Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations

Airborne particulate matter plays an important role in climate change and health impacts, and is generally irregularly shaped and/or forms agglomerates. These particles may be characterized through their light scattering signals. Two-dimensional angular scattering from such particles produce a speck...

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Main Authors: Jaeda M. Mendoza, Kenzie Chen, Sequoyah Walters, Emily Shipley, Kevin B. Aptowicz, Stephen Holler
Format: Article
Language:English
Published: MDPI AG 2022-10-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/27/19/6695
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author Jaeda M. Mendoza
Kenzie Chen
Sequoyah Walters
Emily Shipley
Kevin B. Aptowicz
Stephen Holler
author_facet Jaeda M. Mendoza
Kenzie Chen
Sequoyah Walters
Emily Shipley
Kevin B. Aptowicz
Stephen Holler
author_sort Jaeda M. Mendoza
collection DOAJ
description Airborne particulate matter plays an important role in climate change and health impacts, and is generally irregularly shaped and/or forms agglomerates. These particles may be characterized through their light scattering signals. Two-dimensional angular scattering from such particles produce a speckle pattern that is influenced by their morphology (shape and material composition). In what follows, we revisit morphological descriptors obtained from computationally generated light scattering patterns from aggregates of spherical particles. These descriptors are used as inputs to a multivariate statistical algorithm and then classified via supervised machine learning algorithms. The classification results show improved accuracy over previous efforts and demonstrate the utility of the proposed morphological descriptors.
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spelling doaj.art-37905c1fcd8744e78ca15d62b53af66c2023-11-23T21:15:44ZengMDPI AGMolecules1420-30492022-10-012719669510.3390/molecules27196695Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering SimulationsJaeda M. Mendoza0Kenzie Chen1Sequoyah Walters2Emily Shipley3Kevin B. Aptowicz4Stephen Holler5Department of Physics and Engineering Physics, Fordham University, Bronx, NY 10458, USADepartment of Physics and Engineering Physics, Fordham University, Bronx, NY 10458, USADepartment of Physics and Engineering, West Chester University, West Chester, PA 19383, USADepartment of Physics and Engineering Physics, Fordham University, Bronx, NY 10458, USADepartment of Physics and Engineering, West Chester University, West Chester, PA 19383, USADepartment of Physics and Engineering Physics, Fordham University, Bronx, NY 10458, USAAirborne particulate matter plays an important role in climate change and health impacts, and is generally irregularly shaped and/or forms agglomerates. These particles may be characterized through their light scattering signals. Two-dimensional angular scattering from such particles produce a speckle pattern that is influenced by their morphology (shape and material composition). In what follows, we revisit morphological descriptors obtained from computationally generated light scattering patterns from aggregates of spherical particles. These descriptors are used as inputs to a multivariate statistical algorithm and then classified via supervised machine learning algorithms. The classification results show improved accuracy over previous efforts and demonstrate the utility of the proposed morphological descriptors.https://www.mdpi.com/1420-3049/27/19/6695light scatteringaggregatesT-matrixmachine learningclassificationclusters
spellingShingle Jaeda M. Mendoza
Kenzie Chen
Sequoyah Walters
Emily Shipley
Kevin B. Aptowicz
Stephen Holler
Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
Molecules
light scattering
aggregates
T-matrix
machine learning
classification
clusters
title Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
title_full Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
title_fullStr Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
title_full_unstemmed Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
title_short Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations
title_sort classification of aggregates using multispectral two dimensional angular light scattering simulations
topic light scattering
aggregates
T-matrix
machine learning
classification
clusters
url https://www.mdpi.com/1420-3049/27/19/6695
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