Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application

Ultrafiltration (UF) has been increasingly implemented in drinking water treatment plants; however, algae and their secretions can cause severe membrane fouling and pose great challenges to UF in practice. In this study, a simple and practical chemically enhanced backwashing (CEB) process was develo...

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Main Authors: Xiaobin Tang, Tiecheng Guo, Haiqing Chang, Xiao Yue, Jinlong Wang, Haikuan Yu, Binghan Xie, Xuewu Zhu, Guibai Li, Heng Liang
Format: Article
Language:English
Published: Elsevier 2022-12-01
Series:Engineering
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2095809921001624
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author Xiaobin Tang
Tiecheng Guo
Haiqing Chang
Xiao Yue
Jinlong Wang
Haikuan Yu
Binghan Xie
Xuewu Zhu
Guibai Li
Heng Liang
author_facet Xiaobin Tang
Tiecheng Guo
Haiqing Chang
Xiao Yue
Jinlong Wang
Haikuan Yu
Binghan Xie
Xuewu Zhu
Guibai Li
Heng Liang
author_sort Xiaobin Tang
collection DOAJ
description Ultrafiltration (UF) has been increasingly implemented in drinking water treatment plants; however, algae and their secretions can cause severe membrane fouling and pose great challenges to UF in practice. In this study, a simple and practical chemically enhanced backwashing (CEB) process was developed to address such issues using various cleaning reagents, including sodium hypochlorite (NaClO), sodium chloride (NaCl), sodium hydroxide (NaOH), sodium citrate, and their combinations. The results indicate that the type of chemical played a fundamental role in alleviating the hydraulically irreversible membrane fouling (HIMF), with NaClO as the best-performing reagent, followed by NaCl. Furthermore, a CEB process using a combination of NaClO with NaCl, NaOH, or sodium citrate delivered little improvement in the alleviation of membrane fouling compared with NaClO alone. The optimized dosage and dosing frequency of NaClO were 10 mg·L−1 two times per day. Long-term pilot-scale and full-scale experiments further verified the feasibility of the CEB process in relieving algae-derived membrane fouling. Compared with the conventional hydraulic backwashing without chemical involvement, the CEB process can effectively remove the organic foulants including biopolymers, humic substances, and protein-like substances by means of oxidization, thereby weakening the cohesive forces between the organic foulants and the membrane surface. Therefore, the CEB process can efficiently alleviate the algae-related membrane fouling with lower chemical consumption, and is proposed as an alternative to control membrane fouling in treating the algae-containing surface water.
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spelling doaj.art-3dbaac4cb41b440dbb585a4b507da3d52023-03-09T04:13:14ZengElsevierEngineering2095-80992022-12-01194049Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale ApplicationXiaobin Tang0Tiecheng Guo1Haiqing Chang2Xiao Yue3Jinlong Wang4Haikuan Yu5Binghan Xie6Xuewu Zhu7Guibai Li8Heng Liang9State Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, ChinaState Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, ChinaCollege of Architecture and Environment, Sichuan University, Chengdu 610207, ChinaCollege of Architecture and Civil Engineering, Beijing University of Technology, Beijing 100124, ChinaState Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, ChinaCollege of Architecture and Civil Engineering, Beijing University of Technology, Beijing 100124, ChinaSchool of Marine Science and Technology, Harbin Institute of Technology at Weihai, Weihai 264209, ChinaState Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, ChinaState Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, ChinaState Key Laboratory of Urban Water Resource and Environment (SKLUWRE), School of Environment, Harbin Institute of Technology, Harbin 150090, China; Corresponding author.Ultrafiltration (UF) has been increasingly implemented in drinking water treatment plants; however, algae and their secretions can cause severe membrane fouling and pose great challenges to UF in practice. In this study, a simple and practical chemically enhanced backwashing (CEB) process was developed to address such issues using various cleaning reagents, including sodium hypochlorite (NaClO), sodium chloride (NaCl), sodium hydroxide (NaOH), sodium citrate, and their combinations. The results indicate that the type of chemical played a fundamental role in alleviating the hydraulically irreversible membrane fouling (HIMF), with NaClO as the best-performing reagent, followed by NaCl. Furthermore, a CEB process using a combination of NaClO with NaCl, NaOH, or sodium citrate delivered little improvement in the alleviation of membrane fouling compared with NaClO alone. The optimized dosage and dosing frequency of NaClO were 10 mg·L−1 two times per day. Long-term pilot-scale and full-scale experiments further verified the feasibility of the CEB process in relieving algae-derived membrane fouling. Compared with the conventional hydraulic backwashing without chemical involvement, the CEB process can effectively remove the organic foulants including biopolymers, humic substances, and protein-like substances by means of oxidization, thereby weakening the cohesive forces between the organic foulants and the membrane surface. Therefore, the CEB process can efficiently alleviate the algae-related membrane fouling with lower chemical consumption, and is proposed as an alternative to control membrane fouling in treating the algae-containing surface water.http://www.sciencedirect.com/science/article/pii/S2095809921001624UltrafiltrationMembrane foulingHydraulically irreversible membrane foulingChemically enhanced backwashing (CEB)Algae-containing surface water
spellingShingle Xiaobin Tang
Tiecheng Guo
Haiqing Chang
Xiao Yue
Jinlong Wang
Haikuan Yu
Binghan Xie
Xuewu Zhu
Guibai Li
Heng Liang
Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
Engineering
Ultrafiltration
Membrane fouling
Hydraulically irreversible membrane fouling
Chemically enhanced backwashing (CEB)
Algae-containing surface water
title Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
title_full Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
title_fullStr Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
title_full_unstemmed Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
title_short Membrane Fouling Alleviation by Chemically Enhanced Backwashing in Treating Algae-Containing Surface Water: From Bench-Scale to Full-Scale Application
title_sort membrane fouling alleviation by chemically enhanced backwashing in treating algae containing surface water from bench scale to full scale application
topic Ultrafiltration
Membrane fouling
Hydraulically irreversible membrane fouling
Chemically enhanced backwashing (CEB)
Algae-containing surface water
url http://www.sciencedirect.com/science/article/pii/S2095809921001624
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