Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols

Redistribution of black carbon from the inorganic core to the organic coating of aged aerosols due to liquid-liquid phase separation can reduce radiative absorption by up to 34%, according to field observations and laboratory experiments.

Bibliographic Details
Main Authors: Jian Zhang, Yuanyuan Wang, Xiaomi Teng, Lei Liu, Yisheng Xu, Lihong Ren, Zongbo Shi, Yue Zhang, Jingkun Jiang, Dantong Liu, Min Hu, Longyi Shao, Jianmin Chen, Scot T. Martin, Xiaoye Zhang, Weijun Li
Format: Article
Language:English
Published: Nature Portfolio 2022-06-01
Series:Communications Earth & Environment
Online Access:https://doi.org/10.1038/s43247-022-00462-1
_version_ 1817970579644350464
author Jian Zhang
Yuanyuan Wang
Xiaomi Teng
Lei Liu
Yisheng Xu
Lihong Ren
Zongbo Shi
Yue Zhang
Jingkun Jiang
Dantong Liu
Min Hu
Longyi Shao
Jianmin Chen
Scot T. Martin
Xiaoye Zhang
Weijun Li
author_facet Jian Zhang
Yuanyuan Wang
Xiaomi Teng
Lei Liu
Yisheng Xu
Lihong Ren
Zongbo Shi
Yue Zhang
Jingkun Jiang
Dantong Liu
Min Hu
Longyi Shao
Jianmin Chen
Scot T. Martin
Xiaoye Zhang
Weijun Li
author_sort Jian Zhang
collection DOAJ
description Redistribution of black carbon from the inorganic core to the organic coating of aged aerosols due to liquid-liquid phase separation can reduce radiative absorption by up to 34%, according to field observations and laboratory experiments.
first_indexed 2024-04-13T20:35:58Z
format Article
id doaj.art-40bd010f63b1423b8606b05d16b4b0ae
institution Directory Open Access Journal
issn 2662-4435
language English
last_indexed 2024-04-13T20:35:58Z
publishDate 2022-06-01
publisher Nature Portfolio
record_format Article
series Communications Earth & Environment
spelling doaj.art-40bd010f63b1423b8606b05d16b4b0ae2022-12-22T02:31:02ZengNature PortfolioCommunications Earth & Environment2662-44352022-06-01311910.1038/s43247-022-00462-1Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosolsJian Zhang0Yuanyuan Wang1Xiaomi Teng2Lei Liu3Yisheng Xu4Lihong Ren5Zongbo Shi6Yue Zhang7Jingkun Jiang8Dantong Liu9Min Hu10Longyi Shao11Jianmin Chen12Scot T. Martin13Xiaoye Zhang14Weijun Li15Key Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityKey Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityKey Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityKey Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityState Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental SciencesState Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental SciencesSchool of Geography, Earth and Environmental Sciences, University of BirminghamDepartment of Atmospheric Sciences, Texas A&M UniversityState Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua UniversityKey Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityState Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking UniversityState Key Laboratory of Coal Resources and Safe Mining, China University of Mining and TechnologyShanghai Key Laboratory of Atmospheric Particle Pollution and Prevention, Department of Environmental Science and Engineering, Fudan UniversityJohn A. Paulson School of Engineering and Applied Sciences, Harvard UniversityKey Laboratory of Atmospheric Chemistry of CMA, Institute of Atmospheric Composition, Chinese Academy of Meteorological SciencesKey Laboratory of Geoscience Big Data and Deep Resource of Zhejiang Province, Department of Atmospheric Sciences, School of Earth Sciences, Zhejiang UniversityRedistribution of black carbon from the inorganic core to the organic coating of aged aerosols due to liquid-liquid phase separation can reduce radiative absorption by up to 34%, according to field observations and laboratory experiments.https://doi.org/10.1038/s43247-022-00462-1
spellingShingle Jian Zhang
Yuanyuan Wang
Xiaomi Teng
Lei Liu
Yisheng Xu
Lihong Ren
Zongbo Shi
Yue Zhang
Jingkun Jiang
Dantong Liu
Min Hu
Longyi Shao
Jianmin Chen
Scot T. Martin
Xiaoye Zhang
Weijun Li
Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
Communications Earth & Environment
title Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
title_full Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
title_fullStr Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
title_full_unstemmed Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
title_short Liquid-liquid phase separation reduces radiative absorption by aged black carbon aerosols
title_sort liquid liquid phase separation reduces radiative absorption by aged black carbon aerosols
url https://doi.org/10.1038/s43247-022-00462-1
work_keys_str_mv AT jianzhang liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT yuanyuanwang liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT xiaomiteng liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT leiliu liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT yishengxu liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT lihongren liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT zongboshi liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT yuezhang liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT jingkunjiang liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT dantongliu liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT minhu liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT longyishao liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT jianminchen liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT scottmartin liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT xiaoyezhang liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols
AT weijunli liquidliquidphaseseparationreducesradiativeabsorptionbyagedblackcarbonaerosols