New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo

Abstract A new study of double beta decay processes in natural Zr isotopes using Zr metal samples and an ultra-low-background high-purity germanium detectors was performed at Laboratori Nazionali del Gran Sasso of INFN (Italy). Two data sets were collected with a 736.35 g and a 129.94 g Zr metal ove...

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Main Authors: E. Celi, M. Ješkovský, M. Laubenstein, S. S. Nagorny, V. V. Nahorna, S. Nisi, L. Pagnanini, P. Povinec, P. Wang
Format: Article
Language:English
Published: SpringerOpen 2023-05-01
Series:European Physical Journal C: Particles and Fields
Online Access:https://doi.org/10.1140/epjc/s10052-023-11516-9
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author E. Celi
M. Ješkovský
M. Laubenstein
S. S. Nagorny
V. V. Nahorna
S. Nisi
L. Pagnanini
P. Povinec
P. Wang
author_facet E. Celi
M. Ješkovský
M. Laubenstein
S. S. Nagorny
V. V. Nahorna
S. Nisi
L. Pagnanini
P. Povinec
P. Wang
author_sort E. Celi
collection DOAJ
description Abstract A new study of double beta decay processes in natural Zr isotopes using Zr metal samples and an ultra-low-background high-purity germanium detectors was performed at Laboratori Nazionali del Gran Sasso of INFN (Italy). Two data sets were collected with a 736.35 g and a 129.94 g Zr metal over 59.7 days and 37.3 days, respectively, and were used for a detailed analysis. A new limit on the double beta decay of $$^{94}$$ 94 Zr to the 1st excited level of $$^{94}$$ 94 Mo was set as $$T_{1/2}^{\beta \beta } > 2.1\times 10^{20}~\text {year}$$ T 1 / 2 β β > 2.1 × 10 20 year , which is a factor of three better than the previous result. It is shown that the current radiopurity of Zr metal (tens of Bq/kg), produced via two methods, do not comply with the radiopurity requirements for low-background experiments. Hence, we propose to use a purified ZrCl $$_{4}$$ 4 powder in an optimized geometry as a new approach for future experiments with extended sensitivity focused on studies of rare nuclear processes in Zr isotopes.
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spelling doaj.art-3b5fa2231e4f4d2695f00b01590c8acb2023-07-02T11:25:13ZengSpringerOpenEuropean Physical Journal C: Particles and Fields1434-60522023-05-018351810.1140/epjc/s10052-023-11516-9New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 MoE. Celi0M. Ješkovský1M. Laubenstein2S. S. Nagorny3V. V. Nahorna4S. Nisi5L. Pagnanini6P. Povinec7P. Wang8Gran Sasso Science InstituteFaculty of Mathematics, Physics and Informatics, Comenius UniversityINFN-Laboratori Nazionali del Gran SassoDepartment of Physics, Engineering Physics and Astronomy, Queen’s UniversityDepartment of Chemistry, Queen’s UniversityINFN-Laboratori Nazionali del Gran SassoGran Sasso Science InstituteFaculty of Mathematics, Physics and Informatics, Comenius UniversityArthur B. McDonald Canadian Astroparticle Physics Research InstituteAbstract A new study of double beta decay processes in natural Zr isotopes using Zr metal samples and an ultra-low-background high-purity germanium detectors was performed at Laboratori Nazionali del Gran Sasso of INFN (Italy). Two data sets were collected with a 736.35 g and a 129.94 g Zr metal over 59.7 days and 37.3 days, respectively, and were used for a detailed analysis. A new limit on the double beta decay of $$^{94}$$ 94 Zr to the 1st excited level of $$^{94}$$ 94 Mo was set as $$T_{1/2}^{\beta \beta } > 2.1\times 10^{20}~\text {year}$$ T 1 / 2 β β > 2.1 × 10 20 year , which is a factor of three better than the previous result. It is shown that the current radiopurity of Zr metal (tens of Bq/kg), produced via two methods, do not comply with the radiopurity requirements for low-background experiments. Hence, we propose to use a purified ZrCl $$_{4}$$ 4 powder in an optimized geometry as a new approach for future experiments with extended sensitivity focused on studies of rare nuclear processes in Zr isotopes.https://doi.org/10.1140/epjc/s10052-023-11516-9
spellingShingle E. Celi
M. Ješkovský
M. Laubenstein
S. S. Nagorny
V. V. Nahorna
S. Nisi
L. Pagnanini
P. Povinec
P. Wang
New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
European Physical Journal C: Particles and Fields
title New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
title_full New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
title_fullStr New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
title_full_unstemmed New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
title_short New limit on $$^{94}$$ 94 Zr double beta decay to the 1st excited state of $$^{94}$$ 94 Mo
title_sort new limit on 94 94 zr double beta decay to the 1st excited state of 94 94 mo
url https://doi.org/10.1140/epjc/s10052-023-11516-9
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