Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect

We demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequence...

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Main Authors: Heinrich Stolz, Florian Schöne, Dirk Semkat
Format: Article
Language:English
Published: IOP Publishing 2018-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/aaa396
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author Heinrich Stolz
Florian Schöne
Dirk Semkat
author_facet Heinrich Stolz
Florian Schöne
Dirk Semkat
author_sort Heinrich Stolz
collection DOAJ
description We demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequences for the observation of polariton effects are discussed. We find that an anti-crossing of photon and exciton dispersions exists only for states with main quantum numbers n  > 28, so polariton effects do not play any role in the experiments reported up to now.
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spelling doaj.art-3960583e24164e40ada547857687b2172023-08-08T14:51:06ZengIOP PublishingNew Journal of Physics1367-26302018-01-0120202301910.1088/1367-2630/aaa396Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effectHeinrich Stolz0Florian Schöne1Dirk Semkat2Institut für Physik, Universität Rostock , D-18051 Rostock, GermanyInstitut für Physik, Universität Rostock , D-18051 Rostock, GermanyInstitut für Physik, Universität Rostock , D-18051 Rostock, GermanyWe demonstrate that the optical linewidth of Rydberg excitons in Cu _2 O can be completely explained by scattering with acoustical and optical phonons, whereby the dominant contributions stems from the non-polar optical ${{\rm{\Gamma }}}_{3}^{-}$ and ${{\rm{\Gamma }}}_{5}^{-}$ modes. The consequences for the observation of polariton effects are discussed. We find that an anti-crossing of photon and exciton dispersions exists only for states with main quantum numbers n  > 28, so polariton effects do not play any role in the experiments reported up to now.https://doi.org/10.1088/1367-2630/aaa396Rydberg excitonsphonon scatteringpolaritonscuprous oxide
spellingShingle Heinrich Stolz
Florian Schöne
Dirk Semkat
Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
New Journal of Physics
Rydberg excitons
phonon scattering
polaritons
cuprous oxide
title Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
title_full Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
title_fullStr Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
title_full_unstemmed Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
title_short Interaction of Rydberg excitons in cuprous oxide with phonons and photons: optical linewidth and polariton effect
title_sort interaction of rydberg excitons in cuprous oxide with phonons and photons optical linewidth and polariton effect
topic Rydberg excitons
phonon scattering
polaritons
cuprous oxide
url https://doi.org/10.1088/1367-2630/aaa396
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AT dirksemkat interactionofrydbergexcitonsincuprousoxidewithphononsandphotonsopticallinewidthandpolaritoneffect