Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
We demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequence...
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Format: | Article |
Language: | English |
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IOP Publishing
2018-01-01
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Series: | New Journal of Physics |
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Online Access: | https://doi.org/10.1088/1367-2630/aaa396 |
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author | Heinrich Stolz Florian Schöne Dirk Semkat |
author_facet | Heinrich Stolz Florian Schöne Dirk Semkat |
author_sort | Heinrich Stolz |
collection | DOAJ |
description | We demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequences for the observation of polariton effects are discussed. We find that an anti-crossing of photon and exciton dispersions exists only for states with main quantum numbers n > 28, so polariton effects do not play any role in the experiments reported up to now. |
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id | doaj.art-3960583e24164e40ada547857687b217 |
institution | Directory Open Access Journal |
issn | 1367-2630 |
language | English |
last_indexed | 2024-03-12T16:36:16Z |
publishDate | 2018-01-01 |
publisher | IOP Publishing |
record_format | Article |
series | New Journal of Physics |
spelling | doaj.art-3960583e24164e40ada547857687b2172023-08-08T14:51:06ZengIOP PublishingNew Journal of Physics1367-26302018-01-0120202301910.1088/1367-2630/aaa396Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effectHeinrich Stolz0Florian Schöne1Dirk Semkat2Institut für Physik, Universität Rostock , D-18051 Rostock, GermanyInstitut für Physik, Universität Rostock , D-18051 Rostock, GermanyInstitut für Physik, Universität Rostock , D-18051 Rostock, GermanyWe demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequences for the observation of polariton effects are discussed. We find that an anti-crossing of photon and exciton dispersions exists only for states with main quantum numbers n > 28, so polariton effects do not play any role in the experiments reported up to now.https://doi.org/10.1088/1367-2630/aaa396Rydberg excitonsphonon scatteringpolaritonscuprous oxide |
spellingShingle | Heinrich Stolz Florian Schöne Dirk Semkat Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect New Journal of Physics Rydberg excitons phonon scattering polaritons cuprous oxide |
title | Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect |
title_full | Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect |
title_fullStr | Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect |
title_full_unstemmed | Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect |
title_short | Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect |
title_sort | interaction of rydberg excitons in cuprous oxide with phonons and photons optical linewidth and polariton effect |
topic | Rydberg excitons phonon scattering polaritons cuprous oxide |
url | https://doi.org/10.1088/1367-2630/aaa396 |
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