Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler

In order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These...

Full description

Bibliographic Details
Main Authors: Xuebin Ma, Tao Luo, Xuebin Li, Changyu Liu, Nana Liu, Qiang Liu, Kun Zhang, Jie Chen, Liming Zhu
Format: Article
Language:English
Published: MDPI AG 2024-01-01
Series:Remote Sensing
Subjects:
Online Access:https://www.mdpi.com/2072-4292/16/2/279
_version_ 1827371227214249984
author Xuebin Ma
Tao Luo
Xuebin Li
Changyu Liu
Nana Liu
Qiang Liu
Kun Zhang
Jie Chen
Liming Zhu
author_facet Xuebin Ma
Tao Luo
Xuebin Li
Changyu Liu
Nana Liu
Qiang Liu
Kun Zhang
Jie Chen
Liming Zhu
author_sort Xuebin Ma
collection DOAJ
description In order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These measurements encompassed aerosol particle size distribution as well as standard meteorological parameters including temperature, humidity, atmospheric pressure, and wind speed. Subsequently, this dataset was employed to develop an optimization algorithm for retrieving the equivalent complex refractive indices of near-surface aerosols. The methodology relies on lookup tables containing data for extinction efficiency and absorption efficiency factors. It operates on the premise of aerosol property stability within a defined time frame, utilizing measured extinction and absorption coefficients as simultaneous constraints during this period to inversely derive both the real and imaginary parts of the aerosol complex refractive index. Results from the simulation analysis reveal that the newly optimized retrieval algorithm, which relies on lookup tables, exhibits reduced sensitivity to instrument errors when compared to single-point constraint algorithms. This enhancement results in a more efficient and dependable approach for retrieving the aerosol complex refractive index. Empirical inversion and simulation studies were carried out to determine the aerosol equivalent complex refractive index in the Hefei region, utilizing measured data. This inversion process yielded an average complex refractive index of 1.48-i0.017 for aerosols in the Hefei region throughout the experimental period. Correlation analysis unveiled a positive association between the real part of the aerosol complex refractive index and the single-scattering albedo (SSA), whereas the imaginary part displayed a linear negative correlation with the SSA. The mathematical relationship between the real part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mn>0.19</mn><mi>x</mi><mo>+</mo><mn>0.62</mn></mrow></semantics></math></inline-formula>, and the corresponding relationship between the imaginary part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mo>−</mo><mn>5.3</mn><mi>x</mi><mo>+</mo><mn>0.99</mn></mrow></semantics></math></inline-formula>. This research offers a novel method for the retrieval of the aerosol equivalent complex refractive index.
first_indexed 2024-03-08T10:36:13Z
format Article
id doaj.art-3a7f4c21cee04254bf76826d7ce352e0
institution Directory Open Access Journal
issn 2072-4292
language English
last_indexed 2024-03-08T10:36:13Z
publishDate 2024-01-01
publisher MDPI AG
record_format Article
series Remote Sensing
spelling doaj.art-3a7f4c21cee04254bf76826d7ce352e02024-01-26T18:17:29ZengMDPI AGRemote Sensing2072-42922024-01-0116227910.3390/rs16020279Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle ProfilerXuebin Ma0Tao Luo1Xuebin Li2Changyu Liu3Nana Liu4Qiang Liu5Kun Zhang6Jie Chen7Liming Zhu8Key Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaIn order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These measurements encompassed aerosol particle size distribution as well as standard meteorological parameters including temperature, humidity, atmospheric pressure, and wind speed. Subsequently, this dataset was employed to develop an optimization algorithm for retrieving the equivalent complex refractive indices of near-surface aerosols. The methodology relies on lookup tables containing data for extinction efficiency and absorption efficiency factors. It operates on the premise of aerosol property stability within a defined time frame, utilizing measured extinction and absorption coefficients as simultaneous constraints during this period to inversely derive both the real and imaginary parts of the aerosol complex refractive index. Results from the simulation analysis reveal that the newly optimized retrieval algorithm, which relies on lookup tables, exhibits reduced sensitivity to instrument errors when compared to single-point constraint algorithms. This enhancement results in a more efficient and dependable approach for retrieving the aerosol complex refractive index. Empirical inversion and simulation studies were carried out to determine the aerosol equivalent complex refractive index in the Hefei region, utilizing measured data. This inversion process yielded an average complex refractive index of 1.48-i0.017 for aerosols in the Hefei region throughout the experimental period. Correlation analysis unveiled a positive association between the real part of the aerosol complex refractive index and the single-scattering albedo (SSA), whereas the imaginary part displayed a linear negative correlation with the SSA. The mathematical relationship between the real part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mn>0.19</mn><mi>x</mi><mo>+</mo><mn>0.62</mn></mrow></semantics></math></inline-formula>, and the corresponding relationship between the imaginary part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mo>−</mo><mn>5.3</mn><mi>x</mi><mo>+</mo><mn>0.99</mn></mrow></semantics></math></inline-formula>. This research offers a novel method for the retrieval of the aerosol equivalent complex refractive index.https://www.mdpi.com/2072-4292/16/2/279aerosolmicro-pulse lidarPortable Optical Particle ProfilerAethalometercomplex refractive indexlookup table
spellingShingle Xuebin Ma
Tao Luo
Xuebin Li
Changyu Liu
Nana Liu
Qiang Liu
Kun Zhang
Jie Chen
Liming Zhu
Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
Remote Sensing
aerosol
micro-pulse lidar
Portable Optical Particle Profiler
Aethalometer
complex refractive index
lookup table
title Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
title_full Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
title_fullStr Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
title_full_unstemmed Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
title_short Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
title_sort inversion of near surface aerosol equivalent complex refractive index based on aethalometer micro pulse lidar and portable optical particle profiler
topic aerosol
micro-pulse lidar
Portable Optical Particle Profiler
Aethalometer
complex refractive index
lookup table
url https://www.mdpi.com/2072-4292/16/2/279
work_keys_str_mv AT xuebinma inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT taoluo inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT xuebinli inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT changyuliu inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT nanaliu inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT qiangliu inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT kunzhang inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT jiechen inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler
AT limingzhu inversionofnearsurfaceaerosolequivalentcomplexrefractiveindexbasedonaethalometermicropulselidarandportableopticalparticleprofiler