Bentonite Permeability at Elevated Temperature

Repository designs frequently favour geological disposal of radioactive waste with a backfill material occupying void space around the waste. The backfill material must tolerate the high temperatures produced by decaying radioactive waste to prevent its failure or degradation, leading to increased h...

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Main Authors: Katherine A. Daniels, Jon F. Harrington, Stephanie G. Zihms, Andrew C. Wiseall
Format: Article
Language:English
Published: MDPI AG 2017-01-01
Series:Geosciences
Subjects:
Online Access:http://www.mdpi.com/2076-3263/7/1/3
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author Katherine A. Daniels
Jon F. Harrington
Stephanie G. Zihms
Andrew C. Wiseall
author_facet Katherine A. Daniels
Jon F. Harrington
Stephanie G. Zihms
Andrew C. Wiseall
author_sort Katherine A. Daniels
collection DOAJ
description Repository designs frequently favour geological disposal of radioactive waste with a backfill material occupying void space around the waste. The backfill material must tolerate the high temperatures produced by decaying radioactive waste to prevent its failure or degradation, leading to increased hydraulic conductivity and reduced sealing performance. The results of four experiments investigating the effect of temperature on the permeability of a bentonite backfill are presented. Bentonite is a clay commonly proposed as the backfill in repository designs because of its high swelling capacity and very low permeability. The experiments were conducted in two sets of purpose-built, temperature controlled apparatus, designed to simulate isotropic pressure and constant volume conditions within the testing range of 4–6 MPa average effective stress. The response of bentonite during thermal loading at temperatures up to 200 °C was investigated, extending the previously considered temperature range. The results provide details of bentonite’s intrinsic permeability, total stress, swelling pressure and porewater pressure during thermal cycles. We find that bentonite’s hydraulic properties are sensitive to thermal loading and the type of imposed boundary condition. However, the permeability change is not large and can mostly be accounted for by water viscosity changes. Thus, under 150 °C, temperature has a minimal impact on bentonite’s hydraulic permeability.
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spelling doaj.art-39623477650c432982e560033160100d2022-12-22T01:57:36ZengMDPI AGGeosciences2076-32632017-01-0171310.3390/geosciences7010003geosciences7010003Bentonite Permeability at Elevated TemperatureKatherine A. Daniels0Jon F. Harrington1Stephanie G. Zihms2Andrew C. Wiseall3British Geological Survey, Nicker Hill, Keyworth, Nottinghamshire NG12 5GG, UKBritish Geological Survey, Nicker Hill, Keyworth, Nottinghamshire NG12 5GG, UKBritish Geological Survey, Nicker Hill, Keyworth, Nottinghamshire NG12 5GG, UKBritish Geological Survey, Nicker Hill, Keyworth, Nottinghamshire NG12 5GG, UKRepository designs frequently favour geological disposal of radioactive waste with a backfill material occupying void space around the waste. The backfill material must tolerate the high temperatures produced by decaying radioactive waste to prevent its failure or degradation, leading to increased hydraulic conductivity and reduced sealing performance. The results of four experiments investigating the effect of temperature on the permeability of a bentonite backfill are presented. Bentonite is a clay commonly proposed as the backfill in repository designs because of its high swelling capacity and very low permeability. The experiments were conducted in two sets of purpose-built, temperature controlled apparatus, designed to simulate isotropic pressure and constant volume conditions within the testing range of 4–6 MPa average effective stress. The response of bentonite during thermal loading at temperatures up to 200 °C was investigated, extending the previously considered temperature range. The results provide details of bentonite’s intrinsic permeability, total stress, swelling pressure and porewater pressure during thermal cycles. We find that bentonite’s hydraulic properties are sensitive to thermal loading and the type of imposed boundary condition. However, the permeability change is not large and can mostly be accounted for by water viscosity changes. Thus, under 150 °C, temperature has a minimal impact on bentonite’s hydraulic permeability.http://www.mdpi.com/2076-3263/7/1/3bentonitepermeabilitytemperatureradioactive waste disposalclay responsethermal loading
spellingShingle Katherine A. Daniels
Jon F. Harrington
Stephanie G. Zihms
Andrew C. Wiseall
Bentonite Permeability at Elevated Temperature
Geosciences
bentonite
permeability
temperature
radioactive waste disposal
clay response
thermal loading
title Bentonite Permeability at Elevated Temperature
title_full Bentonite Permeability at Elevated Temperature
title_fullStr Bentonite Permeability at Elevated Temperature
title_full_unstemmed Bentonite Permeability at Elevated Temperature
title_short Bentonite Permeability at Elevated Temperature
title_sort bentonite permeability at elevated temperature
topic bentonite
permeability
temperature
radioactive waste disposal
clay response
thermal loading
url http://www.mdpi.com/2076-3263/7/1/3
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