Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-...
Main Authors: | , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Nature Portfolio
2018-06-01
|
Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-018-04762-z |
_version_ | 1818681969800642560 |
---|---|
author | Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter |
author_facet | Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter |
author_sort | Kevin N. Wood |
collection | DOAJ |
description | Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling. |
first_indexed | 2024-12-17T10:11:24Z |
format | Article |
id | doaj.art-3b0325b8fd93416e85ed8fb7adb46f14 |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-17T10:11:24Z |
publishDate | 2018-06-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-3b0325b8fd93416e85ed8fb7adb46f142022-12-21T21:53:01ZengNature PortfolioNature Communications2041-17232018-06-019111010.1038/s41467-018-04762-zOperando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytesKevin N. Wood0K. Xerxes Steirer1Simon E. Hafner2Chunmei Ban3Shriram Santhanagopalan4Se-Hee Lee5Glenn Teeter6National Renewable Energy LaboratoryColorado School of MinesUniversity of ColoradoNational Renewable Energy LaboratoryNational Renewable Energy LaboratoryUniversity of ColoradoNational Renewable Energy LaboratorySolid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling.https://doi.org/10.1038/s41467-018-04762-z |
spellingShingle | Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes Nature Communications |
title | Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes |
title_full | Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes |
title_fullStr | Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes |
title_full_unstemmed | Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes |
title_short | Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes |
title_sort | operando x ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in li2s p2s5 solid state electrolytes |
url | https://doi.org/10.1038/s41467-018-04762-z |
work_keys_str_mv | AT kevinnwood operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT kxerxessteirer operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT simonehafner operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT chunmeiban operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT shriramsanthanagopalan operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT seheelee operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT glennteeter operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes |