Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes

Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-...

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Main Authors: Kevin N. Wood, K. Xerxes Steirer, Simon E. Hafner, Chunmei Ban, Shriram Santhanagopalan, Se-Hee Lee, Glenn Teeter
Format: Article
Language:English
Published: Nature Portfolio 2018-06-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-018-04762-z
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author Kevin N. Wood
K. Xerxes Steirer
Simon E. Hafner
Chunmei Ban
Shriram Santhanagopalan
Se-Hee Lee
Glenn Teeter
author_facet Kevin N. Wood
K. Xerxes Steirer
Simon E. Hafner
Chunmei Ban
Shriram Santhanagopalan
Se-Hee Lee
Glenn Teeter
author_sort Kevin N. Wood
collection DOAJ
description Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling.
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spelling doaj.art-3b0325b8fd93416e85ed8fb7adb46f142022-12-21T21:53:01ZengNature PortfolioNature Communications2041-17232018-06-019111010.1038/s41467-018-04762-zOperando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytesKevin N. Wood0K. Xerxes Steirer1Simon E. Hafner2Chunmei Ban3Shriram Santhanagopalan4Se-Hee Lee5Glenn Teeter6National Renewable Energy LaboratoryColorado School of MinesUniversity of ColoradoNational Renewable Energy LaboratoryNational Renewable Energy LaboratoryUniversity of ColoradoNational Renewable Energy LaboratorySolid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling.https://doi.org/10.1038/s41467-018-04762-z
spellingShingle Kevin N. Wood
K. Xerxes Steirer
Simon E. Hafner
Chunmei Ban
Shriram Santhanagopalan
Se-Hee Lee
Glenn Teeter
Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
Nature Communications
title Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_full Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_fullStr Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_full_unstemmed Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_short Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_sort operando x ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in li2s p2s5 solid state electrolytes
url https://doi.org/10.1038/s41467-018-04762-z
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