremer, S. Zherlitsyn
Format: Article
Language:English
Published: American Physical Society 2019-10-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.1.033065
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Summary:We report on the magnetocaloric effect and ultrasound studies of the frustrated quasi-one-dimensional spin-1/2 compound LiCuVO_{4}, evidencing a spin-nematic state. The magnetic Grüneisen parameter diverges at the transition to the spin-nematic phase, μ_{0}H_{c3}≈40 T, showing quantum criticality accompanied by entropy accumulation. The observed high-field anomalies in the acoustic properties clearly evidence a strong involvement of the lattice in the spin dynamics. The theoretical approach, based on exchange-striction coupling with dipolar and quadrupolar contributions, suggests that the spin-dipole-strain and quadrupole-strain interactions govern the spin-nematicity in LiCuVO_{4}.
ISSN:2643-1564