Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler
In order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These...
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2024-01-01
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author | Xuebin Ma Tao Luo Xuebin Li Changyu Liu Nana Liu Qiang Liu Kun Zhang Jie Chen Liming Zhu |
author_facet | Xuebin Ma Tao Luo Xuebin Li Changyu Liu Nana Liu Qiang Liu Kun Zhang Jie Chen Liming Zhu |
author_sort | Xuebin Ma |
collection | DOAJ |
description | In order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These measurements encompassed aerosol particle size distribution as well as standard meteorological parameters including temperature, humidity, atmospheric pressure, and wind speed. Subsequently, this dataset was employed to develop an optimization algorithm for retrieving the equivalent complex refractive indices of near-surface aerosols. The methodology relies on lookup tables containing data for extinction efficiency and absorption efficiency factors. It operates on the premise of aerosol property stability within a defined time frame, utilizing measured extinction and absorption coefficients as simultaneous constraints during this period to inversely derive both the real and imaginary parts of the aerosol complex refractive index. Results from the simulation analysis reveal that the newly optimized retrieval algorithm, which relies on lookup tables, exhibits reduced sensitivity to instrument errors when compared to single-point constraint algorithms. This enhancement results in a more efficient and dependable approach for retrieving the aerosol complex refractive index. Empirical inversion and simulation studies were carried out to determine the aerosol equivalent complex refractive index in the Hefei region, utilizing measured data. This inversion process yielded an average complex refractive index of 1.48-i0.017 for aerosols in the Hefei region throughout the experimental period. Correlation analysis unveiled a positive association between the real part of the aerosol complex refractive index and the single-scattering albedo (SSA), whereas the imaginary part displayed a linear negative correlation with the SSA. The mathematical relationship between the real part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mn>0.19</mn><mi>x</mi><mo>+</mo><mn>0.62</mn></mrow></semantics></math></inline-formula>, and the corresponding relationship between the imaginary part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mo>−</mo><mn>5.3</mn><mi>x</mi><mo>+</mo><mn>0.99</mn></mrow></semantics></math></inline-formula>. This research offers a novel method for the retrieval of the aerosol equivalent complex refractive index. |
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spelling | doaj.art-3a7f4c21cee04254bf76826d7ce352e02024-01-26T18:17:29ZengMDPI AGRemote Sensing2072-42922024-01-0116227910.3390/rs16020279Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle ProfilerXuebin Ma0Tao Luo1Xuebin Li2Changyu Liu3Nana Liu4Qiang Liu5Kun Zhang6Jie Chen7Liming Zhu8Key Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaKey Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, ChinaIn order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These measurements encompassed aerosol particle size distribution as well as standard meteorological parameters including temperature, humidity, atmospheric pressure, and wind speed. Subsequently, this dataset was employed to develop an optimization algorithm for retrieving the equivalent complex refractive indices of near-surface aerosols. The methodology relies on lookup tables containing data for extinction efficiency and absorption efficiency factors. It operates on the premise of aerosol property stability within a defined time frame, utilizing measured extinction and absorption coefficients as simultaneous constraints during this period to inversely derive both the real and imaginary parts of the aerosol complex refractive index. Results from the simulation analysis reveal that the newly optimized retrieval algorithm, which relies on lookup tables, exhibits reduced sensitivity to instrument errors when compared to single-point constraint algorithms. This enhancement results in a more efficient and dependable approach for retrieving the aerosol complex refractive index. Empirical inversion and simulation studies were carried out to determine the aerosol equivalent complex refractive index in the Hefei region, utilizing measured data. This inversion process yielded an average complex refractive index of 1.48-i0.017 for aerosols in the Hefei region throughout the experimental period. Correlation analysis unveiled a positive association between the real part of the aerosol complex refractive index and the single-scattering albedo (SSA), whereas the imaginary part displayed a linear negative correlation with the SSA. The mathematical relationship between the real part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mn>0.19</mn><mi>x</mi><mo>+</mo><mn>0.62</mn></mrow></semantics></math></inline-formula>, and the corresponding relationship between the imaginary part and the SSA is <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mi>y</mi><mo>=</mo><mo>−</mo><mn>5.3</mn><mi>x</mi><mo>+</mo><mn>0.99</mn></mrow></semantics></math></inline-formula>. This research offers a novel method for the retrieval of the aerosol equivalent complex refractive index.https://www.mdpi.com/2072-4292/16/2/279aerosolmicro-pulse lidarPortable Optical Particle ProfilerAethalometercomplex refractive indexlookup table |
spellingShingle | Xuebin Ma Tao Luo Xuebin Li Changyu Liu Nana Liu Qiang Liu Kun Zhang Jie Chen Liming Zhu Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler Remote Sensing aerosol micro-pulse lidar Portable Optical Particle Profiler Aethalometer complex refractive index lookup table |
title | Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler |
title_full | Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler |
title_fullStr | Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler |
title_full_unstemmed | Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler |
title_short | Inversion of Near-Surface Aerosol Equivalent Complex Refractive Index Based on Aethalometer, Micro-Pulse Lidar and Portable Optical Particle Profiler |
title_sort | inversion of near surface aerosol equivalent complex refractive index based on aethalometer micro pulse lidar and portable optical particle profiler |
topic | aerosol micro-pulse lidar Portable Optical Particle Profiler Aethalometer complex refractive index lookup table |
url | https://www.mdpi.com/2072-4292/16/2/279 |
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