Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation

A molecular-level understanding of the electronic effects remains a grand challenge in heterogeneous catalysis. Here, the authors report an unconventional kinetics strategy for bridging the upscaling gap between the microscopic fingerprints of active sites and the macroscopic catalytic performance.

Bibliographic Details
Main Authors: Wenyao Chen, Junbo Cao, Jia Yang, Yueqiang Cao, Hao Zhang, Zheng Jiang, Jing Zhang, Gang Qian, Xinggui Zhou, De Chen, Weikang Yuan, Xuezhi Duan
Format: Article
Language:English
Published: Nature Portfolio 2021-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-27238-z
_version_ 1819036570630488064
author Wenyao Chen
Junbo Cao
Jia Yang
Yueqiang Cao
Hao Zhang
Zheng Jiang
Jing Zhang
Gang Qian
Xinggui Zhou
De Chen
Weikang Yuan
Xuezhi Duan
author_facet Wenyao Chen
Junbo Cao
Jia Yang
Yueqiang Cao
Hao Zhang
Zheng Jiang
Jing Zhang
Gang Qian
Xinggui Zhou
De Chen
Weikang Yuan
Xuezhi Duan
author_sort Wenyao Chen
collection DOAJ
description A molecular-level understanding of the electronic effects remains a grand challenge in heterogeneous catalysis. Here, the authors report an unconventional kinetics strategy for bridging the upscaling gap between the microscopic fingerprints of active sites and the macroscopic catalytic performance.
first_indexed 2024-12-21T08:07:37Z
format Article
id doaj.art-3bc3cd4701074e56af88faa5859a2f76
institution Directory Open Access Journal
issn 2041-1723
language English
last_indexed 2024-12-21T08:07:37Z
publishDate 2021-11-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj.art-3bc3cd4701074e56af88faa5859a2f762022-12-21T19:10:44ZengNature PortfolioNature Communications2041-17232021-11-0112111110.1038/s41467-021-27238-zMolecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidationWenyao Chen0Junbo Cao1Jia Yang2Yueqiang Cao3Hao Zhang4Zheng Jiang5Jing Zhang6Gang Qian7Xinggui Zhou8De Chen9Weikang Yuan10Xuezhi Duan11State Key Laboratory of Chemical Engineering, East China University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyDepartment of Chemical Engineering, Norwegian University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyInstitute of Functional Nano & Soft Materials Laboratory (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow UniversityShanghai Institute of Applied Physics, Chinese Academy of SciencesState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyDepartment of Chemical Engineering, Norwegian University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyState Key Laboratory of Chemical Engineering, East China University of Science and TechnologyA molecular-level understanding of the electronic effects remains a grand challenge in heterogeneous catalysis. Here, the authors report an unconventional kinetics strategy for bridging the upscaling gap between the microscopic fingerprints of active sites and the macroscopic catalytic performance.https://doi.org/10.1038/s41467-021-27238-z
spellingShingle Wenyao Chen
Junbo Cao
Jia Yang
Yueqiang Cao
Hao Zhang
Zheng Jiang
Jing Zhang
Gang Qian
Xinggui Zhou
De Chen
Weikang Yuan
Xuezhi Duan
Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
Nature Communications
title Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
title_full Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
title_fullStr Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
title_full_unstemmed Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
title_short Molecular-level insights into the electronic effects in platinum-catalyzed carbon monoxide oxidation
title_sort molecular level insights into the electronic effects in platinum catalyzed carbon monoxide oxidation
url https://doi.org/10.1038/s41467-021-27238-z
work_keys_str_mv AT wenyaochen molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT junbocao molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT jiayang molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT yueqiangcao molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT haozhang molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT zhengjiang molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT jingzhang molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT gangqian molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT xingguizhou molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT dechen molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT weikangyuan molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation
AT xuezhiduan molecularlevelinsightsintotheelectroniceffectsinplatinumcatalyzedcarbonmonoxideoxidation