Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass

The Faraday rotation originates from the mechanism by which the time‐reversal symmetry in the material is broken by the external magnetic field. It is the basis for the development of some magneto‐optical devices, such as optical isolators. In integrated optics and telecommunications, nonreciprocal...

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Main Authors: Han Zhu, Mingsheng Gao, Chi Pang, Rang Li, Lingrui Chu, Feng Ren, Wei Qin, Feng Chen
Format: Article
Language:English
Published: Wiley-VCH 2022-04-01
Series:Small Science
Subjects:
Online Access:https://doi.org/10.1002/smsc.202100094
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author Han Zhu
Mingsheng Gao
Chi Pang
Rang Li
Lingrui Chu
Feng Ren
Wei Qin
Feng Chen
author_facet Han Zhu
Mingsheng Gao
Chi Pang
Rang Li
Lingrui Chu
Feng Ren
Wei Qin
Feng Chen
author_sort Han Zhu
collection DOAJ
description The Faraday rotation originates from the mechanism by which the time‐reversal symmetry in the material is broken by the external magnetic field. It is the basis for the development of some magneto‐optical devices, such as optical isolators. In integrated optics and telecommunications, nonreciprocal photonic devices with high transmittance and strong Faraday rotation are desired for low‐cost, compact optical systems. Localized surface plasmon resonance (LSPR) from the metallic nanoparticles in dielectrics allows the light localization in subwavelength scales, boosting the interaction between nanoparticles and materials, which results in a number of plasmon‐enhanced effects. Herein, the strong Faraday rotation in BK7 glass by embedded metallic nanoparticles through LSPR is reported. It is elucidated that the mechanism of Faraday rotation is the near‐field enhancement of spin–photon coupling effect in the presence of an external magnetic field. The Verdet constant of the thin‐layer BK7 glass with embedded Au nanoparticles is determined as high as 5059.7 rad T−1 m−1 at 532 nm, exhibiting excellent magneto‐optical features. This work opens a new avenue to develop the subwavelength magneto‐optical devices with embedded metallic nanoparticles.
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spelling doaj.art-3b6333fb816546528037d93b7584af452022-12-21T21:59:39ZengWiley-VCHSmall Science2688-40462022-04-0124n/an/a10.1002/smsc.202100094Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in GlassHan Zhu0Mingsheng Gao1Chi Pang2Rang Li3Lingrui Chu4Feng Ren5Wei Qin6Feng Chen7School of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaSchool of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaSchool of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaInstitute of Ion Beam Physics and Materials Research Helmholtz-Zentrum Dresden-Rossendorf 01328 Dresden GermanySchool of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaDepartment of Physics Center for Ion Beam Application and Center for Electron Microscopy Wuhan University Wuhan 430072 ChinaSchool of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaSchool of Physics State Key Laboratory of Crystal Materials Shandong University Jinan 250100 ChinaThe Faraday rotation originates from the mechanism by which the time‐reversal symmetry in the material is broken by the external magnetic field. It is the basis for the development of some magneto‐optical devices, such as optical isolators. In integrated optics and telecommunications, nonreciprocal photonic devices with high transmittance and strong Faraday rotation are desired for low‐cost, compact optical systems. Localized surface plasmon resonance (LSPR) from the metallic nanoparticles in dielectrics allows the light localization in subwavelength scales, boosting the interaction between nanoparticles and materials, which results in a number of plasmon‐enhanced effects. Herein, the strong Faraday rotation in BK7 glass by embedded metallic nanoparticles through LSPR is reported. It is elucidated that the mechanism of Faraday rotation is the near‐field enhancement of spin–photon coupling effect in the presence of an external magnetic field. The Verdet constant of the thin‐layer BK7 glass with embedded Au nanoparticles is determined as high as 5059.7 rad T−1 m−1 at 532 nm, exhibiting excellent magneto‐optical features. This work opens a new avenue to develop the subwavelength magneto‐optical devices with embedded metallic nanoparticles.https://doi.org/10.1002/smsc.202100094Faraday rotationintegrated photonic devicesion implantationlocalized surface plasmon resonanceorbital angular momentum
spellingShingle Han Zhu
Mingsheng Gao
Chi Pang
Rang Li
Lingrui Chu
Feng Ren
Wei Qin
Feng Chen
Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
Small Science
Faraday rotation
integrated photonic devices
ion implantation
localized surface plasmon resonance
orbital angular momentum
title Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
title_full Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
title_fullStr Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
title_full_unstemmed Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
title_short Strong Faraday Rotation Based on Localized Surface Plasmon Enhancement of Embedded Metallic Nanoparticles in Glass
title_sort strong faraday rotation based on localized surface plasmon enhancement of embedded metallic nanoparticles in glass
topic Faraday rotation
integrated photonic devices
ion implantation
localized surface plasmon resonance
orbital angular momentum
url https://doi.org/10.1002/smsc.202100094
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AT lingruichu strongfaradayrotationbasedonlocalizedsurfaceplasmonenhancementofembeddedmetallicnanoparticlesinglass
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