On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.

In the view of transmutation of transuranium (TRU) elements, molten salt fast reactors (MSFRs) offer certain advantages compared to solid fuelled reactor types like sodium cooled fast reactors (SFRs). In the first part these advantages are discussed in comparison with the SFR technology, and the res...

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Main Authors: Bruno Merk, Ulrich Rohde, Varvara Glivici-Cotruţă, Dzianis Litskevich, Susanne Scholl
Format: Article
Language:English
Published: Public Library of Science (PLoS) 2014-01-01
Series:PLoS ONE
Online Access:https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0092776&type=printable
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author Bruno Merk
Ulrich Rohde
Varvara Glivici-Cotruţă
Dzianis Litskevich
Susanne Scholl
author_facet Bruno Merk
Ulrich Rohde
Varvara Glivici-Cotruţă
Dzianis Litskevich
Susanne Scholl
author_sort Bruno Merk
collection DOAJ
description In the view of transmutation of transuranium (TRU) elements, molten salt fast reactors (MSFRs) offer certain advantages compared to solid fuelled reactor types like sodium cooled fast reactors (SFRs). In the first part these advantages are discussed in comparison with the SFR technology, and the research challenges are analyzed. In the second part cycle studies for the MSFR are given for different configurations--a core with U-238 fertile, a fertile free core, and a core with Th-232 as fertile material. For all cases, the transmutation potential is determined and efficient transmutation performance for the case with thorium as a fertile material as well as for the fertile free case is demonstrated and the individual advantages are discussed. The time evolution of different important isotopes is analyzed. In the third part a strategy for the optimization of the transmutation efficiency is developed. The final aim is dictated by the phase out decision of the German government, which requests to put the focus on the determination of the maximal transmutation efficiency and on an as much as possible reduced leftover of transuranium elements at the end of the reactor life. This minimal leftover is achieved by a two step procedure of a first transmuter operation phase followed by a second deep burning phase. There the U-233, which is bred in the blanket of the core consisting of thorium containing salt, is used as feed. It is demonstrated, that transmutation rates up to more than 90% can be achieved for all transuranium isotopes, while the production of undesired high elements like californium is very limited. Additionally, the adaptations needed for the simulation of a MSFR, and the used tool HELIOS 1.10 is described.
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spelling doaj.art-3f7693bc87014ec29df4b5bf8c935ca32025-02-21T05:35:12ZengPublic Library of Science (PLoS)PLoS ONE1932-62032014-01-0194e9277610.1371/journal.pone.0092776On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.Bruno MerkUlrich RohdeVarvara Glivici-CotruţăDzianis LitskevichSusanne SchollIn the view of transmutation of transuranium (TRU) elements, molten salt fast reactors (MSFRs) offer certain advantages compared to solid fuelled reactor types like sodium cooled fast reactors (SFRs). In the first part these advantages are discussed in comparison with the SFR technology, and the research challenges are analyzed. In the second part cycle studies for the MSFR are given for different configurations--a core with U-238 fertile, a fertile free core, and a core with Th-232 as fertile material. For all cases, the transmutation potential is determined and efficient transmutation performance for the case with thorium as a fertile material as well as for the fertile free case is demonstrated and the individual advantages are discussed. The time evolution of different important isotopes is analyzed. In the third part a strategy for the optimization of the transmutation efficiency is developed. The final aim is dictated by the phase out decision of the German government, which requests to put the focus on the determination of the maximal transmutation efficiency and on an as much as possible reduced leftover of transuranium elements at the end of the reactor life. This minimal leftover is achieved by a two step procedure of a first transmuter operation phase followed by a second deep burning phase. There the U-233, which is bred in the blanket of the core consisting of thorium containing salt, is used as feed. It is demonstrated, that transmutation rates up to more than 90% can be achieved for all transuranium isotopes, while the production of undesired high elements like californium is very limited. Additionally, the adaptations needed for the simulation of a MSFR, and the used tool HELIOS 1.10 is described.https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0092776&type=printable
spellingShingle Bruno Merk
Ulrich Rohde
Varvara Glivici-Cotruţă
Dzianis Litskevich
Susanne Scholl
On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
PLoS ONE
title On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
title_full On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
title_fullStr On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
title_full_unstemmed On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
title_short On the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out.
title_sort on the use of a molten salt fast reactor to apply an idealized transmutation scenario for the nuclear phase out
url https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0092776&type=printable
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